the

Understanding the mechanism of byproduct formation with in operando synchrotron techniques and its effects on the electrochemical performance of VO2(B) nanoflakes in aqueous rechargeable zinc batteries

J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA00858C, Paper
Qiang Pang, Hainan Zhao, Ruqian Lian, Qiang Fu, Yingjin Wei, Angelina Sarapulova, Junqi Sun, Chunzhong Wang, Gang Chen, Helmut Ehrenberg
The byproduct protects the vanadium-based positive electrode of ARZBs and facilitates Zn2+ insertion into the electrode.
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A one-step rapid synthesis of TS-1 zeolites with highly catalytically active mononuclear TiO6 species

J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/C9TA13851J, Paper
Wenjing Xu, Tianjun Zhang, Risheng Bai, Peng Zhang, Jihong Yu
The modulation and determination of the coordination environments of Ti active sites in titanosilicate zeolites are key challenges in the rational design of high-performance heterogeneous catalysts.
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The highly efficient collection of underwater oil droplets on an anisotropic porous cone surface via an electric field

J. Mater. Chem. A, 2020, 8,8605-8611
DOI: 10.1039/D0TA02055A, Paper
Yufeng Yan, Qiuya Zhang, Yan Li, Zhenyan Guo, Dongliang Tian, Xiaofang Zhang, Lei Jiang
The highly efficient collection of underwater oil droplets on an anisotropic porous cone surface via an electric field was demonstrated.
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Achieving a 2.7 V aqueous hybrid supercapacitor by the pH-regulation of electrolyte

J. Mater. Chem. A, 2020, 8,8648-8660
DOI: 10.1039/D0TA02926B, Paper
Lijun Su, Qingnuan Zhang, Yue Wang, Jianing Meng, Yongtai Xu, Lingyang Liu, Xingbin Yan
We present an effective electrolyte pH-regulation strategy for cation-intercalated manganese oxides to extend the voltage window of aqueous supercapacitors.
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Simultaneously improving the photovoltaic parameters of organic solar cells via isomerization of benzo[b]benzo[4,5]thieno[2,3-d]thiophene-based octacyclic non-fullerene acceptors

J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA00451K, Paper
Zhijie Zhou, Jiamin Duan, Linglong Ye, Guo Wang, Bin Zhao, Songting Tan, Ping Shen, Hwa Sook Ryu, Han Young Woo, Yanming Sun
Three isomeric FREAs were synthesized and applied in organic solar cells. The OSC devices based on Z1-bb exhibited a PCE of 12.66%. The isomerization of a fused-ring core could be achieve high-performance OSCs with high Jsc, Voc, and FF.
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Decoupled electrolytes towards enhanced energy and high temperature performance of thermally regenerative ammonia batteries

J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA03236K, Paper
Weiguang Wang, Gequn Shu, Xiuping Zhu, Hua Tian
An electrolyte decoupling strategy is proposed for ammonia batteries to restrain the self-discharge and enhance energy density as well as power generation at high temperatures.
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Inexpensive thermochemical energy storage utilising additive enhanced limestone

J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA03080E, Paper
Kasper T. Møller, Ainee Ibrahim, Craig E. Buckley, Mark Paskevicius
A thermochemical energy storage capacity retention of up to 90% over 500 cycles is achieved in cheap and abundant limestone.
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Co-gel strategy for preparing hierarchically porous silica/polyimide nanocomposite aerogel with thermal insulation and flame retardancy

J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/C9TA13011J, Paper
Xinhai Zhang, Xingxing Ni, Chenxi Li, Bo You, Gang Sun
Co-gel strategy for preparing hierarchically porous silica/polyimide aerogel with low density, high specific modulus, hydrophobicity, flame retardancy, and thermal insulation.
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Optical in-situ monitoring during the synthesis of halide perovskite solar cells reveals formation kinetics and evolution of optoelectronic properties

J. Mater. Chem. A, 2020, Accepted Manuscript
DOI: 10.1039/D0TA01237H, Paper
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Klara Suchan, Justus Just, Pascal Becker, Eva Lisa Unger, Thomas Unold
The formation mechanism and the evolution of optoelectronic properties during annealing of chlorine-derived methylammonium lead iodide (MAPbI3-xClx) is investigated in detail combining in-situ und ex-situ optical and structural characterization. Using...
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Reversible changes in the electronic structure of carbon nanotube-hybrids upon NO2 exposure under ambient conditions

