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One-pot synthesis of conjugated vinylene-extended viologen ionic radical polyacetylenes for visible light-promoted photocatalytic CO2 cycloaddition

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Published On ::

Green Chem., 2024, 26,10876-10885
DOI: 10.1039/D4GC03683B, Paper
Yanan Chang, Shuo Wang, Juan Chen, Zixuan Xu, Qing Shi, Yunjie Mao, Yanli Gai, Zhouyang Long, Guojian Chen
In situ synthesis of a conjugated vinylene-extended viologen ionic radical polyacetylene (VIRP-2) for visible light-promoted photocatalytic CO2 cycloaddition under ambient conditions.
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What to do with polyurethane waste? The environmental potential of chemically recycling polyurethane rigid foam

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Green Chem., 2024, 26,10893-10906
DOI: 10.1039/D4GC02594F, Paper
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Martin Pillich, Johannes Schilling, Luca Bosetti, André Bardow
The environmental potential guides through the maze of chemical recycling of polyurethane rigid foams highlighting promising options.
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Feasibility and sustainability of emerging CCU pathways for formic acid production

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Green Chem., 2024, 26,10982-10995
DOI: 10.1039/D4GC02507E, Paper
Tesfalem Aregawi Atsbha, Ha-Jun Yoon, Ali Cherif, Chul-Jin Lee
The thermo-catalytic pathway can be a competitive alternative to the conventional pathway. CO2 source and electricity source highly affected the GWI for the thermo-catalytic pathway and electrochemical reduction pathway respectively.
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Solid phase peptide synthesis using side-chain unprotected arginine and histidine with Oxyma Pure/TBEC in green solvents

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Green Chem., 2024, 26,10929-10939
DOI: 10.1039/D4GC03209H, Paper
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Tommaso Fantoni, Andrea Orlandin, Ilaria Di Stefano, Marco Macis, Alessandra Tolomelli, Antonio Ricci, Walter Cabri, Lucia Ferrazzano
Oxyma Pure/TBEC coupling protocol in green solid phase peptide synthesis (GSPPS) eliminates protective groups on Arg and His, enhancing atom economy and reducing impurities during cleavage. The technology was extended to side-chain-free Tyr and Trp.
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Light-driven ultrafast dual C–C cleavage and coupling of dihydroxyacetone into high-purity carbon monoxide and ethylene glycol

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Green Chem., 2024, 26,10859-10866
DOI: 10.1039/D4GC04180A, Paper
Fanhao Kong, Hongru Zhou, Zhiwei Chen, Zhaolin Dou, Min Wang
Reforming of biomass-based dihydroxyacetone to produce high-purity CO and ethylene glycol is achieved via a distinctive photochemical process under ambient conditions.
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Evaluation on the recovery of lignin from basic [Ch][Lys] systems using low-cost alcohols as anti-solvents under acid-free conditions

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Published On ::

Green Chem., 2024, 26,10950-10959
DOI: 10.1039/D4GC03898C, Paper
Yichen Liu, Wanting Zhao, Qizhen Luo, Jipeng Yan, Jian Sun
An acid-free, high efficiency, and mild method of precipitating and separating lignin from basic ionic liquids (BIL) such as choline lysinate ([Ch][Lys]) by using alchohols (such as tert-butanol) as anti--solvents.
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Straightforward solid-phase modification of TiO2 with propylphosphonic acid via manual grinding and shaker mixing: enhancing modification degree by thermal control while improving atom economy

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Published On ::

Green Chem., 2024, 26,10907-10920
DOI: 10.1039/D4GC03330B, Paper
Open Access
Kaimin Zhang, Jinxin Wang, Nick Gys, Elien Derveaux, Nahal Ghanemnia, Wouter Marchal, Peter Adriaensens, Vera Meynen
The straightforward manual grinding method achieves controllable grafting of organophosphonic acid onto TiO2, demonstrating its atom economy and greenness.
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Monoliths enabling biocatalysis in flow chemistry

