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Reproducible generation of human liver organoids (HLOs) on a pillar plate platform via microarray 3D bioprinting

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Lab Chip, 2024, Accepted Manuscript
DOI: 10.1039/D4LC00149D, Paper
Sunil Shrestha, Vinod Kumar Reddy Lekkala, Prabha Acharya, Soo-Yeon Kang, Manav Goud Vanga, Moo-Yeal Lee
Human liver organoids (HLOs) hold significant potential for recapitulating the architecture and function of liver tissues in vivo. However, conventional culture methos of HLOs, forming Matrigel domes in 6-/24-well plates,...
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Correction: Direct laser writing-enabled 3D printing strategies for microfluidic applications

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Lab Chip, 2024, Advance Article
DOI: 10.1039/D4LC90040E, Correction
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Olivia M. Young, Xin Xu, Sunandita Sarker, Ryan D. Sochol
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Versatile hybrid technique for passive straight micromixer manufacturing by combining pulsed laser ablation, stereolithographic 3D printing and computational fluid dynamics

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Lab Chip, 2024, Advance Article
DOI: 10.1039/D4LC00009A, Paper
Open Access
Bastián Carnero, Yago Radziunas-Salinas, Bruno K. Rodiño-Janeiro, Sylvana Varela Ballesta, M. Teresa Flores-Arias
The proposed hybrid technique for passive straight micromixer manufacturing by combining pulsed laser ablation and stereolithographic 3D printing.
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Drug testing of monodisperse arrays of live microdissected tumors using a valved multiwell microfluidic platform

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Lab Chip, 2024, Advance Article
DOI: 10.1039/D4LC00016A, Paper
Ethan J. Lockhart, Lisa F. Horowitz, Adán Rodríguez, Songli Zhu, Tran Nguyen, Mehdi Mehrabi, Taranjit S. Gujral, Albert Folch
A microfluidic platform was developed that hydrodynamically traps microdissected cuboids for selective drug treatments and isolates conditions with thermoplastic valves.
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ChemPren: a new and economical technology for conversion of waste plastics to light olefins

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React. Chem. Eng., 2024, Advance Article
DOI: 10.1039/D4RE00354C, Perspective
Anne Gaffney, Debtanu Maiti, Debasish Kuila, Gennaro Mafia
With the ever-increasing demand for plastics, sustainable recycling methods is a key necessity.
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Bifunctional catalysts for the coupling processes of CO2 capture and conversion: a minireview

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React. Chem. Eng., 2024, Advance Article
DOI: 10.1039/D4RE00334A, Minireview
Chengxiong Dang, Hao Yu
A bifunctional catalyst for integrated CO2 capture and utilization (ICCU).
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Development and Simulation of Annular Flow Photoreactors: Integration of Light-Diffusing Fibers as optical diffusers with Laser Diodes

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React. Chem. Eng., 2024, Accepted Manuscript
DOI: 10.1039/D4RE00400K, Paper
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Sergio Carrillo De Hert, Rafael Lopez-Rodriguez, Michael Di Maso, Jonathan McMullen, Steven Ferguson
Continuous flow chemical photoreactors have emerged as a highly attractive platform, garnering considerable attention in both industry and academia. Utilizing thin channels, these reactors offer a promising solution for achieving...
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Linear scaling relationships in homogeneous photoredox catalysis

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React. Chem. Eng., 2024, Advance Article
DOI: 10.1039/D4RE00419A, Communication
Kareesa J. Kron, Shaama Mallikarjun Sharada
In the photoredox catalytic cycle of CO2 reduction with organic chromophores, this work observes a linear relationship between the energies of (desirable) electron transfer to CO2 and (undesirable) carboxylation of the chromophore radical anion.
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Digital strategies to improve the product quality and production efficiency of fluorinated polymers: 2. Heat removal performance of reactor with internal and external cooling systems

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React. Chem. Eng., 2024, Advance Article
DOI: 10.1039/D4RE00203B, Paper
Xi-Bao Zhang, Yin-Ning Zhou, Hao Chen, Zheng-Hong Luo, Liyang Zhou, Guojun Yu, Wenwu Liu, Shiping Zhu
A reactor's heat transfer efficiency can be significantly enhanced and the fluid temperature uniformity can be controlled through introducing cooling water in the agitator and regulating the flow ratio of cooling water in the agitator and jacket.
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One-pot enzymatic synthesis of L-5-methyltetrahydrofolate from folic acid using enzyme cascades

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React. Chem. Eng., 2024, Advance Article
DOI: 10.1039/D4RE00237G, Communication
Linjiang Zhu, Yuxin Wang, Linyan Pan, Enyong Lin, Jiayan Wang, Xiaolong Chen
A simple and cost-effective one-pot three-enzyme cascade reaction for high-yield production of L-5-methyltetrahydrofolate, including dihydrofolate reductase, tetrahydrofolate-dependent methyltransferase and alcohol dehydrogenase.
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Kinetics of the valorization of hexoses with Sn-USY catalysts in methanolic media: glycosidation vs. retroaldol cleavage

