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Exploring catecholase activity in dinuclear Mn(II) and Cu(II) complexes: an experimental and theoretical approach

New J. Chem., 2020, Advance Article
DOI: 10.1039/D0NJ00605J, Paper
M. Shahwaz Ahmad, Mohd Khalid, M. Shahnawaz Khan, M. Shahid, Musheer Ahmad, Monika, Azaj Ansari, Mo Ashafaq
Two dinuclear Mn(II) and Cu(II) complexes were prepared, characterised and assessed for non-covalent interactions and catecholase oxidase properties. The catecholase activity of 2 is further corroborated by theoretical calculations using DFT.
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Detection of 3,4-diaminotoluene based on Sr0.3Pb0.7TiO3/CoFe2O4 core/shell nanocomposite via an electrochemical approach

New J. Chem., 2020, Advance Article
DOI: 10.1039/D0NJ01074J, Paper
Ali B. Abou Hammad, Amir Elzwawy, A. M. Mansour, M. M. Alam, Abdullah M. Asiri, Mohammad Razaul Karim, Mohammed M. Rahman, Amany M. El Nahrawy
We reported a scalable sol–gel method for the preparation of Sr0.3Pb0.7TiO3/CoFe2O4 core–shell magnetic nanocomposite with a finely controlled shell and evaluated its efficiency as an electrochemical sensor for the selective detection of 3,4-diaminotoluene.
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Production of furfural from xylose catalyzed by a novel calcium gluconate derived carbon solid acid in 1,4-dioxane

New J. Chem., 2020, Advance Article
DOI: 10.1039/D0NJ00619J, Paper
Tao Yang, Wenzhi Li, Mingxue Su, Yang Liu, Minghou Liu
A novel carbon-based solid acid catalyst (SC-GCa-800) was prepared by the high-temperature carbonization of calcium gluconate followed by sulfonation with 4-diazoniobenzenesulfonate at room temperature.
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Physicochemical properties of a urea/zinc chloride eutectic mixture and its improved effect on the fast and high yield synthesis of indeno[2,1-c]quinolines

New J. Chem., 2020, Advance Article
DOI: 10.1039/D0NJ01342K, Paper
Diana Peña-Solórzano, Vladimir V. Kouznetsov, Cristian Ochoa-Puentes
An environmentally friendly and efficient method for the synthesis of indeno[2,1-c]quinolines is developed using a urea/zinc chloride eutectic mixture as a green mildly acidic medium.
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NMR probe effects on trans-philicity and trans-influence ladders in square planar Pt(II) complexes

New J. Chem., 2020, Advance Article
DOI: 10.1039/D0NJ01336F, Paper
Athanassios C. Tsipis
trans-Philicity ladders for trans-Pt(PMe3)2(X)L (X = H, CH3, CO, NH2, OH2, Cl) complexes are built by σiso X NMR descriptors. Correlations of the σiso X vs popular electronic/structural parameters of L and X demonstrate the origin of trans philicity.
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Photoelectrocatalytic properties and mechanism of rhodamine B degradation using a graphene oxide/Ag3PO4/Ni film electrode

New J. Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0NJ00864H, Paper
Di Zhao, Fu-Cai Dai, Ai-Chang Li, Yu Chen, Gui-Hua Li, Qian Wang, Wen-Shuo Hou, Hong-Zhi Zhou
Graphene oxide (GO)/Ag3PO4/Ni composite film electrodes were prepared by composite electrodeposition using a mixture of ammonium phosphate and GO aqueous suspension as the electrolyte. The morphology, crystallinity, and optical characteristics...
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Preparation of MOFs Catalysts Simultaneously Modulated Metal Nodes and Ligands Via One-Pot Method for Optimizing Cycloaddition Reactions

New J. Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0NJ01086C, Letter
Peng Wang, Sha Wang, Wenlei Zhang, Xiaohan Li, Zhida Gu, Wenze Li, Shuang Zhao, Yu Fu
MOFs catalysts are farbricated in one-pot method by simultaneously adjusting metal nodes and ligands. Pore environments, Lewis acids (LAs) and Brønsted acids (BAs) are controlled when using BAs groups to...
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Effect of number and different types of proton donors on excited-state intramolecular single and double proton transfer in bipyridine derivatives: theoretical insights