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Green Chem., 2024, 26,10718-10738
DOI: 10.1039/D4GC03535F, Critical Review
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Aleksandra Lambarska, Katarzyna Szymańska, Ulf Hanefeld
Biocatalysis in flow improves space time yields and enables straightforward downstream processing. The underlying principles of monolithic flow reactors and their application in mono- and bi-phasic biocatalytic systems are discussed.
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Lipase-entrapped colloidosomes with light-responsive wettability for efficient and recyclable Pickering interfacial biocatalysis

By pubs.rsc.org
Published On ::

Green Chem., 2024, 26,10824-10828
DOI: 10.1039/D4GC03982C, Communication
Dingyi Yang, Qi Zeng, Kaiwen Tan, Haoyue Hou, Xingyuan Fang, Chenlong Guo, Hao Yuan, Tao Meng
We prepared lipase-entrapped TiO2 colloidosomes with excellent recyclability for light-responsive Pickering interfacial biocatalysis, providing a green, recyclable and efficient Pickering interfacial biocatalysis platform.
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Electroreductive deoxygenative carboxylation of alkyl oxalates with CO2

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Green Chem., 2024, 26,10811-10817
DOI: 10.1039/D4GC03452J, Communication
Yong Yuan, Hangfei Jiang, Ya-Nan Zhang, Yuyan Tao, Xincong Liu, Congde Huo
An electroreductive deoxygenative carboxylation of alkyl oxalates with CO2 is demonstrated.
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Electrochemistry-enabled Rh-catalyzed regioselective [4 + 1] and [4 + 2] cycloaddition of benzoic acid with alkynyl esters/amides

By pubs.rsc.org
Published On ::

Green Chem., 2024, 26,10996-11002
DOI: 10.1039/D4GC03753G, Paper
Wei-Jung Chiu, Chung-Ming Sun
The reaction of benzoic acids with alkynyl esters/amides in the presence of a Rh-catalyst and AcOH as an additive to give phthalides by [4 + 1] annulation. In contrast, the additive NaOAc exclusively affords isocoumarins through the [4 + 2] pathway.
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Does enzymatic catalysis lead to more sustainable chemicals production? A life cycle sustainability assessment of isopropyl palmitate

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Green Chem., 2024, Advance Article
DOI: 10.1039/D4GC04514A, Paper
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Pieter Nachtergaele, Ozan Kocak, Yblin Roman Escobar, Jordy Motte, Dries Gabriels, Leopold Mottet, Jo Dewulf
A methodology is presented for assessing the life cycle sustainability of enzymatic catalysis for chemicals production. For IPP, lower environmental impacts, but higher costs and social risks were found for switching to enzymatic catalysis.
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Modular access to multi-substituted allenones via environmentally friendly organocatalytic C–H allenylation of aldehydes

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Green Chem., 2024, Advance Article
DOI: 10.1039/D4GC04550E, Paper
Xinying Hu, Ayisenbati Jialingbieke, Yuzhi Ren, Yifan Yang, Donghui Wei, Jian Gao, Ding Du
Organocatalytic direct C–H allenylation of aldehydes with propargyl bromides has provided a straightforward and step-economical strategy for allenone modular synthesis.
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Advancing green chemistry in environmental monitoring: the role of electropolymerized molecularly imprinted polymer-based electrochemical sensors

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Green Chem., 2024, Advance Article
DOI: 10.1039/D4GC03250K, Tutorial Review
Christopher Mwanza, Wei-Zhi Zhang, Kalulu Mulenga, Shou-Nian Ding
Molecularly imprinted polymers (MIPs) are synthetic materials designed to mimic the natural “lock and key” mechanism observed in biomolecular systems, such as the interactions between antibodies and antigens.
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The Effects of Polyolefin Structure and Source on Pyrolysis-Derived Plastic Oil Composition

