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Hexatic phase in a model of active biological tissues

Soft Matter, 2020, 16,3914-3920
DOI: 10.1039/D0SM00109K, Paper
Anshuman Pasupalak, Li Yan-Wei, Ran Ni, Massimo Pica Ciamarra
Epithelial cell tissues undergo a solid–liquid transition, e.g. as the motility of the cells increases. We find an intermediate hexatic phase in between the solid and the liquid ones, and the transition to follow the KTHNY scenario.
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A heavy intruder in a locally-shaken granular solid

Soft Matter, 2020, 16,3921-3928
DOI: 10.1039/C9SM02498K, Paper
Diego Berzi, Stefano Buzzaccaro
We experimentally investigate the gravitational-driven motion of a heavy object inside a vertical 2D assembly of identical, plastic cylinders arranged in a regular, triangular lattice.
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A practical guide to active colloids: choosing synthetic model systems for soft matter physics research

Soft Matter, 2020, 16,3846-3868
DOI: 10.1039/D0SM00222D, Review Article
Wei Wang, Xianglong Lv, Jeffrey L. Moran, Shifang Duan, Chao Zhou
This review article provides practical, experimentally relevant details on six common types of active colloids useful for soft matter research.
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Effects of sodium chloride on rheological behaviour of the gemini-like surfactants

Soft Matter, 2020, 16,4024-4031
DOI: 10.1039/D0SM00243G, Paper
Xinxin Li, Pengxiang Wang, Xiaoyu Hou, Fang Wang, Han Zhao, Bobo Zhou, Hongwen Zhang, Hongbin Yang, Wanli Kang
Effects of NaCl on the rheological behaviour of the gemini-like surfactants and the mechanism of the effects were investigated.
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Observation of transition cascades in sheared liquid crystalline polymers

Soft Matter, 2020, 16,3891-3901
DOI: 10.1039/D0SM00275E, Paper
Ryan J. Fox, M. Gregory Forest, Stephen J. Picken, Theo J. Dingemans
We observe anomalous shear thickening behavior of a lyotropic liquid crystalline polymer due to the dynamics of the nematic director.
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Surface buckling delamination patterns of film on soft spherical substrates

Soft Matter, 2020, 16,3952-3961
DOI: 10.1039/D0SM00122H, Paper
Kanako Emori, Yusaku Saito, Akio Yonezu, Liangliang Zhu, Xiangbiao Liao, Xi Chen
The morphological transition of film buckling-delamination in an elastomeric bilayer spherical shell system was studied experimentally and numerically. It was changed by the film thickness, Young's modulus, and interfacial adhesion condition, etc.
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Melting scenarios of two-dimensional Hertzian spheres with a single triangular lattice

Soft Matter, 2020, 16,3962-3972
DOI: 10.1039/C9SM02262G, Paper
E. N. Tsiok, E. A. Gaiduk, Yu. D. Fomin, V. N. Ryzhov
We present a molecular dynamics simulation study of the phase diagram and melting scenarios of two-dimensional Hertzian spheres with exponent 7/2.
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Normal and shear forces between boundary sphingomyelin layers under aqueous conditions

Soft Matter, 2020, 16,3973-3980
DOI: 10.1039/D0SM00215A, Paper
Yifeng Cao, Nir Kampf, Weifeng Lin, Jacob Klein
Sphingomyelin boundary layers can maintain extremely low friction under high pressures both in water and at high salt concentration.
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Engineering interfacial entropic effects to generate giant viscosity changes in nanoparticle embedded polymer thin films

Soft Matter, 2020, 16,4065-4073
DOI: 10.1039/D0SM00019A, Paper
Aparna Swain, Nafisa Begam, Sivasurender Chandran, M. S. Bobji, J. K. Basu
We demonstrate a new method to study the viscosity of PNC thin films, consisting of polymer grafted nanoparticles (PGNPs) embedded in un-entangled homopolymer melt films, using atomic force microscopy based force–distance spectroscopy.
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Structural properties of contractile gels based on light-driven molecular motors: a small-angle neutron and X-ray study

