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Synthesis of star-shaped polyzwitterions with adjustable UCST and fast responsiveness by a facile RAFT polymerization

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Polym. Chem., 2020, Advance Article
DOI: 10.1039/D0PY00318B, Paper
Zhi Li, Hao Li, Zhonghe Sun, Botao Hao, Tung-Chun Lee, Anchao Feng, Liqun Zhang, San H. Thang
We describe crosslinking of polyzwitterions for the formation of novel star-shaped polymers with low polydispersities and dual-responsiveness using RAFT polymerization.
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Highly elastic, strong, and reprocessable cross-linked polyolefin elastomers enabled by boronic ester bonds

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Polym. Chem., 2020, Advance Article
DOI: 10.1039/D0PY00235F, Paper
Fei Yang, Li Pan, Zhe Ma, Yahui Lou, Yuanyuan Li, Yuesheng Li
Despite the development of new catalysts and synthetic strategies to prepare polyolefin elastomers (POEs), less progress has been made in balancing their elastomeric properties with processability and resistance to heat and solvents.
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Poly(alanine-nylon-alanine) as a bioplastic: chemoenzymatic synthesis, thermal properties and biological degradation effects

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Polym. Chem., 2020, Advance Article
DOI: 10.1039/D0PY00137F, Paper
Open Access
Prashant G. Gudeangadi, Kei Uchida, Ayaka Tateishi, Kayo Terada, Hiroyasu Masunaga, Kousuke Tsuchiya, Hitoshi Miyakawa, Keiji Numata
Poly(amino acids) such as polypeptides and proteins are attractive biomass-based polymers that potentially contribute to circular economy for plastic.
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Self-crosslinking smart hydrogels through direct complexation between benzoxaborole derivatives and diols from hyaluronic acid

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Polym. Chem., 2020, Advance Article
DOI: 10.1039/D0PY00308E, Paper
Tamiris Figueiredo, Yu Ogawa, Jing Jing, Vanina Cosenza, Isabelle Jeacomine, Johan D. M. Olsson, Thibaud Gerfaud, Jean-Guy Boiteau, Craig Harris, Rachel Auzély-Velty
By tailoring the structure of benzoxaborole (BOR), self-crosslinking hydrogels based on hyaluronic acid (HA) modified with BOR derivatives are obtained for the first time through the direct BOR-HA diol complexation at physiological pH.
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Synthesis of acrylamide-based block-copolymer brushes under flow: monitoring real-time growth and surface restructuring upon drying

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Polym. Chem., 2020, Advance Article
DOI: 10.1039/D0PY00219D, Paper
Open Access
Joydeb Mandal, Andrea Arcifa, Nicholas D. Spencer
Block-copolymer brushes of water-soluble acrylamides have been synthesised by SI-ATRP under continuous flow and their growth monitored in situ by means of a quartz-crystal microbalance with dissipation (QCM-D).
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Preparation of aryl polysulfonates via a highly efficient SuFEx click reaction, their controllable degradation and functionalized behavior

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Polym. Chem., 2020, Advance Article
DOI: 10.1039/D0PY00435A, Communication
Zhenlei Cao, Feng Zhou, Pei-Yang Gu, Dongyun Chen, Jinghui He, John R. Cappiello, Peng Wu, Qingfeng Xu, Jianmei Lu
Polysulfonates obtained from SuFEx click reaction can be degraded using DBU. The degradation process was further utilized to prepare functional polymers.
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Pillar[5]arene-based self-assembled linear supramolecular polymer driven by guest halogen–halogen interactions in solid and solution states

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Polym. Chem., 2020, Advance Article
DOI: 10.1039/D0PY00327A, Paper
Talal F. Al-Azemi, Mickey Vinodh
A pillar[5]arene-based linear supramolecular polymer mediated by guest halogen–halogen interactions (C–Br⋯Br–C) was studied in both the solution and solid states.
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Hydrogen-bonded supramolecular micelle-mediated drug delivery enhances the efficacy and safety of cancer chemotherapy