New J. Chem., 2020, Advance Article
DOI: 10.1039/D0NJ01304H, Paper
Komsun Chaihan, Nawee Kungwan
Intra-HBs are strengthened upon photoexcitation, confirmed by red-shift in vibrational mode and topology analysis. Number and type of donors result in difference in photophysical properties. Occurrence of ESIPT depends on barrier and reaction energy.
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Fabrication of a 3D self-supporting Ni–P/Ni2P/CC composite and its robust hydrogen evolution reaction properties in alkaline solution

New J. Chem., 2020, Advance Article
DOI: 10.1039/D0NJ00727G, Paper
Fan Yang, Shuqin Yang, Qianqian Niu, Siyue Huo, Zimo Song, Laizhou Song
The Ni–P/Ni2P/CC composite exhibits excellent alkaline HER properties derived from Ni–P filling the sites on the CC not occupied by Ni2P nanosheets.
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The effect of vicinal di-halo substituents on the organogelling properties of aromatic supramolecular gelators and their application as soft templates

New J. Chem., 2020, Advance Article
DOI: 10.1039/D0NJ01440K, Paper
Andrea S. Mac Cormack, Verónica M. Busch, M. Laura Japas, Lisandro Giovanetti, Florencia Di Salvo, Pablo H. Di Chenna
Vicinal di-halo substituents have a determinant effect on the supramolecular self-assembly and properties of aromatic physical gelators with application as soft templates.
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Synthesis of characteristic polyisoprenes using rationally designed iminopyridyl metal (Fe and Co) precatalysts: investigation of co-catalysts and steric influence on their catalytic activity

New J. Chem., 2020, Advance Article
DOI: 10.1039/D0NJ00942C, Paper
Wenhua Lin, Liping Zhang, Hongyi Suo, Arumugam Vignesh, Nighat Yousuf, Xiang Hao, Wen-Hua Sun
A series of iminopyridyl ligand-based iron and cobalt complexes are utilized as catalysts in isoprene polymerization, in which the microstructure of resultant polyisoprenes was investigated.
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Water-soluble poly(N-isopropylacrylamide) nanoparticles grafted to trivalent lanthanide complexes as highly sensitive ratiometric nanothermometers

New J. Chem., 2020, Advance Article
DOI: 10.1039/D0NJ01263G, Paper
Josiane Aparecida Sobrinho, Gilmar Araújo Brito Júnior, Italo Odone Mazali, Fernando Aparecido Sigoli
A new water-soluble, luminescent ratiometric nanothermometer with a tunable temperature-responsive range, high thermal sensitivity and good repeatability was designed and synthesized by grafting lanthanide complexes to pNIPAM polymeric nanoparticles.
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Proton conduction in two Cu/Zn dimer-based hydrogen-bonded supramolecular frameworks from imidazole multi-carboxylate

New J. Chem., 2020, Advance Article
DOI: 10.1039/D0NJ01189D, Paper
Qingxu Wang, Zhejun Ye, Guoqing Shi, Kaimeng Guo, Gang Li
At 98% RH and 100 °C, two dimer-based HSFs show the best σ values of 3.13 × 10−4 S cm−1 for 1 and 0.55 × 10−4 S cm−1 for 2, which can be compared to the values of reported HSFs.
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Oligoaniline-functionalized polysiloxane/Prussian blue composite towards bifunctional electrochromic supercapacitors

New J. Chem., 2020, Advance Article
DOI: 10.1039/D0NJ00736F, Paper
Yanyan Wang, Xiaoteng Jia, Meihua Zhu, Xincai Liu, Danming Chao
We report the preparation of a novel oligoaniline-functionalized polysiloxane/Prussian blue composite, which exhibits improved electrochromic properties and approving supercapacitor performance featuring charge storage indicating functionalization.
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Effect of the graphene sheets incorporation on physicochemical properties of nano-alumina

New J. Chem., 2020, Accepted Manuscript
DOI: 10.1039/C9NJ06317J, Paper
Elena A. Trusova, Dmitry D Titov, Alex N Kirichenko, Michael Y Zorin
The colloidal processing method was suggested for obtaining of chemically homogeneous composite powder based on graphene and nano-alumina. The method allows integrating a hybrid structure by mixing components at nanoscale...
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Label-free colorimetric detection of serum cysteine using Ag-NPs probes for immanence of Be2+ ions

