Chem. Sci., 2024, 15,18135-18145
DOI: 10.1039/D4SC04896B, Edge Article

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Jing Jin, Zhaolong He, Di Liu, Yongqiang Mei, Jiahui Wang, Huihui Wan, Jiuyan Li
Spiro-acridine modified N/B/O type MR-TADF emitters realized deep blue fluorescence with an EQE_max of 20.5% and CIE (0.147, 0.048), which is state-of-the-art efficiency for N/B/O type deep-blue MR emitters with CIEy approaching the BT.2020 standard.
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Chem. Sci., 2024, 15,18146-18160
DOI: 10.1039/D4SC05289G, Edge Article

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Ewan McQueen, Noritaka Sakakibara, Kei Kamogawa, Martijn A. Zwijnenburg, Yusuke Tamaki, Osamu Ishitani, Reiner Sebastian Sprick
This highly efficient hybrid photocatalytic system can quantitatively convert CO₂ to formate and produce 0.4 M of formate solution without additional concentration enrichment.
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Chem. Sci., 2024, 15,18060-18066
DOI: 10.1039/D4SC05442C, Edge Article

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Zheng-Xiao Tang, Bin Wang, Zhi-Rui Li, Zhuo Huang, Hai-Xia Zhao, La-Sheng Long, Lan-Sun Zheng
A molecule-based ferroelectric [(CH₃)₃NCH₂CH₂Br][GaBr₄] (1), with a d₃₃ value of 331 pC N⁻¹, was synthesized. The power density of the 1@S-PDMS piezoelectric sensor, featuring optimized microstructures, is up to 490 μW cm⁻².
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Chem. Sci., 2024, 15,18048-18051
DOI: 10.1039/D4SC04980B, Edge Article

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Minling Zhong, Jie Zhang, Zuowei Xie
Reactions of o-carborane-fused diborane(4) with 3H-diazirines lead to the complete cleavage of the NN bond, with one nitrogen atom being incorporated into the B–B bond.
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Chem. Sci., 2024, 15,18085-18092
DOI: 10.1039/D4SC03763D, Edge Article

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Ruyu Xie, Kaitao Li, Rui Tian, Chao Lu
We have proposed an oxygen intermediate-boosted electrochemiluminescence probe for rapid spotting of the d-band centers of single-atom catalysts: the d-band centers closer to the Fermi level contributed to higher luminol ECL intensities.
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Chem. Sci., 2024, 15,17739-17759
DOI: 10.1039/D4SC05489J, Perspective

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Upasana Deori, Gyana Prakash Nanda, Caroline Murawski, Pachaiyappan Rajamalli
The evolution of next-generation HF-OLED technology and current challenges.
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Chem. Sci., 2024, 15,18031-18047
DOI: 10.1039/D4SC02408G, Edge Article

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David Kreutter, Jean-Louis Reymond
Integrating enzymatic reactions into computer-aided synthesis planning (CASP) should help devise more selective, economical, and greener synthetic routes.
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Chem. Sci., 2024, 15,17799-17822
DOI: 10.1039/D4SC05295A, Review Article

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Miaoyu Li, Jie Pu, Qinghe Cao, Wenbo Zhao, Yong Gao, Ting Meng, Jipeng Chen, Cao Guan
The application of hydrogel-based flexible strain sensors in harsh environments, including extreme temperatures, humidity, high mechanical strain, and strong corrosion, is investigated.
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Chem. Sci., 2024, 15,17781-17798
DOI: 10.1039/D4SC05205F, Review Article

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Pengfei Wu, Mengting Guo, Ran-Wei Zhang, Qing Huang, Guibin Wang, Ya-Qian Lan
The study discussed how MOFs treat microplastics, how to make plastic-based MOFs, and how MOF@plastic composites can be used. It aids in understanding how to convert plastic/microplastic concerns into opportunities for high-valued products.
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Chem. Sci., 2024, 15,17843-17851
DOI: 10.1039/D4SC05038J, Edge Article

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Shubham Bansal, Binghe Wang
Reactive oxygen species (ROS) play critical roles in normal physiological processes including cellular signaling and immune responses.
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Chem. Sci., 2024, 15,18093-18098
DOI: 10.1039/D4SC05337K, Edge Article