J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA02749A, Paper
Open Access
Filippo Fedi, Oleg Domanov, Hidetsugu Shiozawa, Kazuhiro Yanagi, Paolo Lacovig, Silvano Lizzit, Andrea Goldoni, Thomas Pichler, Paola Ayala
Single-walled carbon nanotubes have enormous potential for gas sensing. This study shows that cluster filling is a key to high sensitivity and it opens the possibility for a very high desorption at ambient temperature.
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Effect of the interfacial protective layer on the NaFe0.5Ni0.5O2 cathode for rechargeable sodium-ion batteries

J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA02837A, Paper
Iqra Moeez, Dieky Susanto, Ghulam Ali, Hun-Gi Jung, Hee-Dae Lim, Kyung Yoon Chung
Ni-based cathode materials have received significant attentions as the advanced electrode materials for NIBs. However, they suffered from the rapid capacity fading due to the side reactions mainly occurring at cathode-electrolyte interphase (CEI).
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The rational and effective design of nonfullerene acceptors guided by a semi-empirical model for an organic solar cell with an efficiency over 15%

J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA03087B, Paper
Xin Ke, Lingxian Meng, Xiangjian Wan, Mingpeng Li, Yanna Sun, Ziqi Guo, Simin Wu, Hongtao Zhang, Chenxi Li, Yongsheng Chen
Guided by a semi-empirical model, two small-molecule acceptors were rationally designed and an impressive PCE of 15.05% was achieved.
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Fe/Fe3C nanoparticle-decorated N-doped carbon nanofibers for improving the nitrogen selectivity of electrocatalytic nitrate reduction

J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA02317E, Paper
Yue Lan, Junliang Chen, Hui Zhang, Wei-xian Zhang, Jianping Yang
N-doped carbon nanofibers embedded with Fe/Fe3C nanodomains demonstrate superior electrocatalytic nitrate reduction ability and nitrogen selectivity.
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Semiconducting polymer contributes favorably to the Seebeck coefficient in multi-component, high-performance n-type thermoelectric nanocomposites

J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA02388D, Paper
Junhui Tang, Ruisi Chen, Lidong Chen, Guillermo C. Bazan, Ziqi Liang
n-Type Co NWs/N2200 TENCs yield a high S, mainly from the semiconducting polymer, yet σ is limited by poor connectivity between inorganic and organic domains. By adding flexible n-doped SWCNTs to yield more conductive paths, σ and mechanical bendability are greatly enhanced.
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the

The nature of the methylamine–MAPbI3 complex: fundamentals of gas-induced perovskite liquefaction and crystallization

J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA02494E, Paper
Dmitry Bogachuk, Lukas Wagner, Simone Mastroianni, Michael Daub, Harald Hillebrecht, Andreas Hinsch
In this work we scrutinize the exact interaction mechanisms between methylamine and perovskite based on extensive experimental evidence.
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Polyimide/ZIF-7 Mixed-Matrix Membranes: Understanding in-situ Confined Formation of ZIF-7 Phases inside Polymer and Their Effects on Gas Separations

J. Mater. Chem. A, 2020, Accepted Manuscript
DOI: 10.1039/D0TA02761H, Paper
Sunghwan Park, Kie Yong Cho, Hae-Kwon Jeong
Polymer-modification-enabled in-situ metal-organic framework formation (PMMOF) is potentially a paradigm-shifting preparation method for polymer/MOF mixed-matrix membranes (MMMs). However, the actual reaction conditions of in-situ formation of MOF in the confined...
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The fabrication of IMo6@iPAF-1 as an enzyme mimic in heterogeneous catalysis for oxidative desulfurization under O2 or air

J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/C9TA14066B, Paper
Yue Li, Jian Song, Mengting Jiang, Mbage Bawa, Xiaohong Wang, Yuyang Tian, Guangshan Zhu
Na5[IMo6O24]·3H2O and a porous aromatic framework (iPAF-1) were used to build an off-the-shelf building material (IMo6@iPAF-1) to realize the highly efficient oxidation of organic sulfurs like oxygenase.
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the

