J. Mater. Chem. A, 2020, 8,8548-8553
DOI: 10.1039/D0TA02443K, Paper

Rui Ma, Naifang Liu, Ting-Ting Lin, Tianbo Zhao, Sheng-Li Huang, Guo-Yu Yang
Anderson polyoxometalate-based covalent organic frameworks exhibited the highest catalytic activity in the photodegradation of RhB and MB, as well as 100% selective oxidation of sulfides to sulfoxides.
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J. Mater. Chem. A, 2020, 8,8376-8382
DOI: 10.1039/D0TA02033H, Paper

Gang Liu, Hao Cui, Sujuan Wang, Li Zhang, Cheng-Yong Su
A facile synthesis of a series of Fe–oxo chain-based porphyrinic MOFs (namely M-PMOF-3(Fe), M = Fe, Co, Ni, Cu) has been reported.
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J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/C9TA13585E, Paper

Cong Huang, Qunli Tang, Qiushui Feng, Yanhua Li, Yali Xu, Yan Zhang, Aiping Hu, Shiying Zhang, Weina Deng, Xiaohua Chen
An outer–inner dual space utilizing strategy is reported for the fabrication of an ultrahigh volumetric performance polydopamine-coated dopamine/reduced graphene oxide composite film.
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J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA01530J, Review Article

Subramaniam Jayabal, Govindarajan Saranya, Dongsheng Geng, Lu-Yin Lin, Xiangbo Meng
This review aims at providing an overview of the interactions between Pt and supports from experimental and theoretical results, in the hope of correlating the metal–support interactions with the activity and durability of the catalysts in fuel cells.
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J. Mater. Chem. A, 2020, 8,8421-8429
DOI: 10.1039/C9TA13711D, Paper

Hongyu Guo, Jamie A. Trindell, Hao Li, Desiree Fernandez, Simon M. Humphrey, Graeme Henkelman, Richard M. Crooks
Pd_xIr_(100−x) alloys synthesized via a microwave-assisted polyol method serve as an ideal experimental system to improve theoretical insight of the material properties towards the ORR.
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J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA00858C, Paper

Qiang Pang, Hainan Zhao, Ruqian Lian, Qiang Fu, Yingjin Wei, Angelina Sarapulova, Junqi Sun, Chunzhong Wang, Gang Chen, Helmut Ehrenberg
The byproduct protects the vanadium-based positive electrode of ARZBs and facilitates Zn²⁺ insertion into the electrode.
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J. Mater. Chem. A, 2020, 8,8485-8495
DOI: 10.1039/D0TA01901A, Paper

Matthew W. Logan, Spencer Langevin, Bing Tan, Adam W. Freeman, Christopher Hoffman, Douglas B. Trigg, Konstantinos Gerasopoulos
We report UV-cured eutectic gel polymer electrolytes that improve cell performance, non-flammability, and water tolerance compared to the liquid solvent.
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J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/C9TA13851J, Paper

Wenjing Xu, Tianjun Zhang, Risheng Bai, Peng Zhang, Jihong Yu
The modulation and determination of the coordination environments of Ti active sites in titanosilicate zeolites are key challenges in the rational design of high-performance heterogeneous catalysts.
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J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA02027C, Paper

Noho Lee, Junghyeok Kwak, Ji Hye Kwak, Sang-Mun Jung, Jaerim Kim, Anupam Giri, Kaliannan Thiyagarajan, Yong-Tae Kim, Sunshin Jung, Jong Kyu Kim, Unyong Jeong
Although branched WO₃ nanostructures have been investigated for electrochromic devices and catalytic electrodes, a detailed study on their structural evolution mechanism has rarely been carried out.
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J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA02807J, Paper

Cheng Liu, Yi Yang, Xin Liu, Yong Ding, Zulqarnain Arain, Xinye Li, Yuanlong Li, Zian Zhou, Songyuan Dai, Mohammad Khaja Nazeeruddin
Quasi-quantum dots α-CsPbI₃ films are in situ prepared by using a new ligand with ultralow contents. By increasing the film hydrophobicity and surface Gibbs energy, the device with efficiency of 13.5% keeps stable under ambient condition for 30 days.
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J. Mater. Chem. A, 2020, 8,8566-8574
DOI: 10.1039/D0TA01260B, Paper

