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Cage-like silsesquioxanes-based hybrid materials

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Dalton Trans., 2020, 49,5396-5405
DOI: 10.1039/D0DT00587H, Perspective
Yajing Du, Hongzhi Liu
This Perspective reviews recent advances in cage-like silsesquioxanes-based hybrid materials, ranging from monomer functionalization and materials preparation to application.
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Phase transition tuning by Fe(III)/Co(III) substitution in switchable cyano-bridged perovskites: (C3H5N2)2[KFexCo1−x(CN)6]

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Dalton Trans., 2020, 49,5503-5512
DOI: 10.1039/D0DT00615G, Paper
Magdalena Rok, Marcin Moskwa, Andrzej Pawlukojć, Rafał Janicki, Iga Zuba, Piotr Zieliński, Paweł Sobieszczyk, Grażyna Bator
The single-crystals of mixed (C3H5N2)2[KFexCo1−x(CN)6] crystals, with different ratios of x = 0, 0.29, 0.42, 0.51, 0.63, 0.70, 0.85, and 1, have been grown from aqueous solutions.
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Enhanced piezoelectric properties of (1 − x)BiFe0.98(Zn0.5Hf0.5)0.02O3-xBaTiO3 ceramics near the morphotropic phase boundary

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Dalton Trans., 2020, 49,5573-5580
DOI: 10.1039/C9DT04664J, Paper
Yunjing Shi, Hairui Bai, Fei Yan, Rui Hu, Kaikai Chen, Bo Shen, Jiwei Zhai
The component with the R–T phase coexistence near MPB affords an optimal piezoelectric coefficient (d33) of 130 pC N−1.
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Hierarchical Mo-doped CoP3 interconnected nanosheet arrays on carbon cloth as an efficient bifunctional electrocatalyst for water splitting in an alkaline electrolyte

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Dalton Trans., 2020, 49,5563-5572
DOI: 10.1039/D0DT00671H, Paper
Shasha Zhang, Mingjing Guo, Shuyi Song, Ke Zhan, Ya Yan, Junhe Yang, Bin Zhao
Hierarchical Mo-doped CoP3 nanosheet arrays were fabricated on carbon cloth to serve as an efficient and robust bifunctional electrocatalyst for overall water splitting in alkaline media.
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Facile synthesis of porous Co3O4 nanoflakes as an interlayer for high performance lithium–sulfur batteries

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Dalton Trans., 2020, 49,5677-5683
DOI: 10.1039/D0DT00429D, Paper
Xiao-Xiao Zheng, Shi-Xi Zhao, Jin-Lin Yang, Yi-Ming Lu, Qi-Long Wu, Xiang-Tian Zeng
Co3O4 nanoflakes were fabricated using oil bath and calcination methods. Lithium–sulfur batteries with Co3O4–super P interlayer exhibited better performance attributed to the synergistic effects of Co3O4–super P.
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Enhanced conductivity and structure stability of BiPO4@void@C/CNT particles for high-performance bismuth-based batteries

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Dalton Trans., 2020, 49,5636-5645
DOI: 10.1039/D0DT00480D, Paper
Ping Feng, Shu-Ang He, Zhe Cui, Qian Liu, Rujia Zou
By homogeneously confining Bi nanoparticles in Li3PO4 matrix nanorods, an anode based on BiPO4@void@C/CNT composite exhibits a reversible capacity of ∼347.0 mA h g−1 at a high current density of 1000 mA g−1 after 530 cycles.
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Carbazole-based green and blue-BODIPY dyads and triads as donors for bulk heterojunction organic solar cells

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Dalton Trans., 2020, 49,5606-5617
DOI: 10.1039/D0DT00637H, Paper
Jian Yang, Charles H. Devillers, Paul Fleurat-Lessard, Hao Jiang, Shifa Wang, Claude P. Gros, Gaurav Gupta, Ganesh D. Sharma, Haijun Xu
Two BODIPY derivatives with one (B2) and two (B3) carbazole moieties were synthesized and applied as electron-donor materials in organic photovoltaic cells (OPV), showing an overall PCE of 6.41% and 7.47%, respectively.
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Bulky bis(aryl)triazenides: just aspiring amidinates? A structural and spectroscopic study