Understanding the structural phase transitions in lithium vanadium phosphate cathode for lithium-ion batteries

J. Mater. Chem. A, 2020, Accepted Manuscript
DOI: 10.1039/C9TA12435G, Paper
Woong Oh, Hyunyoung Park, Bong-Soo Jin, Ranjith Thangavel, Won-Sub Yoon
Developing high-energy lithium-ion batteries with long stability is critical for realizing sustainable energy applications; however, it remains highly challenging. Exploring multi-redox based electrode materials can help to achieve high capacity...
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the

Ultrahigh Photothermal Temperature in Graphene/Conducting Polymer System Enables Contact Thermochemical Reaction

J. Mater. Chem. A, 2020, Accepted Manuscript
DOI: 10.1039/D0TA03347B, Paper
Yuqiao Chai, Hui Ma, Xinlei Ma, Xinyue Zhang, Yonglin He, Yapei Wang, Qianqian Jiang, Xusheng Wang, Junhui Ji, Mianqi Xue
Photothermal conversion in near-infrared (NIR) wavelengths, which converts light energy into heat energy, has caused great concern and been developing rapidly in recent years for its wide applications in health...
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Hydrophilic ultrafiltration membranes with surface-bound eosin Y for an integrated synthesis-separation system of aqueous RAFT photopolymerization

J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA03112G, Paper
Yujie Zhao, Senlin Shao, Jiangbin Xia, Ya Huang, Yu Chi Zhang, Xue Li, Tao Cai
The photocatalyst-based ultrafiltration membrane fitted integrated synthesis–separation system holds the promises to bridge the gap between the precision of PET-RAFT polymerization and the efficiency of membrane separation process.
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the

Exceeding the Volcano Relationship in Oxygen Reduction/Evolution Reactions using Single-atom-based Catalysts with Dual-active-sites

J. Mater. Chem. A, 2020, Accepted Manuscript
DOI: 10.1039/D0TA01399D, Communication
Xiyu Li, Sai Duan, Edward Sharman, Yuan Zhao, Li Yang, Zhiwen Zhuo, Peng Cui, Jun Jiang, Yi Luo
Finding cost-effective catalysts to drive oxygen reduction/evolution reactions (ORR/OER) is a highly attractive goal. Most catalysts follow a volcano relationship of performance, making it difficult to search thoroughly enough among...
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Nitrogen-doped phosphorene for electrocatalytic ammonia synthesis

J. Mater. Chem. A, 2020, Accepted Manuscript
DOI: 10.1039/D0TA03237A, Paper
Guang-Rui Xu, Hao Li, Abdulaziz Bati, Munkhjargal Bat-Erdene, Md Julker Nine, Dusan Losic, Yu Chen, Joseph G Shapter, Munkhbayar Batmunkh, Tianyi Ma
The rapid surface oxidation of phosphorene under ambient conditions is considered to be serious issue for many applications, but here is used as a strategy to achieve efficient heteroatom doping....
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the

Creating compressive stress at the NiOOH/NiO interface for water oxidation

J. Mater. Chem. A, 2020, Accepted Manuscript
DOI: 10.1039/D0TA04244G, Communication
Chunguang Kuai, Yan Zhang, Li-Li Han, Huolin Xin, Chengjun Sun, Dennis Nordlund, Shizhang Qiao, Xiwen Du, Feng Lin
Enhancing the oxygen evolution reaction (OER) performance of NiO materials will greatly expand their applications as low-cost, bifunctional electrocatalysts for water splitting reactions. Introducing stress into the surface layer of...
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Rational Understanding of the Catalytic Mechanism of Molybdenum Carbide on Polysulfide Conversion in Lithium-Sulfur Battery

J. Mater. Chem. A, 2020, Accepted Manuscript
DOI: 10.1039/D0TA01217C, Paper
Mingzhu Sun, Zhao Wang, Xue Li, Haibo Li, Hongsheng Jia, Xiangxin Xue, Ming Jin, Jiaqi Li, Yu Xie, Ming Feng
Lithium-sulfur (Li-S) batteries are promising candidates for next-generation energy storage devices due to its high theoretical energy density, whose practical applications are mainly hampered by the shuttle effect of intermediate...
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The man who was known as 'Snakehips'

By the time he appeared in the film, Snakehips Tucker was already a name attraction in Harlem nightclubs like the Cotton Club and Connie's Inn




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Now Available: Concerts from the Library of Congress

 

You can get tickets for any 2020 event that is part of Concerts from the Library of Congress.