Soft Matter, 2020, 16,4008-4023
DOI: 10.1039/D0SM00031K, Paper
Giacomo Mariani, Jean-Rémy Colard-Itté, Emilie Moulin, Nicolas Giuseppone, Eric Buhler
The collective rotation of light-driven molecular motors actuates the structural changes and macroscopic contraction of the chemical gels.
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Detachment work of prolate spheroidal particles from fluid droplets: role of viscous dissipation

Soft Matter, 2020, 16,4049-4056
DOI: 10.1039/C9SM02385B, Paper
Sergey V. Lishchuk, Rammile Ettelaie
The minimum possible work done upon removal of an elongated solid particle from the surface of a liquid droplet can be less than that for a sphere.
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Using microprojectiles to study the ballistic limit of polymer thin films

Soft Matter, 2020, 16,3886-3890
DOI: 10.1039/D0SM00295J, Communication
Shawn H. Chen, Amanda J. Souna, Christopher L. Soles, Stephan J. Stranick, Edwin P. Chan
In this work, a microballistic impact test called laser induced projectile impact test (LIPIT) was used to study the perforation behavior of polycarbonate thin films to demonstrate the importance of film thickness on the film's ballistic limit.
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Correction: Preparation of electrospray ALG/PDA–PVP nanocomposites and their application in cancer therapy

Soft Matter, 2020, 16,4074-4074
DOI: 10.1039/D0SM90064H, Correction
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Yangjie Xu, Jiulong Zhao, Zhilun Zhang, Jing Zhang, Mingxian Huang, Shige Wang, Pei Xie
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Modeling atomic force microscopy and shell mechanical properties estimation of coated microbubbles

Soft Matter, 2020, Accepted Manuscript
DOI: 10.1039/D0SM00300J, Paper
Alkmini Lytra, Vassilis Sboros, Antonios Giannakopoulos, Nikos Pelekasis
We present an extensive comparison with experimental data of our theoretical/numerical model for the static response of coated microbubbles (MBs) subject to compression from an atomic force microscope (afm). The...
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Assessing the Extent of Structural and Dynamic Modulation of Membrane Lipids due to Pore Forming Toxins: Insights from Molecular Dynamics Simulations

Soft Matter, 2020, Accepted Manuscript
DOI: 10.1039/D0SM00086H, Paper
Vadhana Varadarajan, Rajat Desikan, Ganapathy Ayappa
Infections in many virulent bacterial strains are triggered by the release of pore forming toxins (PFTs), which form oligomeric transmembrane pore complexes on the target plasma membrane. The spatial extent...
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Marangoni puffs: dramatically enhanced dissolution of droplets with an entrapped bubble

Soft Matter, 2020, Advance Article
DOI: 10.1039/D0SM00093K, Paper
José M. Encarnación Escobar, Jaap Nieland, Arie van Houselt, Xuehua Zhang, Detlef Lohse
We present a curious effect observed during the dissolution process of water-immersed long-chain alcohol drops with an entrapped bubble. When the drop-water interface and the air bubble contact each other, a rapid cyclic motion that accelerates the drop's dissolution is found. We name this eye-catching phenomenon puffing.
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Self similarity of liquid droplet coalescence in a quasi-2D free-standing liquid-crystal film

Soft Matter, 2020, Advance Article
DOI: 10.1039/D0SM00457J, Paper
Christoph Klopp, Torsten Trittel, Ralf Stannarius
Flat droplets coalescing on smectic free-standing films show self-similar dynamics.
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Structural universality in disordered packings with size and shape polydispersity

Soft Matter, 2020, Advance Article
DOI: 10.1039/D0SM00110D, Paper
Ye Yuan, Wei Deng, Shuixiang Li
Normalized free volume collapses on normalized particle size in polydisperse-sized packings for a given non-spherical particle.
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Bioactive scaffolds based on collagen filaments with tunable physico-chemical and biological features