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Dalton Trans., 2020, 49,5653-5661
DOI: 10.1039/D0DT00285B, Paper
Matthew R. Gyton, Anthony R. Leverett, Marcus L. Cole, Alasdair I. McKay
The triazenide ligand is compared to the isoelectronic formamidinate with regards donor capacity, coordination chemistry and capacity to stabilise reactive main group species.
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Diamidophosphites from β-hydroxyamides: readily assembled ligands for Pd-catalyzed asymmetric allylic substitution

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Dalton Trans., 2020, 49,5625-5635
DOI: 10.1039/D0DT00741B, Paper
Ilya V. Chuchelkin, Konstantin N. Gavrilov, Nataliya E. Borisova, Alexander M. Perepukhov, Alexander V. Maximychev, Sergey V. Zheglov, Vladislav K. Gavrilov, Ilya D. Firsin, Vladislav S. Zimarev, Igor S. Mikhel, Victor A. Tafeenko, Elena V. Murashova, Vladimir V. Chernyshev, Nataliya S. Goulioukina
Novel diamidophosphites based on β-hydroxyamides were prepared, and their individual and in situ formed complexes were tested in Pd-mediated allylations.
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Coinage metal tris(dialkylamido)imidophosphorane complexes as transmetallation reagents for cerium complexes

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Dalton Trans., 2020, 49,5420-5423
DOI: 10.1039/D0DT00842G, Communication
Luis M. Aguirre Quintana, Ningxin Jiang, John Bacsa, Henry S. La Pierre
The synthesis of coinage metal tris(dialkylamido)imidophosphorane complexes is reported, and the use of the silver(I) salt as an oxidative transmetallation reagent for the formation of a cerium(IV) complex is described.
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Trinuclear Mn2+/Zn2+ based microporous coordination polymers as efficient catalysts for ipso-hydroxylation of boronic acids

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Dalton Trans., 2020, 49,5454-5462
DOI: 10.1039/D0DT00794C, Paper
Sanchay J. Bora, Rima Paul, Anurag Dutta, Shyam Goswami, Ankur K. Guha, Ashim J. Thakur
Two efficient catalysts based on trinuclear Mn(II)/Zn(II) clusters were synthesized and used for ipso-hydroxylation of phenylboronic acids into the corresponding phenols with excellent yields.
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A bimetallic MOF@graphene oxide composite as an efficient bifunctional oxygen electrocatalyst for rechargeable Zn–air batteries

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Dalton Trans., 2020, 49,5730-5735
DOI: 10.1039/D0DT00976H, Paper
Yao Xiao, Beibei Guo, Jing Zhang, Chun Hu, Ruguang Ma, Deyi Wang, Jiacheng Wang
A bimetallic ZnCo-ZIF@graphene oxide (ZnCo-ZIF@GO) composite was synthesized via an in situ growth strategy. As the air cathode of Zn–air batteries, ZnCo-ZIF@GO showed good charge/discharge performance and long-term stability.
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Two novel lead-based coordination polymers for luminescence sensing of anions, cations and small organic molecules

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Dalton Trans., 2020, 49,5695-5702
DOI: 10.1039/D0DT00533A, Paper
Xue-Yan Zhao, Bing Liang, Ke-Cai Xiong, Yu-Wen Shi, Si-Lei Yang, Ting-Yu Wei, Hui Zhang, Qing-Fu Zhang, Yan-Li Gai
A novel lead-based compound is reported as a multi-responsive luminescent sensor for detecting anions, cations and small organic molecules, especially Cr2O72−, CrO42−, Fe3+ and nitrobenzene.
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Photo-reduction enables catalyst regeneration in Fenton reaction on an Fe2O3-decorated TiO2 nanotube-based photocatalyst

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Dalton Trans., 2020, Advance Article
DOI: 10.1039/D0DT00670J, Paper
Quanming Peng, Guiming Peng, Liangpeng Wu, Yaqian Chen, Bin Han, Qiucheng Su, Shijun Liu, Xinjun Li
Active Fe2+ sites of TNT(Pd)/Fe2O3 with a unique electronic structure for the Fenton reaction can be self-generated.
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A novel self-assembled-derived 1D MnO2@Co3O4 composite as a high-performance Li-ion storage anode material