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Green Chem., 2024, Accepted Manuscript
DOI: 10.1039/D4GC04029E, Paper
Jiayang Wu, Zhen Jiang, Victor S Cecon, Greg W. Curtzwiler, George W. Huber, Keith L. Vorst, Manos Mavrikakis
Seven types of plastics were pyrolyzed in a fluidized bed reactor: post-consumer recycled (PCR) high-density polyethylene (HDPE), PCR polypropylene (PP), virgin resins of varying molecular weights of HDPE, virgin resins...
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Continuous-flow Synthesis of Cyclic Carbonates with Polymer-supported Imidazolium-based Ionic Liquid (Im-PSIL) Catalysts

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Published On ::

Green Chem., 2024, Accepted Manuscript
DOI: 10.1039/D4GC04499A, Communication
Open Access
Zhibo Yu, Haruro Ishitani, Shu Kobayashi
Carbon dioxide (CO2), a major greenhouse gas emitted through human activities, represents a valuable carbon source for chemical production. However, maximizing its efficiency requires novel methods for CO2 conversion that...
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Catalytic hydrodeoxygenation and C–C coupling of lignin and its derivatives into renewable jet-fuel-range cycloalkanes

By pubs.rsc.org
Published On ::

Green Chem., 2024, Advance Article
DOI: 10.1039/D4GC02051K, Critical Review
Xinyong Diao, Ying Xiong, Yawen Shi, Longlong Ma, Chenglong Dong, Shengbo Zhang, Na Ji
This review provides an in-depth understanding of the synthesis pathways and corresponding catalytic systems for the production of jet-fuel-range cycloalkanes from lignin and its derivatives via catalytic hydrodeoxygenation and C–C coupling.
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Engineering high-valence nickel sites in Ni3S2/Ni3Se2 architectures enabling urea-assisted hydrogen evolution reactions

By pubs.rsc.org
Published On ::

Green Chem., 2024, Advance Article
DOI: 10.1039/D4GC04318A, Paper
Taotao Ai, Miaomiao Bai, Weiwei Bao, Jie Han, Xueling Wei, Xiangyu Zou, Jungang Hou, Lizhai Zhang, Zhifeng Deng, Yuxin Zhang
Bifunctional Ni3S2@Ni3Se2 electrocatalysts were constructed for urea-assisted hydrogen evolution. In the HER/UOR two-electrode system, the heterogeneous interface modulates the electronic structure and thus improves the catalytic performance.
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Engineering in situ: N-doped porous carbon-confined FeF3 for efficient lithium storage

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Published On ::

Green Chem., 2024, Advance Article
DOI: 10.1039/D4GC04097J, Paper
Open Access
Jinlong Hu, Weijun Xu, Lingzhi Zhang
Achieving N-doped porous carbon-confined FeF3 with enhanced lithium storage performance via an innovative in situ engineering approach.
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Hypervalent iodine chemistry with a mechanochemical twist

By pubs.rsc.org
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Green Chem., 2024, Advance Article
DOI: 10.1039/D4GC04903A, Communication
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Sayad Doobary, Miguel M. de Vries Ibáñez, Berit Olofsson
An assessment of mechanochemistry's utility with hypervalent iodine reagents highlighted its effectiveness, which showed better selectivity, reaction times and differing reactivity.
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Photo-Induced FeCl3-catalysed direct denitrative chlorination of (hetero)nitroarenes at room temperature

By pubs.rsc.org
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Green Chem., 2024, Accepted Manuscript
DOI: 10.1039/D4GC04210G, Communication
Mingjing Deng, Ke Liu, Zhaolun Ma, Guanzhong Luo, Longyang Dian
We present herein an iron-catalyzed denitrative chlorination of (hetero)nitroarenes at room temperature under visible light irradiation. In this study, FeCl3 catalyzed direct chlorination was achieved through denitrative chlorination under light...
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Photo-driven reduction/cyclization of nitroarenes via electron donor–acceptor complexes: a novel method for the acquisition of N-heterocycles

By pubs.rsc.org
Published On ::