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João V. Schober, Croix J. Laconsay, Judy I. Wu
Diene- and ene-like reactivity in transition metal coordinated arenes can be expected when there is a notable degree of aromaticity loss at the complexed arene.
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Chem. Sci., 2024, 15,17823-17830
DOI: 10.1039/D4SC03546A, Edge Article

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Jonghwan Lee, Sungsik Eom, Hyungjun Kim
This work explores intramolecular singlet fission chromophores having diverse thiophene-based linkers and highlights the relation between quantum interference and nonadiabatic coupling in the multiexciton formation step of singlet fission.
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Chem. Sci., 2024, 15,18161-18169
DOI: 10.1039/D4SC04318A, Edge Article

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Xiaoqin Cui, Xuehuan Zhang, Ting Li, Sheng Zhu, Gaoyi Han, Huan Li
A sterically demanding ortho-CF₃ substituent defines not only the arrangement of ligands on a Ag₉₈(2-CF₃PhCC)₄₈Cl₄ nanocluster (Ag₉₈) but also the inter-cluster interactions. Ag₉₈ shows excellent methanol tolerance in the oxygen reduction reaction.
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Chem. Sci., 2024, 15,17881-17891
DOI: 10.1039/D4SC04630G, Edge Article

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Shi Xuan Leong, Sergio Pablo-García, Zijian Zhang, Alán Aspuru-Guzik
Leveraging multimodal large language models (MLLMs) to process multimodal data inputs and complex inter-modality data dependencies for automated (electro)chemical data mining from scientific literature.
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Chem. Sci., 2024, 15,17950-17961
DOI: 10.1039/D4SC05006A, Edge Article

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Kazuya Tanimura, Kento Tanaka, Masayuki Gon, Kazuo Tanaka
The study focuses on dinuclear hypervalent tin(IV) compounds with near-infrared (NIR) emission and unique quadrupolar orientations, showing potential for constructing electronic structures with narrow energy gaps.
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Chem. Sci., 2024, 15,17971-17978
DOI: 10.1039/D4SC04685D, Edge Article

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Shuo Li, Guoli Zhang, Qianrui Li, Tianshun He, Xiaoqi Sun
A facile self-saturation strategy, realized by the introduction of a hydrophobic methyl group on naphthoquinone, is demonstrated to suppress the dissolution of small molecule cathode materials and achieve stable cycling in aqueous zinc cells.
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Chem. Sci., 2024, 15,18170-18178
DOI: 10.1039/D4SC04404E, Edge Article

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Jing Xu, Yujin Li, Futing Wang, Xinqi Luo, Wei Zhang, Yifan Lyu, Hongfen Yang, Ren Cai, Weihong Tan
A bidirectional self-powered biosensor is constructed for the quasi-simultaneous detection of Pb²⁺ and Hg²⁺ based on MoS2@CuS heterostructures as an accelerator and hybridization chain reaction as a signal amplification strategy.
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Chem. Sci., 2024, 15,18022-18030
DOI: 10.1039/D4SC04429K, Edge Article

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Julius A. Knöller, Franziska Müller, Tomas Matulaitis, John M. dos Santos, Abhishek Kumar Gupta, Eli Zysman-Colman, Sabine Laschat
We developed a MR-TADF based, columnar liquid crystalline host system and doped it with a MR-TADF guest. Efficient FRET allowed us to construct the first columnar liquid crystal with narrowband MR-TADF from the strongly aggregated mesophase.
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Chem. Sci., 2024, 15,18111-18126
DOI: 10.1039/D4SC04852K, Edge Article

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Feng An, Jan Brossette, Harish Jangra, Yin Wei, Min Shi, Hendrik Zipse, Armin R. Ofial
Combined experimental and quantum-chemical studies were used to characterise the philicity/fugality features of tertiary phosphines and Michael acceptors in phospha-Michael reactions, which are key steps in phosphine-catalysed organic reactions.
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Chem. Sci., 2024, 15,18127-18134
DOI: 10.1039/D4SC04874A, Edge Article