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Polym. Chem., 2020, 11,2791-2798
DOI: 10.1039/D0PY00082E, Paper
Chih-Chia Cheng, Ya-Ting Sun, Ai-Wei Lee, Shan-You Huang, Wen-Lu Fan, Yu-Hsuan Chiao, Chih-Wei Chiu, Juin-Yih Lai
Multiple hydrogen-bonded supramolecular polymers tend to form stable spherical micelles with oppositely charged anticancer drugs in biological environments, which improves cellular drug uptake and more effectively induces apoptosis in cancer cells.
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Polymerization of dopamine accompanying its coupling to induce self-assembly of block copolymer and application in drug delivery

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Polym. Chem., 2020, 11,2811-2821
DOI: 10.1039/D0PY00085J, Paper
Yudian Qiu, Zongyuan Zhu, Yalei Miao, Panke Zhang, Xu Jia, Zhongyi Liu, Xubo Zhao
The polymerization of dopamine and its coupling occur in succession, which synergistically induces the self-assembly of block copolymer to yield ordered structures, including micelles and vesicles.
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Simple improvements to Gilch synthesis and molecular weight modulation of MEH-PPV

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Polym. Chem., 2020, 11,2831-2837
DOI: 10.1039/D0PY00072H, Paper
Riley O'shea, Wallace W. H. Wong
The solvent and temperature used in the Gilch synthesis of poly[2-methoxy-5-(2-ethylhexyloxy)-1,4-phenylenevinylene] (MEH-PPV) were varied to achieve an improved set of reaction conditions.
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Vesicular assemblies of thermoresponsive amphiphilic polypeptide copolymers for guest encapsulation and release

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Polym. Chem., 2020, 11,2889-2903
DOI: 10.1039/D0PY00135J, Paper
Mahammad Anas, Somdeb Jana, Tarun K. Mandal
Thermoresponsive amphiphilic polypeptide copolymers are synthesized via different polymerization techniques for their self-assembly into vesicular aggregates for guest encapsulation and release.
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Self-supported rhodium catalysts based on a microporous metal–organic framework for polymerization of phenylacetylene and its derivatives

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Polym. Chem., 2020, 11,2904-2913
DOI: 10.1039/D0PY00170H, Paper
Li Zhang, Qingbin Cao, Fei Gao, Yuping Dong, Xiaofang Li
Highly efficient, cis-selective, stable, recyclable and reusable heterogeneous single-site MOF-supported rhodium catalysts polymerize PA and its derivatives, producing cis-transoidal PPAs and their functional derivatives having a helical configuration or AIE properties.
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Synthesis of biscarboxylic acid functionalised EDTA mimicking polymers and their ability to form Zr(IV) chelation mediated nanostructures

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Polym. Chem., 2020, 11,2799-2810
DOI: 10.1039/D0PY00304B, Paper
Meike N. Leiske, Julia A. Walker, Aadarash Zia, Nicholas L. Fletcher, Kristofer J. Thurecht, Thomas P. Davis, Kristian Kempe
We present a new biscarboxylic acid acrylate, which is used for the synthesis of double hydrophilic EDTA-mimicking block copolymers capable of self-assembly upon zirconium complexation.
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A high performance phenyl-free LED photoinitiator for cationic or hybrid photopolymerization and its application in LED cationic 3D printing

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Polym. Chem., 2020, 11,2855-2863
DOI: 10.1039/D0PY00142B, Paper
Liqun Tang, Jun Nie, Xiaoqun Zhu
In this work, a high performance LED photoinitiator, 1,3-bis(1-methyl-1H-pyrrol-2-yl)prop-2-en-1-one (BMO), without a benzene ring was synthesized through a one-step aldehyde–ketone condensation reaction.
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Incorporating trifunctional 1,6-heptadiyne moiety into polyacetylene ionomer for improving its physical and conductive properties

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Polym. Chem., 2020, Advance Article
DOI: 10.1039/D0PY00109K, Paper
Hongfei Li, Hengchen Zhang, Xiaojuan Liao, Ruyi Sun, Meiran Xie
A trifunctional diyne comonomer can regulate the structure and optimize the physical state of polyacetylene ionomers, which exhibit a high ionic conductivity of 2.6 × 10−5–1.0 × 10−3 S cm−1 at 30 °C.
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Outstanding Reviewers for Polymer Chemistry in 2019