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Dalton Trans., 2020, Advance Article
DOI: 10.1039/D0DT00980F, Paper
Zongtang Li, Xiao Lian, Mingzai Wu, Fangcai Zheng, Yuanhao Gao, Helin Niu
Manganese dioxide (MnO2) is a high-performance anodic material and applied widely in lithium-ion batteries (LIBs).
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Reply to the ‘Comment on “Investigation on the structure and thermoelectric properties of CuxTe binary compounds”’ by A. H. Barajas-Aguilar, A. M. Garay-Tapia, and S. J. Jiménez-Sandoval, Dalton Trans., 2020, 49, DOI: 10.1039/C9DT03607E

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Dalton Trans., 2020, 49,5738-5740
DOI: 10.1039/D0DT00412J, Comment
Shriparna Mukherjee, Raju Chetty, P. V. Prakash Madduri, Ajaya K. Nayak, Krzysztof Wojciechowski, Tanmoy Ghosh, Kamanio Chattopadhyay, Satyam Suwas, Ramesh Chandra Mallik
In a communication to Dalton Transaction and in a paper in Journal of Physics: Condensed Matter, Aarón H. Barajas-Aguilar et al. have raised comments on our paper published earlier in Dalton Transactions.
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Self-assembled gold nanoparticles and amphiphile peptides: a colorimetric probe for copper(II) ion detection

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Dalton Trans., 2020, Advance Article
DOI: 10.1039/D0DT00844C, Paper
Juliane N. B. D. Pelin, Charlotte J. C. Edwards-Gayle, Herculano Martinho, Barbara B. Gerbelli, Valeria Castelletto, Ian W. Hamley, Wendel A. Alves
We show that arginine/phenylalanine based peptides can be used to control the aggregation of gold nanoparticles in different ways. The arrangement provides a colorimetric approach to detect Cu2+ ions in water.
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Self-assembly of mixed-valent and heterometallic metallocycles: efficient catalyst for oxidation of alcohols to aldehydes with ambient air

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Dalton Trans., 2020, Accepted Manuscript
DOI: 10.1039/D0DT01340D, Communication
Ya-Liang Lai, Xue-Zhi Wang, Rui-Rong Dai, Yong-Liang Huang, Xian-Chao Zhou, Xiao-Ping Zhou, Dan Li
Two mixed-valent CuII/CuI and two heterometallic CuII/AgI metallocycles have been synthesized by the assembly of designed metalloligands and CuI/AgI ions, respectively. The CuII/CuI metallocycle can catalyze oxidation of alcohols to...
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Water-locking molecule-assisted fabrication of natural-inspired Mg(OH)2 for high-efficient and economical uranium capture

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Dalton Trans., 2020, Accepted Manuscript
DOI: 10.1039/D0DT00618A, Paper
Hengbin Xu, Zhenyuan Bai, Milin Zhang, Jun Wang, Yongde Yan, Min Qiu, Jiaming Chen
With the depletion of uranium terrestrial deposits, researchers have focused on the development of adsorbents to extract radioactive uranium from seawater/wastewater. However, there are still considerable challenges to manipulate this...
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An ultra-effective pathway for fully removing the oxygen components of graphene oxide by a flame-assisted microwave process

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Dalton Trans., 2020, Accepted Manuscript
DOI: 10.1039/D0DT01483D, Communication
Xuefeng Zou, Qin Hu, Hengxiu Yang, Feng Chen, Bin Xiang, Xinyue Liang, Qibing Wu, Hujun Shen
Here we report an ultra-effective, reliable pathway to reduce GO into graphene by an about 4-seconds flame-assisted microwave process. A holey graphene with a C/O atom ratio of 31.1, a...
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Influence of Eu valence in the optical activity of BaTiO3 decorated with CaF2 synthesized by microwave-assisted hydrothermal method

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Dalton Trans., 2020, Accepted Manuscript
DOI: 10.1039/D0DT01321H, Paper
Tatiane Strelow Lilge, Adriano Borges Andrade, Claudiane dos Santos Bezerra, Giordano Frederico da Cunha Bispo, Zélia Soares Macedo, Mario Lucio Lúcio Moreira, Mário Ernesto Giroldo Valerio
Inorganic hybrid materials are promising applications in absorbers and photon harvesting of solar irradiation, such as DSSC cell photoanodes. Moreover, the investigation of the interaction between the photoanode constituent materials...
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Luminescent organic dyes containing a phenanthro[9,10-D]imidazole core and [Ir(N^C)(N^N)]+ complexes based on the cyclometalating and diimine ligands of this type