Green Chem., 2024, Advance Article
DOI: 10.1039/D4GC04082A, Communication
Bin Sun, Chun Lv, Xiaohui Zhuang, Yan Xu, Haijing Song, Jiayin Wang, Zhaokang Zhang, Jiayang Wang, Can Jin
An EDA complex-based method for the reduction/cyclization of nitroarenes to obtain N-heterocycles with H2O as a clean by-product is presented.
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High Efficiency Leaching of Valuable Metals from Waste Lithium-ion ternary Batteries under Mild Conditions Using Green Deep Eutectic Solvents

By pubs.rsc.org
Published On ::

Green Chem., 2024, Accepted Manuscript
DOI: 10.1039/D4GC04373A, Paper
Bo Li, Zhengfu Zhang, Chengping Li, Jinsong Wang, Rundong Wan, Jiangzhao Chen, Ying Liu, Yuejing Bin, xiaoping yang, Chongjun Bao, Shaohua Ju
Recently, the production and demand for lithium-ion batteries (LIBs) has increased owing to increasing number of electric vehicles and products. This surge has considerably increased spent LIBs, leading to environmental...
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Catalytic synthesis of renewable lubricant base oils with methyl oleate and aromatics

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Published On ::

Green Chem., 2024, 26,11249-11258
DOI: 10.1039/D4GC03448A, Paper
Binbin Zhou, Nan Wang, Sibao Liu, Guozhu Liu
Aromatic-ester and cyclo-branched alkane renewable lubricant base oils were produced from methyl oleate and biomass-derived aromatics by alkylation and alkylation followed by hydrodeoxygenation (HDO).
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Shell biorefineries: mixed biofuel production from chitin

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Green Chem., 2024, 26,11280-11289
DOI: 10.1039/D4GC03761H, Paper
Hao Huang, Guangping Zhou, Xiaolan Cai, Min Zhuang, Shaoqu Xie
Bioenergy is a key strategy for sustainability, yet the potential for biofuel production from chitin is under-exploited.
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Selective electrosynthesis of aldehydes at industrially relevant current densities via tandem electrochemical–chemical catalysis

By pubs.rsc.org
Published On ::

Green Chem., 2024, 26,11290-11302
DOI: 10.1039/D4GC04536J, Paper
Ting Lin, Menglu Cai, Huijie Chen, Yiming Mo
A closed-loop tandem electrochemical–chemical catalysis system for aldehyde synthesis was developed, demonstrating a viable approach for the electrosynthesis of valuable intermediates under practical current densities with minimal waste electrolyte.
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Chemodivergent alkylation of trifluoromethyl alkenes via photocatalytic coupling with alkanes

By pubs.rsc.org
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Green Chem., 2024, 26,11196-11205
DOI: 10.1039/D4GC04176C, Paper
Open Access
Pol Martínez-Balart, Álvaro Velasco-Rubio, Sergio Barbeira-Arán, Hugo Jiménez-Cristóbal, Martín Fañanás-Mastral
A photocatalytic methodology for the chemodivergent direct cross-coupling of simple alkanes with trifluoromethyl alkenes that enables the selective formation of gem-difluoroalkenes and trifluoromethyl alkanes is presented.
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Production of nanochitins via a shell biorefinery process for self-assembly applications as photonic films and Pickering emulsions

By pubs.rsc.org
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Green Chem., 2024, 26,11222-11237
DOI: 10.1039/D4GC02680B, Paper
Open Access
Xuhai Zhu, Fuyan Peng, Hui Li, Rongjun Lin, Rui Lu, Fang Lu
A simple, environmentally friendly, and flexible shell biorefinery process for integrated utilization of all NCh products in high-value applications, such as photonic films and Pickering emulsions.
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Thermodynamically stable synthesis of high entropy alloys and efficiently catalyzed oxidation of 5-hydroxymethylfurfural into 2,5-furandicarboxylic acid under base-free conditions

By pubs.rsc.org
Published On ::

Green Chem., 2024, 26,11316-11327
DOI: 10.1039/D4GC04186K, Paper
Guangqiang Lv, Shan Liu, Xiaoyan Chen, Mengxin Chen, Yanjuan Wu, Yuji Gao, Shuai Wang, Furong Tao, Jingui Wang, Liwei Niu
In a completely non-alkaline aqueous system, a high-entropy alloy catalyst composed of FeCoNiCuGaPt activates O2 and H2O molecules to form hydroxyl radicals (˙OH) and efficiently oxidizes 5-hydroxymethylfurfural into 2,5-furandicarboxylic acid.
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Converting waste PET into dimethyl terephthalate and diverse boronic esters under metal-free conditions