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Polym. Chem., 2020, 11,2774-2774
DOI: 10.1039/D0PY90061C, Editorial

We would like to take this opportunity to highlight the Outstanding Reviewers for Polymer Chemistry in 2019, as selected by the editorial team for their significant contribution to the journal.
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Aromatic thioketone-mediated radical polymerization of methacrylates and the preparation of amphiphilic quasi-block copolymers

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Polym. Chem., 2020, Advance Article
DOI: 10.1039/D0PY00322K, Paper
Haoyu Yu, Jianwei Shao, Dong Chen, Li Wang, Wantai Yang
TfXT exhibits strong ability to control radical polymerization of methyl methacrylate and has been used in preparing amphiphilic quasi-block copolymer.
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Alternating ring-opening copolymerization of epoxides with saturated and unsaturated cyclic anhydrides: reduced viscosity poly(propylene fumarate) oligomers for use in cDLP 3D printing

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Polym. Chem., 2020, Advance Article
DOI: 10.1039/D0PY00453G, Paper
Yongjun Shin, Matthew L. Becker
A ring-opening copolymerization of propylene oxide with saturated and unsaturated anhydrides using Mg(BHT)2(THF)2 catalyst followed by an isomerization yields poly(propylene fumarate) (PPF) oligomers with improved properties for 3D printing.
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Sequential and alternating RAFT single unit monomer insertion: model trimers as the guide for discrete oligomer synthesis

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Polym. Chem., 2020, Advance Article
DOI: 10.1039/D0PY00390E, Paper
Ruizhe Liu, Lei Zhang, Zixuan Huang, Jiangtao Xu
A complete set of model trimers and their synthetic kinetics are established to guide the synthesis of diverse sequence-defined polymers.
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Self-assembly of strawberry-like organic–inorganic hybrid particle clusters with directionally distributed bimetal and facile transformation of the core and corona

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Published On ::

Polym. Chem., 2020, Advance Article
DOI: 10.1039/D0PY00237B, Paper
Shuxing Mei, Mingwang Pan, Juan Wang, Xiaopeng Zhang, Shaofeng Song, Chao Li, Gang Liu
Controllable structure of organic–inorganic hybrid particle clusters were successfully fabricated by self-assembly which derived from the strong interaction between carboxyl groups of the organic particles and amino groups of the inorganic particles.
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Multi-photon polymerization of bio-inspired, thymol-functionalized hybrid materials with biocompatible and antimicrobial activity

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Polym. Chem., 2020, Advance Article
DOI: 10.1039/D0PY00281J, Communication
Open Access
Kostas Parkatzidis, Maria Chatzinikolaidou, Eleftherios Koufakis, Maria Kaliva, Maria Farsari, Maria Vamvakaki
Thymyl-methacrylate functionalized, hybrid 3D scaffolds, fabricated by multi-photon lithography, exhibit excellent biocompatibility and antimicrobial action for bone and dental tissue engineering.
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Epoxy-functional diblock copolymer spheres, worms and vesicles via polymerization-induced self-assembly in mineral oil

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Polym. Chem., 2020, Advance Article
DOI: 10.1039/D0PY00380H, Paper
Philip J. Docherty, Chloé Girou, Matthew J. Derry, Steven P. Armes
Epoxy-functional poly(stearyl methacrylate)-poly(glycidyl methacrylate) spheres, worms or vesicles can be prepared by RAFT dispersion polymerization of glycidyl methacrylate in mineral oil at 70 °C.
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Comprehensive theoretical and experimental study of near infrared absorbing copolymers based on dithienosilole

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Published On ::

Polym. Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0PY00330A, Paper
Katarzyna Brymora, Wissem Khelifi, Sylvie Blanc, Lionel Hirsch, Antoine Bousquet, Christine Lartigau-Dagron, Frederic Castet
In recent contributions [Eur. Polym. J. 2013, 49, 4176; Macromolecules 2019, 52, 13, 4820], we reported a series of low band gap copolymers with the objective of shifting the absorption...
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Correction: Flow-facilitated ring opening metathesis polymerization (ROMP) and post-polymerization modification reactions