Soft Matter, 2020, Advance Article
DOI: 10.1039/D0SM00233J, Paper
Ting Lu, Hong Hu, Yuanqi Li, Qingsong Jiang, Jinlei Su, Hai Lin, Yun Xiao, Xiangdong Zhu, Xingdong Zhang
Native tissues such as nerve bundles, blood vessels and tendons have extracellular matrices with a characteristic linear orientation, which cannot be fully achieved with the current technology for the development of regenerative biomaterials.
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Formation of Fibrillar Crystals Strongly Accelerates the Form II to I Transformation of Polybutene-1

Soft Matter, 2020, Accepted Manuscript
DOI: 10.1039/D0SM00572J, Paper
Jiaqi Zhang, Chang Liu, Xintong Zhao, Zhijie Zhang, Quan Chen
This study examines shear-induced formation of fibrillar form II crystals and subsequent form II to I transformation of an isotactic polybutene-1 sample through a combination of rheology, polarized optical microscope...
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Review and reproducibility of forming adsorbed layers from solvent washing of melt annealed films

Soft Matter, 2020, Advance Article
DOI: 10.1039/D0SM00565G, Paper
Michael F. Thees, Jennifer A. McGuire, Connie B. Roth
Efforts to reproduce the “Guiselin’s experiment” procedure finds hads(t) curves to be far less reliable than implied in the literature, being strongly dependent on solvent washing conditions, consistent with how adsorption in solution is understood.
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Mix and match—a versatile equilibrium approach for hybrid colloidal synthesis

Soft Matter, 2020, Advance Article
DOI: 10.1039/D0SM00202J, Communication
Matan Yah Ben Zion, Yaelin Caba, Ruojie Sha, Nadrian C. Seeman, Paul M. Chaikin
We outline a simple yet general equilibrium technique for a scalable, high-purity, hybrid-colloidal synthesis with controlled valency. The method is applicable for liquid and solid particles and to a range of particle interactions.
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Liposomal adhesion via electrostatic interactions and osmotic deflation increase membrane tension and lipid diffusion coefficient

Soft Matter, 2020, Advance Article
DOI: 10.1039/D0SM00416B, Paper
Atsushi Oda, Chiho Watanabe, Natsumi Aoki, Miho Yanagisawa
Liposome–liposome adhesion by electrostatic interactions and osmotic contraction increase membrane tension and the lipid diffusion coefficient compared to isolated liposomes.
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Developing Super Tough Gelatin-based Hydrogels by Incorporating Linear Poly(methacrylic Acid) to Facilitate Sacrificial Hydrogen Bonding

Soft Matter, 2020, Accepted Manuscript
DOI: 10.1039/D0SM00422G, Communication
Hui Jie Zhang, Li Ni Wang, Xuechuan Wang, Qingxin Han, Xiangyou You
Mechanically robust protein-based hydrogels are strongly desired but their construction remains a significant challenge. In this work, gelatin, together with methacrylic acid, is used to construct a novel hydrogen-bonded hydrogel...
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Classical and Non-Classical Melatonin Receptor Agonist-Directed Micellization of Bipyridinium-Based Supramolecular Amphiphiles in Water

Soft Matter, 2020, Accepted Manuscript
DOI: 10.1039/D0SM00424C, Paper
Zhimin Sun, Lihui Xi, Kai Zheng, Zhao Zhang, Kim Baldridge, Mark Anthony Olson
The addition of molecular recognition units into structures of amphiphiles is a means by which soft matter capable of undergoing template-directed micellization can be obtained. These supramolecular amphiphiles can bind...
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Coalescence of isotropic droplets in overheated free standing smectic films