PLEASE NOTE: All films, talks and pre-concert events this year are general admission with no ticket required, unless otherwise indicated. You can still register for reminders and updates about those events, but seating will be first-come, first-served.

Click here for more information.

Request ADA accommodations five business days in advance at (202) 707-6362 or ADA@loc.gov.




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Live! At the Library Event Series Launched

The Library of Congress is extending its public hours on Thursday evenings and will feature regular live programming for visitors as part of a new initiative, Live! At the Library, beginning April 2 to showcase the broad range of literature, poetry, art, music, digital collections and other holdings at the national library.

The Library’s Thomas Jefferson Building and all exhibitions at the Library – currently featuring the long fight for women’s voting rights and Rosa Parks’ groundbreaking role in civil rights – will be open for extended hours on Thursday evenings from 5 to 8 p.m. every week. Exhibitions and programs will remain free and open to everyone. The Main Reading Room will be open for research during this time, and visitors and researchers will have the opportunity to register for reader cards. Other selected reading rooms may also be open on Thursday nights as a part of evening programming.

Click here for more information.

Request ADA accommodations five business days in advance at (202) 707-6362 or ADA@loc.gov.




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NEWS: Library Buildings Closed Until Further Notice

Out of an abundance of caution, all Library of Congress buildings and facilities will be closed to the public, including researchers and others with reader identification cards, until further notice to reduce the risk of transmitting COVID-19 coronavirus. The Library has reduced the number of people in Library buildings to a very small number of necessary individuals.

Click here for more information.




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The Best CSS Spinners & Loaders

Using modern CSS techniques, it has never been easier to create a loader/spinner of any kind. This article showcases over 40 different techniques and styles.




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Prog: On the air.

MEDIA PhonCD ML5.P76 v.89




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Prog: One of the few.

MEDIA PhonCD ML5.P76 v.88




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Betty and the sensory world: experimental electronic music / Doug Bielmeier

MEDIA PhonCD B4763 bet




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All that the man left behind when he died / Daichi Fujiki

MEDIA PhonCD F95509 all




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The book of keyboards / Philippe Manoury

MEDIA PhonCD M3167 chamu




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In the loop / WoodWired

MEDIA PhonCD W878 in




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Into the silence / Nicholas DiEugenio, Mimi Solomon

MEDIA PhonCD D5678 int




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The early immersive music of Joan La Barbara.

MEDIA PhonCD L111 vocmu b




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The Andrée expedition: From the diary of Virginia Woolf / Dominick Argento

MEDIA PhonCD Ar37 song




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Color theory: music for saxophones, percussion and Harry Partch instruments / Prism Quartet, Sō Percussion, Partch

MEDIA PhonCD P937 col




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You're the man / Marvin Gaye

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There is no other / Rhiannon Giddens ; with Francesco Turrisi

MEDIA PhonCD F G3701.C6.G533




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Yiddish glory: the lost songs of World War II.

MEDIA PhonCD F G6967.J4.Y533




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Cat o' nine tails: The dead man ; Memento mori ; Kol nidre / John Zorn

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Prog: Behind the lines

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Phenomenal woman: the Maya Angelou songs ; and, Songs without words / Capathia Jenkins & Louis Rosen

MEDIA PhonCD J R722 phe




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The poetry of places.

MEDIA PhonCD Sh823 poe




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Tasmin Little plays Clara Schumann, Dame Ethel Smyth, Amy Beach.

MEDIA PhonCD L728 tas




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Petite fleur: the music of Sidney Bechet / David Liebman ; John Stowell

MEDIA PhonCD J B387 pet




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Divine theatre: sacred motets / by Giaches de Wert

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Les liaisons dangereuses 1960 / Thelonious Monk

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