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Polym. Chem., 2020, Advance Article
DOI: 10.1039/D0PY90065F, Correction
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Selesha I. Subnaik, Christopher E. Hobbs
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Photo-induced copper mediated copolymerization of activated-ester methacrylate polymers and their use as reactive precursors to prepare multi-dentate ligands for the water transfer of inorganic nanoparticles

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Polym. Chem., 2020, 11,2969-2985
DOI: 10.1039/D0PY00212G, Paper
Binh T. Mai, Markus J. Barthel, Aidin Lak, Tommaso Avellini, Ana Maria Panaite, Emille M. Rodrigues, Luca Goldoni, Teresa Pellegrino
Polymers bearing activated ester groups are synthesized using photo-ATRP and used as precursors for direct synthesis of multi-phosphonic acid functionalized ligands which are able to transfer different nanoparticles with distinct cores into water.
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Viscoelastic and thermoreversible networks crosslinked by non-covalent interactions between “clickable” nucleic acid oligomers and DNA

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Published On ::

Polym. Chem., 2020, 11,2959-2968
DOI: 10.1039/D0PY00165A, Paper
Alex J. Anderson, Heidi R. Culver, Stephanie J. Bryant, Christopher N. Bowman
An approach to efficient and scalable production of oligonucleotide-based gel networks is presented.
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Effects of tacticity and chiral center-to-dipole distance on mesogen-free liquid crystalline self-assembly of sulfonyl-containing comb-like polymers

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Published On ::

Polym. Chem., 2020, 11,3018-3031
DOI: 10.1039/D0PY00199F, Paper
Caleb A. Bohannon, Man-Hin Kwok, Ruipeng Li, Lei Zhu, Bin Zhao
Mesogen-free comb-like polyethers bearing strongly interacting mono- and di-sulfonylated side chains exhibit well-defined liquid crystalline self-assembly.
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Development and disassembly of single and multiple acid-cleavable block copolymer nanoassemblies for drug delivery

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Published On ::

Polym. Chem., 2020, 11,2934-2954
DOI: 10.1039/D0PY00234H, Review Article
Arman Moini Jazani, Jung Kwon Oh
Acid-degradable block copolymer-based nanoassemblies are promising intracellular candidates for tumor-targeting drug delivery as they exhibit the enhanced release of encapsulated drugs through their dissociation.
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Synthesis of well-defined heteroglycopolymers via combining sequential click reactions and PPM: the effects of linker and heterogeneity on Con A binding

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Polym. Chem., 2020, 11,3054-3065
DOI: 10.1039/D0PY00302F, Paper
Meina Liu, Xingyou Wang, Dengyun Miao, Caiyun Wang, Wei Deng
A versatile post- polymerization modification strategy to synthesize well-defined glycopolymers via the combination of RAFT polymerization and sequential CuAAC and thiol–ene click reactions was developed.
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Metal-free polycycloaddition of aldehyde-activated internal diynes and diazides toward post-functionalizable poly(formyl-1,2,3-triazole)s

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Published On ::

Polym. Chem., 2020, 11,3075-3083
DOI: 10.1039/D0PY00193G, Paper
Baixue Li, Anjun Qin, Ben Zhong Tang
A metal-free polycycloaddition of aldehyde-activated internal diynes and diazides was successfully established and post-functionalizable poly(formyl-1,2,3-triazole)s were readily produced.
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Two-stage thiol-based click reactions for the preparation and adhesion of hydrogels

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Published On ::

Polym. Chem., 2020, 11,2986-2994
DOI: 10.1039/C9PY01503E, Paper
Wen Jing Yang, Wenya Xu, Xi Tao, Wen Wang, Yaqin Hu, Xue Li, En-Tang Kang, Lianhui Wang
Two-stage thiol-based click reactions have been employed as a facile strategy for hydrogel preparation and self-adhesion.
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Synthesis, thermoresponsivity and multi-tunable hierarchical self-assembly of multi-responsive (AB)mC miktobrush-coil terpolymers

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Published On ::