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React. Chem. Eng., 2024, Advance Article
DOI: 10.1039/D4RE00307A, Paper
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
J. M. Jimenez-Martin, M. El Tawil-Lucas, C. García-Jerez, J. Moreno, A. García, B. Hernández, J. Iglesias
Two operational regions in the transformation of hexoses have been revealed by experimental and kinetic analysis: glycosidation and retroaldol cleavage at low and high temperatures, respectively.
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Evaluating metal-free quaternized boronate esters as efficient catalysts for the fixation of CO2 with epoxides to form cyclic carbonates under suitable conditions

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React. Chem. Eng., 2024, 9,2938-2953
DOI: 10.1039/D4RE00282B, Paper
Eyyup Yasar, Emine Aytar, Ahmet Kilic
The conversion of CO2 into high value-added chemicals is receiving increasing attention from the scientific community, commercial enterprises, and policymakers due to environmental problems like global warming.
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The graph automorphism group of the dissociation microequilibrium of polyprotic acids

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React. Chem. Eng., 2024, 9,2925-2937
DOI: 10.1039/D4RE00271G, Paper
Nicolás Salas, Justin López, Carlos A. Arango
Effect of permutations σ12,0 and σ21 on graph G2.
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Propane dehydrogenation on an extra-framework and framework-embedded metal site within ZSM-5 zeolite from first-principles microkinetic simulations

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React. Chem. Eng., 2024, 9,2892-2901
DOI: 10.1039/D4RE00269E, Paper
Yujue Du, Wende Hu, Yunlei Chen, Chuanming Wang, Weimin Yang
The Lewis acid sites in ZSM-5 zeolite involving Co, Ni, and Cu cations were computationally studied on the stability and the PDH catalytic activity.
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Kinetics of thermal dry reforming of methane for syngas production and solid carbon capture

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React. Chem. Eng., 2024, 9,2902-2914
DOI: 10.1039/D4RE00312H, Paper
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Manas Mokashi, Akash Bhimrao Shirsath, Sinan Demir, Ahmet Çelik, Patrick Lott, Steffen Tischer, Olaf Deutschmann
By combining numerical simulations and experiments, catalyst-free thermal dry reforming of biogas for sustainable syngas production and solid carbon capture is investigated under industrially viable conditions.
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A novel magnetic nanoparticle as an efficient and recyclable heterogeneous catalyst for the Suzuki cross-coupling reaction

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React. Chem. Eng., 2024, 9,2954-2962
DOI: 10.1039/D4RE00226A, Paper
Hui Jin, Mengyu Cui, Peiwen Liu, Zhuo Wang, Tongxia Jin, Yonghui Yang, Weiping Zhu, Xuhong Qian
A novel magnetically recyclable heterogeneous palladium catalyst Fe3O4@FSM@Pd was constructed and characterized, which is highly efficient and reusable for the Suzuki–Miyaura cross-coupling reaction.
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Current research status on the structural properties and modification of LiFePO4 cathode materials

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React. Chem. Eng., 2024, 9,2830-2845
DOI: 10.1039/D4RE00263F, Review Article
Guo Xiaoying, Bao Yuanyuan, Li Wei, Zhao Siqin, Huang Chao
With the current global economy developing at a rapid pace, research into lithium-ion batteries has become a focal point in many major areas.
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Fabrication of black TiO2 through microwave heating for visible light-driven photocatalytic degradation of rhodamine 6G

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React. Chem. Eng., 2024, 9,3003-3015
DOI: 10.1039/D4RE00202D, Paper
Riska Rachmantyo, Afif Akmal Afkauni, Ricky Reinaldo, Lei Zhang, Arramel Arramel, Muhammad Danang Birowosuto, Arie Wibowo, Hermawan Judawisastra
This study shows that a narrower band gap TiO2, namely black TiO2, can be prepared using NaBH4 as a reducing material and microwave heating, which is a faster, greener, and simpler method than the existing method using furnace heating.
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Immobilization of cationic dye on photoluminescent hydroxyapatite particles through a citric acid bonding layer

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React. Chem. Eng., 2024, 9,2863-2867
DOI: 10.1039/D4RE00277F, Communication
Daichi Noda, Wanyu Shi, Aiga Yamada, Zizhen Liu, Motohiro Tagaya
Promotion of the immobilization of cationic porphyrin on Eu(III) ion-doped hydroxyapatite nanoparticles through citric acid as the bonding layer was achieved.
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Kinetic analysis of kraft lignin conversion via the Fenton process: process optimization and stochastic modelling