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Dalton Trans., 2020, Advance Article
DOI: 10.1039/D0DT00568A, Paper
Anastasia I. Solomatina, Kirill M. Kuznetsov, Vladislav V. Gurzhiy, Vladimir V. Pavlovskiy, Vitaly V. Porsev, Robert A. Evarestov, Sergey P. Tunik
New N^N and N^C luminescent ligands with solvatochromic behavior and their iridium complexes were synthesized, characterized and investigated.
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MnO2 flowery nanocomposites for efficient and fast removal of mercury(II) from aqueous solution: a facile strategy and mechanistic interpretation

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Dalton Trans., 2020, Advance Article
DOI: 10.1039/D0DT01054E, Paper
Sankar Das, Arnab Samanta, Kanika Kole, Gautam Gangopadhyay, Subhra Jana
MnO2 flowery nanocomposites were explored as a novel and cost effective nanoadsorbent for the fast and efficient extraction of toxic inorganic contaminants from aqueous solution.
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Amorphous Ni–Fe–Se hollow nanospheres electrodeposited on nickel foam as a highly active and bifunctional catalyst for alkaline water splitting

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Dalton Trans., 2020, Advance Article
DOI: 10.1039/C9DT04755G, Paper
Xuerui Yi, Xiaobo He, Fengxiang Yin, Biaohua Chen, Guoru Li, Huaqiang Yin
The electrodeposition of amorphous Ni–Fe–Se hollow nanospheres as a highly efficient bifunctional catalyst for the sustainable production of hydrogen.
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Rapid mechanochemical synthesis of metal–organic frameworks using exogenous organic base

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Dalton Trans., 2020, Advance Article
DOI: 10.1039/D0DT01240H, Paper
Zihao Wang, Zongzhe Li, Marcus Ng, Phillip J. Milner
We describe the mechanochemical, solvent-free synthesis of metal–organic frameworks using liquid organic base for the first time.
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Tin based organic-inorganic hybrid semiconductors with reversible phase transition and dielectric anomaly

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Dalton Trans., 2020, Accepted Manuscript
DOI: 10.1039/D0DT01401J, Paper
Zhenhong Wei, Xiuli You, Jiaojiao Yao
Organic−inorganic hybrid materials with perovskite structure have recently attracted tremendous interest due to their structural tunability and rich functional properties, such as phase transition and photoelectric properties. Within this context,...
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Oxacalix[4]arene Derived Dual Sensing Fluorescence Probe for the Detection of As (V) and Cr (VI) Oxyanions in Aqueous Media

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Dalton Trans., 2020, Accepted Manuscript
DOI: 10.1039/D0DT00452A, Paper
Shuvankar Dey, Anshu Kumar, Pradip Mondal, Krunal M. Modi, Deepak Chopra, Vinod K. Jain
An oxacalix[4]arene-Ce (III) complex viz. L-Ce(III) has been introduced for selective detection of As (V) and Cr (VI) oxyanions in aqueous medium. Binding mode of L-Ce(III) + AsO43-/ CrO42- was...
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A molecular boron cluster-based chromophore with dual emission

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Dalton Trans., 2020, Advance Article
DOI: 10.1039/D0DT00826E, Paper
Kierstyn P. Anderson, Mary A. Waddington, Gary J. Balaich, Julia M. Stauber, Nicholas A. Bernier, Justin R. Caram, Peter I. Djurovich, Alexander M. Spokoyny
Bromination of the luminescent borane, anti-B18H22, via electrophilic substitution using AlCl3 and Br2, yields the monosubstituted derivative 4-Br-anti-B18H21 as an air-stable crystalline solid.
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Amide and ester derivatives of chlorido[4-carboxy-1,2-disalicylideneaminobenzene]iron(III) as necroptosis and ferroptosis inducers

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Dalton Trans., 2020, Advance Article
DOI: 10.1039/D0DT00168F, Paper
Daniel Baecker, Benjamin N. Ma, Jessica Sagasser, Lukas Schultz, Carina Hörschläger, Maria Weinreich, Lucy Steiner, Brigitte Kircher, Ronald Gust
Amide and ester derivatives of chlorido[4-carboxy-1,2-disalicylideneaminobenzene]iron(III) were synthesized and characterized as necroptosis and ferroptosis inducers using the acute myeloid leukemia cell line HL-60.
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Reactive metallocene cations as sensitive indicators of gas-phase oxygen and water