By pubs.rsc.org
Published On ::

Green Chem., 2024, 26,11132-11139
DOI: 10.1039/D4GC03358B, Communication
Minghao Zhang, Yunkai Yu, Zhuo Wang, Shaoyu Zhang, Xiong Gao, Jiaming Liu, Jing Li, Weixiang Wu, Qingqing Mei
An ionic liquid-catalyzed metal-free approach was proposed to upcycle waste PET into dimethyl terephthalate and boronic esters, facilitated by multiple hydrogen bonds.
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A green and sustainable multi-enzyme cascade for the biosynthesis of 1,3-propanediamine from crude glycerol in vitro

By pubs.rsc.org
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Green Chem., 2024, Advance Article
DOI: 10.1039/D4GC03777D, Paper
Daocheng Liao, Shiming Tang, Ying Lin, Suiping Zheng
This paper designs a novel multi-enzyme cascade reaction capable of efficiently synthesizing 1,3-propanediamine from glycerol in vitro.
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Reusable Co-catalysts for general and selective α-alkylation of nitriles with alcohols

By pubs.rsc.org
Published On ::

Green Chem., 2024, 26,11140-11146
DOI: 10.1039/D3GC04436J, Communication
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Zhuang Ma, Zechen Wu, Carsten Kreyenschulte, Stephan Bartling, Henrik Lund, Matthias Beller, Rajenahally V. Jagadeesh
A general cobalt-catalyzed α-alkylation of nitriles with alcohols is reported.
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Development of a highly efficient electrocatalytic hydrogenation and dehalogenation system using a flow cell with a Pd tube cathode

By pubs.rsc.org
Published On ::

Green Chem., 2024, 26,11328-11333
DOI: 10.1039/D4GC04617J, Paper
Hiroaki Tajima, Hideki Ishii, Shinsuke Inagi, Toshio Fuchigami
A novel flow and circulation electrolytic system has been developed for the highly efficient cathodic hydrogenation of unsaturated compounds and dehalogenation of various aromatic halides.
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Economic and environmental sustainability of bio-based HMF production and recovery from lignocellulosic biomass

By pubs.rsc.org
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Green Chem., 2024, 26,11340-11350
DOI: 10.1039/D4GC04270K, Paper
Yuyao Jia, Shraddha Maitra, Lavanya Kudli, Jeremy S. Guest, Vijay Singh
Transforming waste stream of biorefinery into high-value bioproducts.
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Review of carbon-based catalysts for electrochemical nitrate reduction and green ammonia synthesis

By pubs.rsc.org
Published On ::

Green Chem., 2024, Advance Article
DOI: 10.1039/D4GC04640D, Tutorial Review
Guanting Liao, Richard L. Smith Jr., Haixin Guo, Xinhua Qi
This work aims to review the latest developments in carbon-based electrocatalysts applied in electrocatalytic nitrate reduction, including pure carbon materials, heteroatom doping or metal-bonding catalysts, and carbon substrate-supported composites.
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Utilize rather than create: transforming phthalonitrile resin into N-rich hierarchical porous carbon for supercapacitor materials

By pubs.rsc.org
Published On ::

Green Chem., 2024, Advance Article
DOI: 10.1039/D4GC04103H, Paper
Yi Li, Qiancheng Liu, Qian Zhang, Xiaoxiao Li, Yang Yang, Pan Wang, Kui Li, Ying Li, Fei Zhong, Qi Liu, Yun Zheng, Xulin Yang, Peng Zhao
The “utilize rather than create” strategy employs the reaction product (RPH) as the precursor and the by-product (KCl) as the template for the synthesis of N-rich hierarchical porous carbon for high performance supercapacitor materials.
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CdS/Mg–Fe layered double hydroxide: a versatile heterogeneous photocatalyst for the acylation of indoles with α-keto acids