Soft Matter, 2020, Advance Article
DOI: 10.1039/C9SM02292A, Paper
Elena S. Pikina, Boris I. Ostrovskii, Sergey A. Pikin
A theoretical study of the interaction and coalescence of isotropic droplets in overheated free-standing smectic films (FSSF) is presented.
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Polymorphism of asymmetric catalysts based on amphiphilic lipopeptides in solution

Soft Matter, 2020, Advance Article
DOI: 10.1039/D0SM00245C, Paper
Juliane N. B. D. Pelin, Charlotte J. C. Edwards-Gayle, Andrea M. Aguilar, Amanpreet Kaur, Ian W. Hamley, Wendel A. Alves
The self-assembly of model [P]RWG lipopeptides (P: L-proline, R: L-arginine, W: L-tryptophan, G: L-glycine), containing one or two aliphatic octadecyl (C18) chains in water and cyclohexanone/water solutions was examined. The enantiomeric selectivity was found to be related to the assembly of catalyst molecules.
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On the pressure dependence of the thermodynamical scaling exponent γ

Soft Matter, 2020, Advance Article
DOI: 10.1039/D0SM00254B, Paper
R. Casalini, T. C. Ransom
In materials with a constant scaling parameter γS, the Isomorph γI is found to vary with pressure, demonstrating γSγI.
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Effect of polar amino acid incorporation on Fmoc-diphenylalanine-based tetrapeptides

Soft Matter, 2020, Accepted Manuscript
DOI: 10.1039/D0SM00320D, Paper
Alexandra Daryl Ariawan, Biyun Sun, Jonathan Pawel Wojciechowski, Ian Lin, Eric Y Du, Sophia C Goodchild, Charles Gordon Cranfield, Lars M Ittner, Pall Thordarson, Adam David Martin
Peptide hydrogels show great promise as extracellular matrix mimics due to their tuneable, fibrous nature. Through incorporation of polar cationic, polar anionic or polar neutral amino acids into the Fmoc-diphenylalanine...
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Effects of Eigen and Actual Frequencies of Soft Elastic Surfaces on droplet Rebound from Stationary Flexible Feather Vanes

Soft Matter, 2020, Accepted Manuscript
DOI: 10.1039/D0SM00315H, Paper
Chengchun Zhang, Zhengyang Wu, Chun Shen, Yihua Zheng, LIANG YANG, Yan Liu, Luquan Ren
The aim of this paper is to investigate the effect of eigenfrequency and the actual frequency of the elastic surface for the droplet rebound. The elastic surface used in this...
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Impact of Chiral Supramolecular Nanostructure on the Mechanical and Electrical Performances of Triphenylene-based discotic physical gels

Soft Matter, 2020, Accepted Manuscript
DOI: 10.1039/D0SM00152J, Paper
Hongli Zhang, Junjie Cheng, Qiang Zhou, Qijin Zhang, Gang Zou
Discotic π-conjugated supramolecular assemblies, especially with chiral supramolecular nanostructures, have been attracting growing research interests due to their significant optoelectronic properties and the possibilities of their applications in the new...
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Simultaneous determination of interfacial molarities of an alcohol, bromide ion, and water during an alcohol induced microstructural transition: The difference between medium and long chain alcohols.

Soft Matter, 2020, Accepted Manuscript
DOI: 10.1039/D0SM00665C, Paper
Kaixin Yao, Lijie Sun, Xiaoxuan Ding, Yuzhao Wang, Tianze Liu, Changyao Liu, Jiajing Tan, Li Zhao, Baocai Xu, Laurence S. Romsted
The transitions between surfactant aggregate structures are triggered by changes in chemical or physical stimulations, including addition of additives. Effects of added alcohols on aggregate morphologies correlate strongly with alcohol...
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Evaluation of the subtle trade-off between physical stability and thermo-responsiveness in crosslinked methylcellulose hydrogels