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Dalton Trans., 2020, Advance Article
DOI: 10.1039/D0DT00798F, Paper
Anuj Joshi, Sofia Donnecke, Ori Granot, Dongju Shin, Scott Collins, Irina Paci, J. Scott McIndoe
Gas-phase oxidation of air-sensitive organometallic compounds does not proceed to a significant extent in mass spectrometric analysis unless a vacant coordination site is generated, making nitrogen generators a suitable source of desolvation gas.
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Two [Ln4] molecular rings folded as compact tetrahedra

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Dalton Trans., 2020, Accepted Manuscript
DOI: 10.1039/D0DT01259A, Paper
Guillem Aromi, Olivier Roubeau, Leoní Alejandra Barrios, Jorge Salinas-Uber
The design of photoactive ligands may provide an entry into multifunctional molecular nanomagnets. We report here the design and synthesis of a new multitopic chelating ligand, 1,2-bis-(5-(N’-(pyridine-2-yl-methylene)-carbohydrazide)-3-methyl-thien-3-yl)-cyclopentene (H2L), bearing a...
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Heat-resistant Pb(II)-based X-ray scintillating metal-organic frameworks for sensitive dosage detection via the aggregation-induced luminescent chromophore

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Dalton Trans., 2020, Accepted Manuscript
DOI: 10.1039/D0DT00974A, Communication
Jian Lu, Shuai-Hua Wang, Yan Li, Wen-Fei Wang, Cai Sun, Pei-Xin Li, Fa-Kun Zheng, Guo-Cong Guo
The synergy of unusual X-aggregation induced luminescent chromophores and heavy Pb(II) ions has facilitated excellent X-ray scintillation of two structurally similar Pb-SMOFs, which are heat-resistant due to solvent-free lattices. Owing...
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High Pressure and Elastic properties of a Guanidinium -formate Hybrid Perovskite

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Dalton Trans., 2020, Accepted Manuscript
DOI: 10.1039/C9DT04805G, Paper
Hong-Qiang Gao, Chao Li, Lin-Sui Li, Wen-Juan Wei, Yu-hui Tan, Yun Zhi Tang
The high pressure and elastic properties in a hybrid ABX3-type perovskite, [C(NH2)3][Cd(HCOO)3] (CdGF), based on the A-site guest molecular is revealed via combining the high-pressure synchrotron X-ray diffraction experiments with...
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Spin-frustration with two quasi-degenerated spin states of a copper(II) heptanuclear complex obtained from an amino acid ligand

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Dalton Trans., 2020, Accepted Manuscript
DOI: 10.1039/C9DT04501E, Paper
Catiúcia Rodrigues Marcelino Oliveira Matos, Henrique Silva Jr, Dayenny D’Amato, Guilherme Guedes, Glaucio Braga Ferreira, Odivaldo Cambraia Alves, Filipe Barra de Almeida, Sergio Pinheiro, Acácio Souza, Flavio Garcia, Célia Machado Ronconi
The Cu(II) heptanuclear complex (Cu7atac) was synthesised using the hydrated amino acid ligand 2-(5-amino-1H-1,2,4-triazol-3-yl)acetic acid (Hatac.H2O). Single crystal X-ray diffraction analysis revealed a μ3-hydroxo bridged Cu(II) heptanuclear complex, consisting of...
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Rhenium and technetium-complexed silicon rhodamines as near-infrared imaging probes for bimodal SPECT- and optical imaging

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Dalton Trans., 2020, Accepted Manuscript
DOI: 10.1039/D0DT01084G, Communication
Thines Kanagasundaram, Carsten Sven Kramer, Eszter Boros, Klaus Kopka
Radiolabelled fluorescent dyes are decisive for bimodal imaging and currently in demand for scintigraphic and optical imaging. This powerful method allows the combination of nuclear imaging (e.g. SPECT-imaging) and optical...
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Big History Ebooks Now Available For WH & BHP Classes