Polym. Chem., 2020, 11,3003-3017
DOI: 10.1039/D0PY00245C, Paper
Xiaomin Zhu, Jian Zhang, Cheng Miao, Siyu Li, Youliang Zhao
Stimuli-responsive miktobrush-coil terpolymers can exhibit unique physical properties and hierarchical self-assembly behaviors dependent on composition, concentration and external stimuli.
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Gold nanoparticles standing on PEG/PAMAM/thiol-functionalized nanographene oxide as aqueous catalysts

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Published On ::

Polym. Chem., 2020, Advance Article
DOI: 10.1039/D0PY00471E, Paper
Bingjie Hao, Guolin Lu, Sen Zhang, Yongjun Li, Aishun Ding, Xiaoyu Huang
Gold nanoparticles were aptly in situ grown on PEG/PAMAM/thiol-functionalized nanographene oxide platforms for aqueous catalysis.
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Construction of polyphosphoesters with the main chain of rigid backbones and stereostructures via organocatalyzed ring-opening polymerization

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Published On ::

Polym. Chem., 2020, Advance Article
DOI: 10.1039/D0PY00262C, Paper
Yu-Jia Zheng, Guan-Wen Yang, Bo Li, Guang-Peng Wu
A highly stereoregular polyphosphoester with a rigid cyclohexylene structure in the main chain was constructed via ring-opening polymerization (ROP) in the presence of an organic catalyst system.
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Effect of the side, ethylene glycol and hydroxyl groups on the polymerization kinetics of oligo(ethylene glycol methacrylates). An experimental and modeling investigation

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Published On ::

Polym. Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0PY00498G, Paper
Mohammad Siddiqui, Dimitris Achilias, Halim Hamid Redhwi
Polymers based on methacrylates bearing short oligo(ethylene glycol) side parts constitute a modern class of stimuli-responsive, biocompatible materials exhibiting several important biological applications. A study of their polymerization kinetics considering...
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Light and Latex: Advances in the photochemistry of polymer colloids

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Published On ::

Polym. Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0PY00349B, Review Article
Philip Scott, Christopher Kasprzak, Keyton Feller, Viswanath Meenakshisundaram, Christopher Williams, Timothy Long
Unparalleled temporal and spatial control of colloidal chemical processes introduces immense potential for the manufacturing, modification, and manipulation of latex particles. This review highlights major advances in photochemistry, both as...
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Morphological Evolution and Mechanical Properties of "Anchor Chain" Nanodomain Structure of Reactive Amphiphilic Triblock Copolymer in Epoxy Resin

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Published On ::

Polym. Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0PY00365D, Paper
Quan Zhou, Qi Liu, Yueru Yu, Yuxiao Zhuang, Yizhe Lv, Hanliang Xiao, Ning Song, Lizhong Ni
A novel epoxy-reactive amphiphilic poly(3,4-epoxy cyclohexyl methyl methacrylate)-block-poly(dimethylsiloxane)-block-poly(3,4-epoxy cyclohexylmethyl methacrylate) (PMETHB-b-PDMS-b-PMETHB) triblock polymer was synthesized via atomic transfer radical polymerization (ATRP) with a controlled molecular chain length and low dispersion,...
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Organocatalyzed ring opening polymerization of regio-isomeric lactones: reactivity and thermodynamics considerations

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Published On ::

Polym. Chem., 2020, Accepted Manuscript
DOI: 10.1039/C9PY01777A, Paper
Marie A. F. Delgove, Ola Wróblewska, Jules Stouten, Christian A. M. R. van Slagmaat, Jurrie Noordijk, Stefaan de Wildeman, Katrien V. Bernaerts
Organocatalysts are increasingly gaining attention for the ring opening polymerization (ROP) of lactones due to numerous advantages. In this work, the goal is to expand the scope of catalysts for...
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Diphenyl Functional Porphyrins and Their Metal Complexes as Visible-Light Photoinitiators for Free-Radical, Cationic and Thiol-Ene Polymerizations

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Published On ::