New J. Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0NJ00967A, Paper
Chandrababu Rejeeth, Alok Sharma, Varukattu Nipun babu, Rahul Gautam
Amino acids play a crucial role in a variety of significant metabolic processes and their homeostasis is essential for cell growth and survival. Cysteine (Cys) furnishes imperative information about peculiar...
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Recent progress and approaches on the synthesis of Mn-doped zinc oxide nanoparticles: A theoretical and experimental investigation on the photocatalytic performance

New J. Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0NJ01530J, Paper
Joyce Silva, Nivaldo Freire Andrade Neto, Marisa Carvalho Oliveira, Renan Pontes Ribeiro, S Lazaro, Yara Gomes, Carlos Paskocimas, Mauricio Bomio, Fabiana Motta
Transition metal-doped semiconductors are promising to conduct the future of environmental remediation from photocatalysis. In this study, the role of Mn-doping on the structural, electronic, morphological, optical, and photocatalytic properties...
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Ultrastable conductive microporous covalent triazine frameworks based on pyrene moieties provide high-performance CO2 uptake and supercapacitance

New J. Chem., 2020, Advance Article
DOI: 10.1039/D0NJ01292K, Paper
Mohamed Gamal Mohamed, Ahmed F. M. EL-Mahdy, Yasuno Takashi, Shiao-Wei Kuo
Two pyrene-functionalized CTFs through ionothermal treatment TCNPy in the presence of molten zinc chloride at 500 °C, which displayed high-performance CO2 uptake and supercapacitance.
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Single-pot template-free synthesis of a glycerol-derived C–Si–Zr mesoporous composite catalyst for fuel additive production

New J. Chem., 2020, Advance Article
DOI: 10.1039/D0NJ00523A, Paper
Saurabh Kumar, Nagabhatla Viswanadham, Sandeep K. Saxena, Arumugam Selvamani, Jitendra Diwakar, Ala’a H. Al-Muhtaseb
The C–Si–Zr material synthesized from bio-derived waste glycerol, ZrO(NO3)2 and TEOS exhibits excellent catalytic activity for tri-acetin production from low-value glycerol.
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Linear dicarboxylate based pyridyl appended cobalt(II) coordination polymers in search of opto-electronic properties

New J. Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0NJ00567C, Paper
Faruk Ahmed, Joydeep Datta, Samim Khan, Basudeb Dutta, Sakhiul Islam, Sanobar Naaz, Partha Pratim Ray, Mohammad Hedayetullah Mir
Two new coordination polymers (CPs) [Co(adc)(4-ppy)(H2O)2]n, (1) and [Co(adc)(4-bppy)(H2O)2]n, (2) (H2adc = acetylenedicarboxylic acid, 4-ppy = 4-phenylpyridine and 4-bppy = 4-(4-bromophenyl)pyridine) have been synthesized and characterized by various techniques including...
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Trifluoromethyl functionalized polyindoles: Electrosyntheses, characterization, and improved capacitive performance

New J. Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0NJ00812E, Paper
Rui Wang, Yu Xue, Fengxing Jiang, Weiqiang Zhou, Jingkun Xu, Xuemin Duan, Danhua Zhu, Liming Xu, Yue Cai, Aiqin Liang
Fluorination of conjugated polymers has been explored as a viable strategy for enhancing the overall performance of corresponding polymers. In this work, two trifluoromethylated polyindoles (5-PFMIn and 6-PFMIn) are synthesized...
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Oxidative cyclization of thiosemicarbazide: chemo-dosimetric approach for highly selective fluorescence detection of cerium(IV)

New J. Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0NJ01100B, Paper
Ahad Shaikh, Pallabi Mukherjee, Sabyasachi Ta, Arun Bhattacharyya, Abhijit Ghosh, Debasis Das
A simple thiosemicarbazide based chemodosimeter detects Ce4+ ion through turn-on fluorescence. The sensing mechanism is based on oxidative cyclyzation. The chemodosimeter shows exceptional selectivity for Ce4+ that allows to detect...
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Whole Genome Sequence Analysis and Homology Modelling of Main Protease and Non-Structural Protein 3 of the SARS-CoV-2 reveals an Aza-Peptide and a Lead Inhibitor with Possible Antiviral Properties