Chujun Zhang, Jun Yuan, Ka Lok Chiu, Hang Yin, Weifang Liu, Guanhaojie Zheng, Johnny Ka Wai Ho, Suzhen Huang, Gaoxing Yu, Feng Gao, Yingping Zou, Shu Kong So
A disorder-free molecular conformation caused by alkyl side chains facilitates electron transport, heat transfer and reduces electronic disorder.
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J. Mater. Chem. A, 2020, 8,8605-8611
DOI: 10.1039/D0TA02055A, Paper

Yufeng Yan, Qiuya Zhang, Yan Li, Zhenyan Guo, Dongliang Tian, Xiaofang Zhang, Lei Jiang
The highly efficient collection of underwater oil droplets on an anisotropic porous cone surface via an electric field was demonstrated.
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J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA01968B, Paper

Ruihao Chen, Yong Hui, Binghui Wu, Yongke Wang, Xiaofeng Huang, Zhongyuan Xu, Pengpeng Ruan, Wuyong Zhang, Fangwen Cheng, Weijie Zhang, Jun Yin, Jing Li, Nanfeng Zheng
Crown ether effectively stabilizes the cubic phase of CsPbI₃ to inhibit the moisture invasion and phase transformation of CsPbI₃ films, producing large-area devices and improving device performance.
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J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA00451K, Paper

Zhijie Zhou, Jiamin Duan, Linglong Ye, Guo Wang, Bin Zhao, Songting Tan, Ping Shen, Hwa Sook Ryu, Han Young Woo, Yanming Sun
Three isomeric FREAs were synthesized and applied in organic solar cells. The OSC devices based on Z1-bb exhibited a PCE of 12.66%. The isomerization of a fused-ring core could be achieve high-performance OSCs with high J_sc, V_oc, and FF.
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J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA03169K, Paper

Guangping Sun, Weirui Qian, Jianmin Jiao, Tingting Han, Yukun Shi, Xiao-Yu Hu, Leyong Wang
An efficient artificial light-harvesting system with two-step sequential energy transfer has been successfully constructed based on supramolecular self-assembly.
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J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/C9TA13980J, Communication

Jinheng Li, Huixin Zhang, Lingyan Zhang, Ke Wang, Zhengkang Wang, Guiyan Liu, Yanli Zhao, Yongfei Zeng
Two new two-dimensional covalent–organic frameworks are synthesized using a three-connected building block, showing ultrahigh iodine capture capacities of 5.625 g g⁻¹ and 4.820 g g⁻¹ on account of physical–chemical adsorption.
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J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA03080E, Paper

Kasper T. Møller, Ainee Ibrahim, Craig E. Buckley, Mark Paskevicius
A thermochemical energy storage capacity retention of up to 90% over 500 cycles is achieved in cheap and abundant limestone.
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J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA03128C, Paper

Hanjian Lai, Hui Chen, Yulin Zhu, Lin Chen, Hsin-Hsiang Huang, Feng He
This work provides a strategy of symmetry breaking in an A–DAD–A-type acceptor with a PCE of 15.43%, which is the highest value reported to date for asymmetrical fused-ring acceptors.
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J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/C9TA13011J, Paper

Xinhai Zhang, Xingxing Ni, Chenxi Li, Bo You, Gang Sun
Co-gel strategy for preparing hierarchically porous silica/polyimide aerogel with low density, high specific modulus, hydrophobicity, flame retardancy, and thermal insulation.
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J. Mater. Chem. A, 2020, Accepted Manuscript
DOI: 10.1039/D0TA01549K, Paper

Guanjun Chen, Huaqiang Shan, Yan Li, Hongwei Bao, Tingwei Hu, Long Zhang, Shuai Liu, Fei Ma
Alloying Pt with less expensive 3d transition metal to form bimetallic nanoparticles (NPs) has been proven to be an ideal strategy for synthesis of catalysts, especially in the field of...
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J. Mater. Chem. A, 2020, Accepted Manuscript
DOI: 10.1039/D0TA01237H, Paper

Open Access

  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.