Polym. Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0PY00468E, Paper
Davy-Louis Versace, Yusuf Yagci, Agata Blacha-Grzechnik, Nicolas Bogliotti, V. Brezova, Jean-Pierre Malval, Marc Presset, Hugo Marcille
This investigation demonstrates the excellent photoinitiating properties of novel visible-light absorbing diphenylporphyrins (DPPs) for the free-radical (FRP), cationic (CP) and thiol-ene polymerizations under visible LEDs irradiation (405 and 530 nm)...
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Precise Tracking and Modulating Aggregation Structures of Conjugated Copolymers in Solutions

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Polym. Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0PY00456A, Paper
Zi-Yuan Wang, Ze-Fan Yao, Yang Lu, Li Ding, Zi-Di Yu, Hao-Yang You, Xin-Yi Wang, Yang-Yang Zhou, Lin Zou, Jie-Yu Wang, Jian Pei
The effects of the backbone shape of the conjugated polymers on the aggregation features in solutions, and further on the morphology in solid states are rarely reported. Herein, four copolymers,...
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Alkene-Azide Chemistry: A Facile, One-Step, Solvent- and Catalyst-Free Approach for Developing New Functional Monomers and Polymers

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Published On ::

Polym. Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0PY00346H, Paper
Santimukul Santra, Ren Bean, Blaze Heckert, Zachary Shaw, Vedant Jain, Lok Shrestha, Raghunath Narayanam, Quentin Austin
In this study, a one-step Hüisgen 1,3-dipolar cycloaddition reaction, alkene-azide chemistry, was explored using a solvent and catalyst free method forming 1,2,3-triazoline ring-containing molecules. This facile method was utilized by...
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Ring-opening copolymerization of cyclic epoxide and anhydride using a five-coordinate chromium complex with a sterically demanding amino triphenolate ligand

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Polym. Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0PY00155D, Paper
Ho Kyun Ryu, Dae Young Bae, Hyeongi Lim, Eunsung Lee, Kyung-sun Son
An alternating ring-opening copolymerization (ROCOP) of epoxides (cyclohexene oxide, limonene oxide) and anhydrides (phthalic anhydride, naphthalic anhydride and maleic anhydride) was performed using a chromium complex containing a sterically demanding...
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Highly conductive mechanically robust high Mw polyfluorene anion exchange membrane for alkaline fuel cell and water electrolysis application

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Published On ::

Polym. Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0PY00334D, Paper
Shoji Miyanishi, Takeo Yamaguchi
New, high molecular weight poly-(fluorene-alt-tetrafluorophenylene) anion exchange membranes were synthesized by a Pd-catalyzed C–H activation method. The synthesized membranes exhibited high OH− conductivity over 100 mS/cm, and membrane swelling could...
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Income Splitting: Opportunities and Pitfalls

By www.cch.ca
Published On :: Mon, 07 Jul 2014 09:28:21 GMT

In this webinar, the tax lawyers of Minden Gross LLP will provide a practical overview of income splitting strategies available today. This webinar will review in detail the various attribution rules devised to thwart income planning, and guide participants to strategies still available for safe and effective income splitting.

Available Sessions for this Seminar:

May 12, 2015 12:00 PM - 2:00 PM EST


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The burden: fossil fuel, the military and national security

By library.mit.edu
Published On :: Sun, 10 Jan 2016 06:17:19 EST

Hayden Library - HD9502.U52 B864 2014


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The girls in the band /

By library.mit.edu
Published On :: Sun, 28 Aug 2016 06:09:33 EDT

Hayden Library - ML82.G57 2014


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Awake: the life of Yogananda

By library.mit.edu
Published On :: Sun, 28 Aug 2016 06:09:33 EDT

Hayden Library - BP605.S43 Y6 2014


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Band of brothers

By library.mit.edu
Published On :: Sun, 18 Sep 2016 06:08:07 EDT

Hayden Library - PN1992.77.B274 A1 2014


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Great unsung women of computing: the computers, the coders and the future makers

By library.mit.edu
Published On :: Sun, 18 Dec 2016 06:33:13 EST

Hayden Library - QA76.2.A2 G74 2016


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Homeland.

By library.mit.edu
Published On :: Sun, 25 Dec 2016 06:35:37 EST

Hayden Library - PN1992.77.H58 A1 2014


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