By pubs.rsc.org
Published On ::

Green Chem., 2024, Advance Article
DOI: 10.1039/D4GC05239K, Paper
Jun-Bo Wang, Tong Yue, Ling Xu, Zhi-Qiang Hao, Zhan-Hui Zhang
The composite CdS/Mg–Fe layered double hydroxide was constructed and confirmed as an efficient recyclable heterogeneous photocatalyst for C-3 acylation of indoles with α-keto acids under light irradiation at room temperature.
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Ball milling-promoting difunctionalization of alkynyl sulfonium salts with sulfinic acids towards (Z)-1,2-disulfonylethenes

By pubs.rsc.org
Published On ::

Green Chem., 2024, Advance Article
DOI: 10.1039/D4GC04895D, Paper
Li-Hua Yang, Bei Li, Lin Chen, Wen-Shi Yao, Han-Yue Peng, Sha Peng, Long-Yong Xie
A simple ball milling-mediated disulfonylation of alkynyl sulfonium salts with sulfinic acids for the stereoselective synthesis of various (Z)-1,2-disulfonylethenes has been developed under catalyst-, additive- and solvent-free conditions.
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1D/3D hierarchical carbon skeleton confined NiFe nanoparticles with optimized three-phase interfaces as tri-functional electrocatalysts

By pubs.rsc.org
Published On ::

Green Chem., 2024, Advance Article
DOI: 10.1039/D4GC04466E, Paper
Yuqing Chen, Binyang Liu, Xuesong Liu, Jiahui Ye, Kuan Deng, Chengjie Wu, Qiang Niu, Tao Yang, Wen Tian, Junyi Ji
Multilevel 1D/3D CNTs/carbon spheres with hydrophilicity can promote the infiltration of an electrolyte into the interior and guide bubble diffusion, thus constructing an optimal gas–solid–liquid interface to enhance the electrocatalytic process.
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CO2 switchable solvents for sustainable dissolution, modification, and processing of cellulose materials: a critical review

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Published On ::

Green Chem., 2024, Advance Article
DOI: 10.1039/D4GC04032E, Critical Review
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Peter McNeice, Ben L. Feringa
CO2 switchable solvents provide a convenient and environmental method to dissolve and process cellulose.
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Hitman: Songs you must listen to this week

By www.thehindu.com
Published On :: Sat, 09 Apr 2016 19:47:15 +0530


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Hitman: Songs you must listen to this week

By www.thehindu.com
Published On :: Sat, 07 May 2016 17:34:00 +0530


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Hitman: Songs you must listen to this week

By www.thehindu.com
Published On :: Sat, 14 May 2016 17:20:45 +0530


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Hitman: Songs you must listen to this week

By www.thehindu.com
Published On :: Sat, 18 Jun 2016 18:56:05 +0530


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The Brexit conundrum

By www.thehindu.com
Published On :: Sat, 25 Jun 2016 15:42:39 +0530

Now that the U.K. has voted to leave the EU, how will British cinema be affected?


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Hitman: Songs you must listen to this week

By www.thehindu.com
Published On :: Sat, 25 Jun 2016 20:36:46 +0530


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Hitman

By www.thehindu.com
Published On :: Sat, 02 Jul 2016 18:00:20 +0530

Songs you must listen to this week


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Where are the hits?

By www.thehindu.com
Published On :: Sat, 09 Jul 2016 15:01:45 +0530

A half-yearly report on Kollywood’s run at the box office


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Hitman: Songs you must listen to this week

By www.thehindu.com
Published On :: Sat, 30 Jul 2016 19:19:14 +0530


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Avan Pithana? (1966)

By www.thehindu.com
Published On :: Sat, 13 Aug 2016 15:37:00 +0530

S. S. Rajendran, C. R. Vijayakumari, S. V. Sahasranamam, T. P. Muthulakshmi, C. K. Nagesh, A. Karunanidhi, Kumari Sachu


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