Klara Suchan, Justus Just, Pascal Becker, Eva Lisa Unger, Thomas Unold
The formation mechanism and the evolution of optoelectronic properties during annealing of chlorine-derived methylammonium lead iodide (MAPbI3-xClx) is investigated in detail combining in-situ und ex-situ optical and structural characterization. Using...
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J. Mater. Chem. A, 2020, Accepted Manuscript
DOI: 10.1039/D0TA02896G, Review Article

Yaewon Park, Xi Chen
Water-responsive (WR) materials that mechanically change volume in response to changes in relative humidity (RH) can generate significantly higher energy actuation over natural muscles and conventional actuators. Recent proof-of-concept demonstrations...
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J. Mater. Chem. A, 2020, Accepted Manuscript
DOI: 10.1039/D0TA03165H, Paper

Pingge He, Jiaohao Liu, Xudong Zhao, Zhenping Ding, Peng Gao, Li-Zhen Fan
Aqueous zinc ion batteries (ZIBs) have attracted intensive attention due to their low cost, environmental friendliness and high safety. However, exploring suitable cathode materials and deep understanding of their energy...
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J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA02749A, Paper

Open Access

  This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence.

Filippo Fedi, Oleg Domanov, Hidetsugu Shiozawa, Kazuhiro Yanagi, Paolo Lacovig, Silvano Lizzit, Andrea Goldoni, Thomas Pichler, Paola Ayala
Single-walled carbon nanotubes have enormous potential for gas sensing. This study shows that cluster filling is a key to high sensitivity and it opens the possibility for a very high desorption at ambient temperature.
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J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA02499F, Paper

Fei Ye, Xiu Zhang, Kaiming Liao, Qian Lu, Xiaohong Zou, Ran Ran, Wei Zhou, Yijun Zhong, Zongping Shao
A new conceptional lithiophilic polymer-filler-reinforced gel polymer electrolyte was proposed and prepared to guide uniform Li-ion flux during the Li plating/stripping process.
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J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA02833A, Paper

Hongxia Liu, Meng Wang, Jiantai Ma, Gongxuan Lu
New high active low-cost Pd-Sn alloy catalyst for hydrogen evolution from toxic formaldehyde driven by visible light was developed via alloying of Pd with abundance element Sn.
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J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA02710C, Paper

Yifan Kong, Jianmin Li, Zengyang Ma, Zheng Chi, Xudong Xiao
By introducing a pre-deposited CuGaSe₂ layer, a steep Ga back grading has been formed in a submicron CIGS layer with a high-temperature process for the first time.
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J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA03087B, Paper

Xin Ke, Lingxian Meng, Xiangjian Wan, Mingpeng Li, Yanna Sun, Ziqi Guo, Simin Wu, Hongtao Zhang, Chenxi Li, Yongsheng Chen
Guided by a semi-empirical model, two small-molecule acceptors were rationally designed and an impressive PCE of 15.05% was achieved.
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J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA02317E, Paper

Yue Lan, Junliang Chen, Hui Zhang, Wei-xian Zhang, Jianping Yang
N-doped carbon nanofibers embedded with Fe/Fe₃C nanodomains demonstrate superior electrocatalytic nitrate reduction ability and nitrogen selectivity.
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J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA00384K, Paper

Xurui Zhang, Yanxing Zhang, Qingqing Li, Xiaodong Zhou, Qingyu Li, Jin Yi, Yuyu Liu, Jiujun Zhang
Electrochemical reduction of carbon dioxide (ERCO₂) to low-carbon fuel and useful chemicals, which can simultaneously store renewable energy and recover CO₂ in a green manner, has proven to be a viable energy storage and conversion strategy.
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J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA02471F, Paper

Jingjing Jia, Haijun Zhang, Zhongxu Wang, Jingxiang Zhao, Zhen Zhou
By means of first-principles computations, we identified that metallic Cu₂B₂ monolayer with planar heptacoordinate motifs could effectively reduce CO to ethanol through the “carbene” mechanism with a low limiting potential and a small barrier for C–C coupling.
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J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA02388D, Paper

Junhui Tang, Ruisi Chen, Lidong Chen, Guillermo C. Bazan, Ziqi Liang
n-Type Co NWs/N2200 TENCs yield a high S, mainly from the semiconducting polymer, yet σ is limited by poor connectivity between inorganic and organic domains. By adding flexible n-doped SWCNTs to yield more conductive paths, σ and mechanical bendability are greatly enhanced.
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J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA01727B, Paper