Soft Matter, 2020, Accepted Manuscript
DOI: 10.1039/D0SM00269K, Paper
Lorenzo Bonetti, Luigi De Nardo, Fabio Variola, Silvia Fare
Methylcellulose (MC) hydrogels, undergoing sol-gel reversible transition upon temperature changes, lend themselves to smart system applications. However, their reduced stability in aqueous environment and unsatisfactory mechanical properties limit the breadth...
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Self-assembly of isomeric naphthalene appended glucono derivatives: nanofibers and nanotwists with circularly polarized luminescence emission

Soft Matter, 2020, 16,4115-4120
DOI: 10.1039/C9SM02542A, Paper
Zongwen Liu, Yuqian Jiang, Jian Jiang, Donghua Zhai, Decai Wang, Minghua Liu
Two isomers of naphthalene derivatives are self-assembled into nanofibers and nanotwists with CPL emission, respectively.
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Photo-tunable hydrogel mechanical heterogeneity informed by predictive transport kinetics model

Soft Matter, 2020, 16,4131-4141
DOI: 10.1039/D0SM00052C, Paper
Callie I. Higgins, Jason P. Killgore, Frank W. DelRio, Stephanie J. Bryant, Robert R. McLeod
Photo-tunable hydrogel mechanical heterogeneity using a single resin is presented here, informed by a predictive transport kinetics and swelling model.
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Pinning dislocations in colloidal crystals with active particles that seek stacking faults

Soft Matter, 2020, 16,4182-4191
DOI: 10.1039/C9SM02514F, Paper
Bryan VanSaders, Sharon C. Glotzer
By designing the shape of an active particle, its transport through a dense crystal can be tailored, as well as its interaction with dislocation defects present in the host crystal.
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Experimental observation of boundary-driven oscillations in a reaction–diffusion–advection system

Soft Matter, 2020, 16,4243-4255
DOI: 10.1039/C9SM02291K, Paper
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Torsten Eckstein, Estefania Vidal-Henriquez, Azam Gholami
Boundary-driven oscillations are observed experimentally in a reaction-diffusion-advection system, namely in the signaling population of Dictyostelium discoideum cells.
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Geometry underlies the mechanical stiffening and softening of an indented floating film

Soft Matter, 2020, 16,4121-4130
DOI: 10.1039/D0SM00250J, Paper
Open Access
Monica M. Ripp, Vincent Démery, Teng Zhang, Joseph D. Paulsen
Using experiments, simulations, and theory, we map out the remarkably rich mechanical response of a floating polymer film to indentation.
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Lattice self-consistent field calculations of confined symmetric block copolymers of various chain architectures

Soft Matter, 2020, 16,4311-4323
DOI: 10.1039/D0SM00293C, Paper
Jingxue Zhang, Jiaping Wu, Run Jiang, Zheng Wang, Yuhua Yin, Baohui Li, Qiang Wang
The effects of chain architecture on the structural details and orientation of confined lamellae formed by symmetric AB-type block copolymer melts are studied.
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High antisite defect concentrations in hard-sphere colloidal Laves phases

Soft Matter, 2020, 16,4155-4161
DOI: 10.1039/D0SM00335B, Paper
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Berend van der Meer, Frank Smallenburg, Marjolein Dijkstra, Laura Filion
We show that the equilibrium Laves phase in binary hard-sphere mixtures contains an extraordinarily high concentration of antisite defects:  we find stable regions where up to 2% of the large-particle lattice sites are occupied by a small particle.
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Phenylalanine dimer assembly structure as the basic building block of an amyloid like photoluminescent nanofibril network

Soft Matter, 2020, 16,4105-4109
DOI: 10.1039/D0SM00387E, Communication
Prabhjot Singh, Nishima Wangoo, Rohit K. Sharma
Self-assembled phenylalanine dimer as the basic supramolecular structure of β-amyloid like photoluminescent nanofibrils.
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Ordering of binary colloidal crystals by random potentials