By www.berkshirepublishing.com
Published On :: Thu, 09 Jan 2020 09:56:10 +0000

Cynthia Stokes Brown wrote BIG HISTORY, SMALL WORLD to help Big History Project students and their teachers, many of whom she knew and befriended in the earliest days of big history education. David Christian's THIS FLEETING WORLD is widely used in AP World History as well as big history courses. BIG HISTORY: A BERKSHIRE ESSENTIAL is a collection of essays by

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First Look at the T S Eliot – Emily Hale Letters (podcast)

By www.berkshirepublishing.com
Published On :: Wed, 15 Jan 2020 00:36:24 +0000

In what one scholar called “the literary event of the decade,” on 2 January 2020, Princeton University Library opened up more than 1,100 letters that the Nobel-Prize-winning poet T.S. Eliot wrote over the course of three decades to an American speech professor and amateur actress named Emily Hale. The day became even more

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Gastrodiplomacy in China; T S Eliot’s Love Letters

By www.berkshirepublishing.com
Published On :: Fri, 21 Feb 2020 10:04:19 +0000

Chinese food, anyone? I'll be co-presenting a program about gastrodiplomacy at Schwarzman College in Beijing next month, and I am looking for stories to share, from history as well as personal experience. Schwarzman College 苏世民书院 is a residential college at Tsinghua University. Schwarzman scholarships are modeled on the Rhodes Scholarships at Oxford. The one-year MA

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COVID-19 is here (& where has all the toilet paper gone?)

By www.berkshirepublishing.com
Published On :: Tue, 31 Mar 2020 09:19:45 +0000

We lived through the ‘80s. We lived through the ‘90s. We lived through the ‘00s. We lived through the ‘10s. And we’ve lived through March. Most of us, that is, have lived. I’m still coming to terms with what is happening. It’s like grief. I go about my day, getting absorbed in work, or a

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Do exclusionary rules ensure a fair trial?: a comparative perspective on evidentiary rules / Sabine Gless, Thomas Richter, editors

By library.mit.edu
Published On :: Sun, 21 Jul 2019 09:24:23 EDT

Online Resource


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First: Sandra Day O'Connor / Evan Thomas

By library.mit.edu
Published On :: Sun, 28 Jul 2019 10:20:39 EDT

Dewey Library - KF8745.O25 T46 2019


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Real estate finance in a nutshell / Vada Waters Lindsey, Associate Professor of Law, Marquette University Law School

By library.mit.edu
Published On :: Sun, 28 Jul 2019 10:20:39 EDT

Rotch Library - KF695.Z9 L56 2018


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Decarcerating America: from mass punishment to public health / edited by Ernest Drucker

By library.mit.edu
Published On :: Sun, 28 Jul 2019 10:20:39 EDT

Dewey Library - KF9730.D43 2018


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Practitioner's guide to project-based vouchers: a successor to the Beginner's guide / Sarah Molseed and Julie S. McGovern

By library.mit.edu
Published On :: Sun, 28 Jul 2019 10:20:39 EDT

Rotch Library - KF5735.M654 2018


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Networked press freedom: creating infrastructures for a public right to hear / Mike Ananny

By library.mit.edu
Published On :: Sun, 28 Jul 2019 10:20:39 EDT

Dewey Library - K3255.A958 2018


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Gender quotas in South America's big three: national and subnational impacts / Adriana Piatti-Crocker, Gregory D. Schmidt, and Clara Araujo

By library.mit.edu
Published On :: Sun, 4 Aug 2019 10:22:43 EDT

Dewey Library - KH136.W64 P53 2017


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Practical Guide to LTE-A, VoLTE and IoT: Paving the way towards 5G / by Ayman Elnashar, Mohamed El-Saidny

By library.mit.edu
Published On :: Sun, 11 Aug 2019 10:25:18 EDT

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Habeas data: privacy vs. the rise of surveillance tech / Cyrus Farivar

By library.mit.edu
Published On :: Sun, 11 Aug 2019 10:25:18 EDT

Dewey Library - KF1262.F37 2018


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Women as constitution-makers: case studies from the new democratic era / edited by Ruth Rubio-Marín, Helen Irving

By library.mit.edu
Published On :: Sun, 8 Sep 2019 10:29:39 EDT

Dewey Library - K3243.W66 2019


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Analogy and Exemplary Reasoning in Legal Discourse.

By library.mit.edu
Published On :: Sun, 8 Sep 2019 10:29:39 EDT

Online Resource


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