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Renjith Nadarajan, Sraboni Dey, Arijit Kayal, Joy Mitra, Manikoth M. Shaijumon
The synergistic creation of vacancy defects, along with strain-induced active sites is shown to enhance hydrogen evolution reaction (HER) performance of CVD-grown monolayer MoS₂.
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Chem. Sci., 2024, Advance Article
DOI: 10.1039/D4SC04620J, Edge Article

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Odin Zhang, Yufei Huang, Shichen Cheng, Mengyao Yu, Xujun Zhang, Haitao Lin, Yundian Zeng, Mingyang Wang, Zhenxing Wu, Huifeng Zhao, Zaixi Zhang, Chenqing Hua, Yu Kang, Sunliang Cui, Peichen Pan, Chang-Yu Hsieh, Tingjun Hou
FragGen introduces a novel fragment-based AI-based molecular design method. It proposes the geometry handling protocol to improve the generation quality and has been applied to design highly bioactive type II kinase inhibitors.
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Chem. Sci., 2024, 15,17720-17738
DOI: 10.1039/D4SC04288C, Perspective

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Errui Li, Kevin M. Siniard, Zhenzhen Yang, Sheng Dai
In this perspective, recent discoveries in the integration of gas storage and catalysis by leveraging PL platforms have been summarized, highlighting the unique features different from those of traditional homogeneous or heterogeneous procedures.
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Chem. Sci., 2024, Advance Article
DOI: 10.1039/D4SC06060A, Edge Article

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Yipeng You, Xue-Jie Zhang, Wen Xiao, Thittaya Kunthic, Zheng Xiang, Chen Xu
A unified synthetic strategy for drimane meroterpenoids was developed by combining heterologous biosynthesis, enzymatic oxidation, and transition metal catalysis. Six drimane meroterpenoids were synthesized in a concise and enantiospecific manner.
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Chem. Sci., 2024, Advance Article
DOI: 10.1039/D4SC04879B, Edge Article

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Jingjing Yu, Marius Gaedke, Satyajit Das, Daniel L. Stares, Christoph A. Schalley, Fredrik Schaufelberger
Dynamic covalent boronic ester bonds can pre-organise diol-containing threads and V-shaped boronic acid ligands towards mechanical interlocking. After interlocking, the pre-rotaxane could be modified to create many unique [2]rotaxanes architectures.
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Chem. Sci., 2024, Advance Article
DOI: 10.1039/D4SC05998K, Edge Article

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Xue Bai, Yin Wang, Jingyi Han, Siyu Chen, Xiaodi Niu, Jingqi Guan
Utilizing double coordination shell modulation, we construct a novel nitrogen-free single-atom manganese coordination configuration catalyst on graphene oxide (Mn–S₁O₄G), which exhibits excellent ORR and zinc–air battery performances.
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Chem. Sci., 2024, Advance Article
DOI: 10.1039/D4SC06780K, Edge Article

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Jihoon Jang, Ho Seong Hwang, Haeryeong Jeong, Eun Jin Cho
An electrochemical trifluoromethylation method for terminal alkynes has been developed, facilitating the synthesis of CF₃-alkynes with DMSO as a masking auxiliary.
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Chem. Sci., 2024, Accepted Manuscript
DOI: 10.1039/D4SC05437G, Perspective

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Li Li, Wenhan Xu, Guanchun Rui, Shixian Zhang, Qiming Zhang, Qing Wang
Electrostatic capacitors (ECs) are critical components in advanced electronics and electric power systems due to their rapid charge-discharge rate and high power density. While polymers are ideal for ECs due...
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Chem. Sci., 2024, Accepted Manuscript
DOI: 10.1039/D4SC05424E, Edge Article

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Laurent Knerr, Thomas Cogswell, Marie. Ahlqvist, Richard James Lewis, Anneli Nordqvist, Christian Sköld
Conformational control of drug candidates to engineer improved potency and ADME properties is an ongoing area of research. Macrocyclic rings tend to offer a greater degree of rigidity than non-cyclised...
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Chem. Sci., 2024, Advance Article
DOI: 10.1039/D4SC90219J, Correction

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Tayyaba Najam, Syed Shoaib Ahmad Shah, Hanqing Yin, Xin Xiao, Shamraiz Talib, Qianqian Ji, Yonggui Deng, Muhammad Sufyan Javed, Jie Hu, Ruo Zhao, Aijun Du, Xingke Cai, Qiang Xu
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Chem. Sci., 2024, Advance Article
DOI: 10.1039/D4SC04767B, Edge Article