New J. Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0NJ00974A, Paper
Arun K Shankar, Divya Bhanu, Anjani Alluri, Samriddhi Gupta
The family of viruses belonging to Coronaviridae consist of virulent pathogens that have a zoonotic property, Severe Acute Respiratory Syndrome (SARS-CoV) and Middle East Respiratory Syndrome (MERS-CoV) of this family...
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A non-enzymatic electrochemical approach for L-Lactic acid sensor development based on CuO.MWCNT nanocomposites modified with a nafion matrix

New J. Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0NJ01715A, Paper
Mohammad M. Hussain, Abdullah M. Asiri, Mohammed M. Rahman
Copper oxide ornamented multi-walled carbon nanotube nanocomposites (CuO.MWCNT NCs) were prepared using an unsophisticated wet-chemical technique in basic medium. CuO.MWCNT NCs was examined by using various analytical techniques for example...
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Cu(II)Cl2 Containing Bispyridine-based Porous Organic Polymer Support Prepared via Alkyne-Azide Cycloaddition as a Heterogeneous Catalyst for Oxidation of Various Olefins

New J. Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0NJ01174F, Letter
Jong Ho Yoon, Hye Min Choi, Suk Joong Lee
New class of porous organic polymer (POP) based heterogeneous catalyst Cu-POP was prepared from immobilizing Cu(II)Cl2 into bpy containing POP prepared via alkyne-azide cycloaddition. This new catalyst showed efficient catalytic...
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A Concise Guide to Bible Prophecy

Stan Guthrie’s helpful survey.




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Get Prufrock

An indispensable literary newsletter.




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The Tallgrass Prairie Reader

Glimpses of a lost world.




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The Novel as Protestant Art

Previewing the March/April issue of Books & Culture.




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How I think about solving problems

Early on in my career as a software developer I thought my primary contribution was writing code. After all, software engineers are paid to ship software and writing code is a key component of that. It took several years for me to realize that there are numerous other contributions that go into shipping software (if...




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[ASAP] Pyrimidine Analogues as a New Class of Gram-Positive Antibiotics, Mainly Targeting Thymineless-Death Related Proteins

ACS Infectious Diseases
DOI: 10.1021/acsinfecdis.9b00305




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[ASAP] Potentiation of Antibiotics against Gram-Negative Bacteria by Polymyxin B Analogue SPR741 from Unique Perturbation of the Outer Membrane

ACS Infectious Diseases
DOI: 10.1021/acsinfecdis.9b00159




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[ASAP] Multitarget Approaches against Multiresistant Superbugs

ACS Infectious Diseases
DOI: 10.1021/acsinfecdis.0c00001




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[ASAP] Target-Based Design of Promysalin Analogues Identifies a New Putative Binding Cleft in Succinate Dehydrogenase

ACS Infectious Diseases
DOI: 10.1021/acsinfecdis.0c00024




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[ASAP] <italic toggle="yes">Plasmodium falciparum</italic> Artemisinin Resistance: The Effect of Heme, Protein Damage, and Parasite Cell Stress Response

ACS Infectious Diseases
DOI: 10.1021/acsinfecdis.9b00527




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Freedom of the Press . . . To Lampoon!

It has been said that “politics is a blood sport.” Even so, American politicians are expected to have some sense of humor, to be able to take a joke at their expense—at least under well understood terms of engagement. In New York City, those terms have included the annual political roast written, produced and performed...

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Treasure Trove: Our Oldest Printed Book

While the collections of the New-York Historical Society’s Patricia D. Klingenstein Library contain many oddities acquired over a long period of time, none is, at first blush, stranger than our oldest printed book: a copy of the Moralia of Pope Gregory the Great, printed in Basel in 1496. Why strange? Because in collections shaped largely...

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Spreading the News of Yellow Fever

Every year when the seasons change from cold to warm, I get sick. Usually it’s allergies or a cold, but like clockwork I am out of commission for a few days. I suspect this has happened to people since time began, but if you lived on Manhattan Island during the 1790s, and even as late...

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Rare Books Revealed: Text Corrections in Printed Books

While working on the Patricia D. Klingenstein Library’s hidden collections cataloging project, I’ve found some examples of the different methods authors and printers used to fix small errors in a text after an item was printed. Shown below are a few examples of the corrections that were made directly to the page. In the first...