Xiao Sui, Ziwen Yuan, Chang Liu, Li Wei, Meiying Xu, Fei Liu, Alejandro Montoya, Kunli Goh, Yuan Chen
Porous yet rigid 2D covalent–organic framework nanosheets can not only increase the interlayer spacing between graphene oxide nanosheets and provide direct transfer channels but also enhance the self-supporting capacity of graphene oxide laminates.
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J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/C9TA14066B, Paper

Yue Li, Jian Song, Mengting Jiang, Mbage Bawa, Xiaohong Wang, Yuyang Tian, Guangshan Zhu
Na₅[IMo₆O₂₄]·3H₂O and a porous aromatic framework (iPAF-1) were used to build an off-the-shelf building material (IMo₆@iPAF-1) to realize the highly efficient oxidation of organic sulfurs like oxygenase.
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J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA03321A, Review Article

Hao Wang, Chang-Jiang Yao, Hai-Jing Nie, Ke-Zhi Wang, Yu-Wu Zhong, Pengwan Chen, Shilin Mei, Qichun Zhang
Lithium-ion batteries (LIBs) have been demonstrated as one of the most promising energy storage devices for applications in electric vehicles, smart grids, large-scale energy storage systems, and portable electronics.
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J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/C9TA13812A, Paper

Ying Ling, Farhad M. D. Kazim, Shuangxiu Ma, Quan Zhang, Konggang Qu, Yangang Wang, Shenglin Xiao, Weiwei Cai, Zehui Yang
Incorporation of WO₂ to WS₂ nanosheets can efficiently suppress the competitive hydrogen evolution reaction (HER) due to the reduction of edge defects and create new planar defects at heterointerfaces for nitrogen reduction reaction (NRR).
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J. Mater. Chem. A, 2020, Accepted Manuscript
DOI: 10.1039/D0TA01633K, Paper

Shiao Zhang, Dingzhong Yuan, Qinghua Zhang, Yun Wang, Yan Liu, Jizhou Zhao, Bibo Chen
It is very necessary to develop the magnetic adsorbents for the efficient extraction of uranium from highly acidic media. In this work, a novel magnetic adsorbent Fe3O4/P (DMAA-DMP) functionalized with...
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J. Mater. Chem. A, 2020, Accepted Manuscript
DOI: 10.1039/D0TA00517G, Paper

Yosef Nikodimos, Meng-Che Tsai, Ljalem Hadush Abrha, Haile Hisho Weldeyohannis, Shuo-Feng Chiu, Hailemariam Kassa Bezabh, Kassie Nigus Shitaw, Fekadu Wubatu Fenta, She-Huang Wu, Wei-Nien Su, Yang Chun-Chen, Bing Joe Hwang
LiGe2(PO4)3 (LGP), a NASICON type solid electrolyte has many advantages like superior electrochemical and thermal stability to use in all solid state lithium batteries. However, its low ionic conductivity is...
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J. Mater. Chem. A, 2020, Accepted Manuscript
DOI: 10.1039/D0TA02507K, Paper

Yimin Jiang, Miao Yang, Meijiao Qu, Yi Wang, Zhouchunyu Yang, Qingliang Feng, Xia Deng, Wei Shen, Ming Li, Rongxing He
Promoting the industrialization and widespread application of Pt-based catalysts is essential to electrochemical water-splitting systems. However, the development of cost-effective Pt-based catalysts still remains a high challenge. Here we report...
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J. Mater. Chem. A, 2020, Accepted Manuscript
DOI: 10.1039/D0TA03347B, Paper

Yuqiao Chai, Hui Ma, Xinlei Ma, Xinyue Zhang, Yonglin He, Yapei Wang, Qianqian Jiang, Xusheng Wang, Junhui Ji, Mianqi Xue
Photothermal conversion in near-infrared (NIR) wavelengths, which converts light energy into heat energy, has caused great concern and been developing rapidly in recent years for its wide applications in health...
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J. Mater. Chem. A, 2020, Accepted Manuscript
DOI: 10.1039/D0TA03427D, Paper

Rong Xia, Sheng Zhang, Xinbin Ma, Feng Jiao
Rational design and synthesis of efficient catalysts for electrochemical CO2 reduction is a critical step towards practical CO2 electrolyzer systems. In this work, we report a strategy to tune the...
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J. Mater. Chem. A, 2020, Accepted Manuscript
DOI: 10.1039/D0TA02692A, Paper