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Lucie Pedussaut, Nolwenn Mahieu, Camille Chartier, Thayalan Rajeshkumar, Maxime Tricoire, Iskander Douair, Nicolas Casaretto, Laurent Maron, Grégory Danoun, Grégory Nocton
Reversible light isomerization in organometallic complexes of lanthanides: the low-energy wavelengths favor the cis isomer, and the high-energy wavelengths favor the trans isomer.
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Chem. Sci., 2024, Advance Article
DOI: 10.1039/D4SC05736H, Review Article

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Ritu Gupta, Anujit Balo, Rabia Garg, Amit Kumar Mondal, Koyel Banerjee Ghosh, Prakash Chandra Mondal
This review highlights recent experimental findings related to the chirality-induced spin selectivity effect. This effect is demonstrated to explain asymmetric electron's spin transport in chiral molecules for various technological applications.
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Chem. Sci., 2024, Accepted Manuscript
DOI: 10.1039/D4SC06820C, Review Article

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Seungwon Sun, Jisu Choe, Jaeheung Cho
In biological systems, nitric oxide (NO) is a crucial signaling molecule that regulates a wide range of physiological and pathological processes. Given the significance of NO, there has been considerable...
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Chem. Sci., 2024, Accepted Manuscript
DOI: 10.1039/D4SC05375C, Edge Article

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Guanlun Zhang, Xu Wu, Shiyu Mao, Mengqi Li, Honglong Hu, Bing-Feng Shi, Weihong Zhu
Sterically-hindered diarylethenes with intrinsic chirality have shown great potential in chiral signal regulation, light-controlled liquid crystals (LCs), etc. Their unique enantiospecific phototransformation between axial chirality of ring-open isomer and central...
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Chem. Sci., 2024, Accepted Manuscript
DOI: 10.1039/D4SC04738A, Edge Article

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Hao-Ting Qu, Iida Partanen, Kai-Hsin Chang, Yan-Ding Lin, Igor O Koshevoy, Andrey Belyaev, Pi-Tai Chou
By strategic design and synthesis of a new series of phosphonium salts (compounds 1–7[OTf]), where [OTf]- stands for the trifluoromethanesulfonate anion, we performed comprehensive spectroscopic and dynamic studies on the...
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Chem. Sci., 2024, Accepted Manuscript
DOI: 10.1039/D4SC04589K, Edge Article

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Athulya Nadol, Florian Venel, Raynald Giovine, Maeva Leloire, Christophe Volkringer, Thierry Loiseau, Christel Gervais, Caroline Mellot-Draznieks, Bertrand Doumert, Julien Trébosc, Olivier Lafon, Frédérique Pourpoint
The stability of metal-organic frameworks (MOFs) in the presence of water is crucial for a wide range of applications, including the production of freshwater, desiccation, humidity control, heat pumps/chillers and...
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Chem. Sci., 2024, Accepted Manuscript
DOI: 10.1039/D4SC03942D, Edge Article

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Darren Dolan, Rebekah Brucato, Christopher William Reid, Adam F. Lee, Karen Wilson, Adelina M Voutchkova-Kostal
Cleavage of lignin ether bonds via transfer hydrogenolysis is a promising route to valorize lignin, but processes that use mild reaction conditions and exploit renewable hydrogen donor solvents (rather than...
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Chem. Sci., 2024, Advance Article
DOI: 10.1039/D4SC05788K, Edge Article

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Utsav Dey Sarkar, Mahima Rana, Harinath Chakrapani
A new series of phenacylselenoesters that generate hydrogen selenide in the presence of esterase and a biological thiol under ambient conditions is reported.
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Chem. Sci., 2024, Advance Article
DOI: 10.1039/D4SC05121A, Edge Article

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Saideep Singh, Joaquín Martínez-Ortigosa, Nuria Ortuño, Vivek Polshettiwar, Javier García-Martínez
By optimizing zeolite pore confinement, polymer diffusion and up-cycling efficiency in hierarchical catalysts are significantly enhanced, reducing plastic degradation temperatures and providing a suitable route to sustainable plastic-to-fuel pathways.
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