Soft Matter, 2020, 16,4267-4273
DOI: 10.1039/D0SM00208A, Paper
André S. Nunes, Sabareesh K. P. Velu, Iryna Kasianiuk, Denis Kasyanyuk, Agnese Callegari, Giorgio Volpe, Margarida M. Telo da Gama, Giovanni Volpe, Nuno A. M. Araújo
A random potential can control the number of defects in a binary colloidal crystal.
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Effect of network homogeneity on mechanical, thermal and electrochemical properties of solid polymer electrolytes prepared by homogeneous 4-arm poly(ethylene glycols)

Soft Matter, 2020, 16,4290-4298
DOI: 10.1039/D0SM00289E, Paper
Monami Tosa, Kei Hashimoto, Hisashi Kokubo, Kazuhide Ueno, Masayoshi Watanabe
The effect of network inhomogeneity in solid polymer electrolytes on its electrolyte properties was investigated by employing a model polymer network composed of a homogeneous 4-arm poly(ethylene glycol) (tetra-PEG) network and Li salt.
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Filamentous and step-like behavior of gelling coarse fibrin networks revealed by high-frequency microrheology

Soft Matter, 2020, 16,4234-4242
DOI: 10.1039/C9SM02228G, Paper
Pablo Domínguez-García, Giovanni Dietler, László Forró, Sylvia Jeney
By a micro-experimental methodology, we study the ongoing molecular process inside coarse fibrin networks by means of microrheology.
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Rapid analysis of cell-generated forces within a multicellular aggregate using microsphere-based traction force microscopy

Soft Matter, 2020, 16,4192-4199
DOI: 10.1039/C9SM02377A, Paper
Buğra Kaytanlı, Aimal H. Khankhel, Noy Cohen, Megan T. Valentine
We measure cell-generated forces from the deformations of elastic microspheres embedded within multicellular aggregates. Using a computationally efficient analytical model, we directly obtain the full 3D mapping of surface stresses within minutes.
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Rapid characterization of neutral polymer brush with a conventional zetameter and a variable pinch of salt

Soft Matter, 2020, 16,4274-4282
DOI: 10.1039/C9SM01850F, Paper
Mena Youssef, Alexandre Morin, Antoine Aubret, Stefano Sacanna, Jérémie Palacci
We take advantage of the nanoscopic nature of the Debye length and used it as a probe to characterize polymer brushes on colloidal particles.
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Surface-topology-controlled mechanical characteristics of triply periodic carbon Schwarzite foams

Soft Matter, 2020, 16,4324-4338
DOI: 10.1039/D0SM00136H, Paper
Hao Gong, Jinjie Liu, Ke Xu, Jianyang Wu, Yang Li
Carbon Schwarzites exhibit unique mechanical characteristics that are dominated by their topologies, rather than the mass density.
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Structural characterization of fibrous synthetic hydrogels using fluorescence microscopy

Soft Matter, 2020, 16,4210-4219
DOI: 10.1039/C9SM01828J, Paper
Open Access
Johannes Vandaele, Boris Louis, Kaizheng Liu, Rafael Camacho, Paul H. J. Kouwer, Susana Rocha
The structural features of the matrix surrounding the cells play a crucial role in regulating their behavior.
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Vesicle adhesion in the electrostatic strong-coupling regime studied by time-resolved small-angle X-ray scattering

Soft Matter, 2020, 16,4142-4154
DOI: 10.1039/D0SM00259C, Paper
Open Access
Karlo Komorowski, Jannis Schaeper, Michael Sztucki, Lewis Sharpnack, Gerrit Brehm, Sarah Köster, Tim Salditt
We have used time-resolved small-angle X-ray scattering (SAXS) to study the adhesion of lipid vesicles in the electrostatic strong-coupling regime induced by divalent ions.
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Mechanical robustness of monolayer nanoparticle-covered liquid marbles

Soft Matter, 2020, Advance Article
DOI: 10.1039/D0SM00496K, Paper
Junchao Huang, Ziheng Wang, Haixiao Shi, Xiaoguang Li
A particle shell as thin as ∼20 nm cannot protect internal liquid from wetting external solid.
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