Zhanshuang Jin, Ming Zhao, Tianning Lin, Bingqiu Liu, Qi Zhang, Lingyu Zhang, Lihua Chen, Lu Li, Zhong-Min Su, Chungang Wang
The physical confinement and chemical catalysis of lithium polysulfides (LiPSs) are effective ways to improve the performance of lithium-sulfur (Li-S) batteries. How to effectively combine physical confinement and chemical catalysis...
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J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA03112G, Paper

Yujie Zhao, Senlin Shao, Jiangbin Xia, Ya Huang, Yu Chi Zhang, Xue Li, Tao Cai
The photocatalyst-based ultrafiltration membrane fitted integrated synthesis–separation system holds the promises to bridge the gap between the precision of PET-RAFT polymerization and the efficiency of membrane separation process.
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J. Mater. Chem. A, 2020, Accepted Manuscript
DOI: 10.1039/C9TA14174J, Paper

Nait Saada Tamazouzt, Anderson da Silva, Palaniappan Subramanian, Liuqing Pang, Noual Adnane, Bahram Djafari-Rouhani, Vladyslav Mishyn, Dalila Meziane, Sorin Melinte, Georgiana Sandu, Franck Dumeignil, Sebastien Paul, Robert Wojcieszak, Rabah Boukherroub, Sabine Szunerits
Plasmon-driven chemical transformation has become a promising approach for enhancing sluggish electrocatalytic reactions. Herein, an alternative enhancement strategy employing plasmon-induced hot electrons is developed to be competitive with oxygen reduction...
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J. Mater. Chem. A, 2020, Accepted Manuscript
DOI: 10.1039/D0TA02633F, Review Article

Woong Choi, Da Hye Won, Yun Jeong Hwang
The gradual increase in the atmospheric CO2 concentration due to the combustion of fossil fuels is an urgent issue that poses a threat to human beings. Recently, the electrochemical CO2...
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J. Mater. Chem. A, 2020, Accepted Manuscript
DOI: 10.1039/D0TA03237A, Paper

Guang-Rui Xu, Hao Li, Abdulaziz Bati, Munkhjargal Bat-Erdene, Md Julker Nine, Dusan Losic, Yu Chen, Joseph G Shapter, Munkhbayar Batmunkh, Tianyi Ma
The rapid surface oxidation of phosphorene under ambient conditions is considered to be serious issue for many applications, but here is used as a strategy to achieve efficient heteroatom doping....
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J. Mater. Chem. A, 2020, Accepted Manuscript
DOI: 10.1039/D0TA02865G, Paper

Junhui Miao, Bin Meng, Zicheng Ding, Jun Liu, Lixiang Wang
Inorganic or organic solar cells always operate at temperature lower than 100 °C and are not suitable for operating at high temperature. In this work, using blends of small molecular...
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J. Mater. Chem. A, 2020, Accepted Manuscript
DOI: 10.1039/D0TA00876A, Paper

Chenglin Zhong, Zhen Han, Tongtong Wang, Qin-chao Wang, Zihan Shen, Qingwen Zhou, Jiaao Wang, Shuo Zhang, Xin Jin, Shengwen Li, Peng Wang, Daqiang Gao, Yong-Ning Zhou, Huigang Zhang
High-efficiency non-precious electrocatalysts are urgently demanded in hydrogen evolution reaction (HER) and oxygen evolution reaction (OER). Transition metal oxides catalysts have shown high activity for the OER in alkaline medium,...
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J. Mater. Chem. A, 2020, Accepted Manuscript
DOI: 10.1039/D0TA01419B, Paper

Xiwei Xu, Songqi Ma, Sheng Wang, Jiahui Wu, Qiong Li, na lu, yanlin liu, Jintao Yang, Jie Feng, Jin Zhu
Covalent adaptable networks (CANs) provide a promising approach to the recycle issue of thermosets due to their dynamic cross-linked networks. However, CANs are susceptible to creep at relatively low temperatures,...
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J. Mater. Chem. A, 2020, Accepted Manuscript
DOI: 10.1039/D0TA01217C, Paper

Mingzhu Sun, Zhao Wang, Xue Li, Haibo Li, Hongsheng Jia, Xiangxin Xue, Ming Jin, Jiaqi Li, Yu Xie, Ming Feng
Lithium-sulfur (Li-S) batteries are promising candidates for next-generation energy storage devices due to its high theoretical energy density, whose practical applications are mainly hampered by the shuttle effect of intermediate...
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