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Copying History: A Handmade Facsimile of a Rare Franklin Imprint

In 1725, a then unknown nineteen-year-old journeyman printer named Benjamin Franklin printed A Dissertation on Liberty and Necessity, Pleasure and Pain, responding to William Wollaston’s The Religion of Nature Delineated. Later, having second thoughts about the soundness of his argument, Franklin destroyed most of the remaining copies of what was already a small run. Fortunately, his distribution of...

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“The Good Lord protected me”: A soldier’s letter on the Meuse-Argonne Offensive

This Sunday will be the 100th anniversary of the armistice that ended World War I, a war that remains etched in the collective memory for the physical and psychological toll wrought on those who lived through it. With that in mind, it seems fitting to mark this occasion through the words of a soldier who...

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Camp Sagan: The Forgotten Prisoners of World War I

The fact that Russian World War I soldiers remained prisoners of war well after the November 1918 Armistice is one of the more obscure aspects of the war’s history. But with civil war raging in Russia, concerns arose over repatriating soldiers that might return to reinforce the Bolsheviks. This meant large number of Russian soldiers remained in...

The post Camp Sagan: The Forgotten Prisoners of World War I appeared first on New-York Historical Society.




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Tinker, Tailor, Printer, Spy: Pierrette Jeanne Sophie Charpentier de Mailly

An unassuming French pamphlet sits on the shelves at the New-York Historical Society. However, there is far more than meets the eye beneath its aged, brown wrappers. Premier rapport fait au nom du Comité de salut public, sur les moyens d’extirper la mendicité dans les campagnes, & sur les secours que doit accorder la République...

The post Tinker, Tailor, Printer, Spy: Pierrette Jeanne Sophie Charpentier de Mailly appeared first on New-York Historical Society.




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Now on View–“Padlocked”: New York’s Prohibition Years

Set to commence on January 17, 1920, the great social experiment of Prohibition had already begun with a “dry run” for Americans adapting to the restriction of alcohol inspired by World War I. That was followed by a full year anticipating the event through the process of Constitutional amendment and the passage of enforcement legislation...

The post Now on View–“Padlocked”: New York’s Prohibition Years appeared first on New-York Historical Society.




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Puppies Preserved!

August 26th is National Dog Day! What better way to celebrate than by sharing a unique,  dog-centric artifact from our library.   This daguerreotype of an unidentified dog (PR-012-2-263)  has the formality of a portrait. The animal’s pose and eye contact with the camera (and us as viewers) personifies it. One of our ongoing preservation projects includes rehousing...

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Gustavus Conyngham: American Privateer

On July 3, 1776, the Continental Congress authorized privateering on the high seas. Essentially, any private citizen who obtained a Commission of Marque and Reprisal would be permitted to capture British ships. A common warfare tactic since the Middle Ages, the intent of the act was to weaken the enemy at sea while trading confiscated...

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“A Correct and Perfect Recollection”: David Grim’s Map of Prerevolutionary Manhattan

Little is known about long-lived David Grim (1737-1826) outside of the brief personal account of his life held by the New-York Historical Society Library. What can be said is that his memory was sound. A tavern keeper, merchant, and owner of Hessian’s Coffee House from 1767 to 1789, Grim sought to leave behind more than an...

The post “A Correct and Perfect Recollection”: David Grim’s Map of Prerevolutionary Manhattan appeared first on New-York Historical Society.




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Lab Notes: Conserving a George B. Post Presentation Drawing

George B. Post (1837-1913), an American architect trained in the Beaux-Arts tradition, is perhaps best known for his New York City landmark buildings, including the New York Stock Exchange, City College, and the Brooklyn Historical Society. After working as a draftsman for Richard Morris Hunt, Post opened his first architectural firm in New York City...

The post Lab Notes: Conserving a George B. Post Presentation Drawing appeared first on New-York Historical Society.




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Insight into the Landscape of Professional Development in Head Start from FACES 2014

A new research brief illuminates the landscape of professional development in Head Start programs. Using data from the spring 2017 round of the FACES 2014 Survey, researchers explore professional development experiences of Head Start program directors, center directors, teachers, and other staff.




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Mathematica Experts Showcase MACBIS Expertise and Present on Medicaid Methods and Topics at Medicaid Enterprise Systems Conference

Mathematica experts will showcase their expertise in providing business analytics and data quality development for the Medicaid and CHIP (Children’s Health Insurance Program) Business Information Solution (MACBIS) at this year’s Medicaid Enterprise Systems Conference in Chicago.