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React. Chem. Eng., 2024, Advance Article
DOI: 10.1039/D4RE00401A, Paper
Lucas Ramos, Giovani Maltempi-Mendes, Adriano Francisco Siqueira, Diovana Aparecida dos Santos Napoleão, Anuj Kumar Chandel
Lignin conversion through an advanced oxidative process.
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Unveiling the dynamic CO2 capture performance of MgO promoted with molten salts and CaCO3 via fixed bed reactor experiments

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React. Chem. Eng., 2024, Advance Article
DOI: 10.1039/D4RE00432A, Paper
Open Access
Theodoros Papalas, Andy N. Antzaras, Angeliki A. Lemonidou
MgO promoted with molten alkali salts and CaCO3 displayed efficient CO2 capture activity in a fixed bed reactor, attaining 75% CO2 removal at 275 °C and stable cyclic performance, with the promoters providing an alternative carbonation mechanism.
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CO2 hydrogenation to light olefins over Fe–Co/K–Al2O3 catalysts prepared via microwave calcination

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React. Chem. Eng., 2024, Advance Article
DOI: 10.1039/D4RE00428K, Paper
Nutkamaithorn Polsomboon, Thanapha Numpilai, Kulpavee Jitapunkul, Kajornsak Faungnawakij, Metta Chareonpanich, Xingda An, Le He, Günther Rupprechter, Thongthai Witoon
Microwave calcination optimizes the Fe–C/Fe3O4 ratio to 0.34, enhancing CO2 conversion and light olefin yield.
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Selective Separation of Li, Ni, Co and Mn from Model Spent Li Ion Battery Cathode by Dry Processing using Combination of Chlorination and Oxidation

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React. Chem. Eng., 2024, Accepted Manuscript
DOI: 10.1039/D4RE00328D, Paper
Naoto Tsubouchi, Yuuki Mochizuki
The volatilization of Li, Ni, Co, and Mn during chlorination treatment of LNO, LCO, and LMO (model materials for used LIB cathode material) was investigated with the aim of developing...
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Design and performance evaluation of low-volatility and low-viscosity absorbents for CO2 capture

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React. Chem. Eng., 2024, Advance Article
DOI: 10.1039/D4RE00379A, Paper
Ning Ma, Liu Yang, Zhenchang Fang, Kaijia Jiang, Xinling Li, Zhen Huang
This study synthesized a novel homogeneous non-aqueous absorbent and analyzed hydrogen bonds and viscosities, which were rarely studied before.
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Sugar additive with a halogen group enabling a highly reversible and dendrite-free Zn anode

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React. Chem. Eng., 2024, Advance Article
DOI: 10.1039/D4RE00366G, Paper
Weihao Xu, Xipo Ma, Pengbo Lyu, Zhenren Gao, Chunshuang Yan, Chade Lv
Sucralose, a weakly polar sugar electrolyte additive containing halogen elements, enables a highly reversible and dendrite-free Zn anode.
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Nickel foam supported biochar doped Ni–Mo bimetallic oxide for supercapacitor application

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React. Chem. Eng., 2024, Advance Article
DOI: 10.1039/D4RE00471J, Paper
Zhongxin Jin, Kaijia Hu, Feng Lin, Siqi Liu, Ruining Gu, Wei Zhang, Siyu Liu, Caiying Li, Hongyang Liao, Xinping Cai, Haijun Pang, Chunjing Zhang, Huiyuan Ma
A novel C-MoO3-NiO2/NF electrode derived from polyoxometalate and rice is obtained and provides a new strategy for the development of high-performance supercapacitors.
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Trapping bond exchange phenomenon revealed for off-stoichiometry cross-linking of phase-separated vitrimer-like materials

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Soft Matter, 2024, 20,2961-2968
DOI: 10.1039/D4SM00074A, Paper
Takumi Kito, Mikihiro Hayashi
Unusual relaxation and creep properties by the trapping bond exchange phenomenon is revealed for vitrimer-like materials with bond exchangeable domains of quaternized pyridines, in the special case of off- stoichiometric cross-linking condition.
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A computational study of nematic core structure and disclination interactions in elastically anisotropic nematics

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Soft Matter, 2024, 20,2900-2914
DOI: 10.1039/D3SM01616A, Paper
Lucas Myers, Carter Swift, Jonas Rønning, Luiza Angheluta, Jorge Viñals
The structure of isolated disclinations and disclination dipoles in anisotropically elastic nematic liquid crystals is explored via a singular potential computational model.
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Motion of microswimmers in cylindrical microchannels

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Soft Matter, 2024, 20,3007-3020
DOI: 10.1039/D3SM01480K, Paper
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Florian A. Overberg, Gerhard Gompper, Dmitry A. Fedosov
Microswimmers in confinement slow down, and can exert pulling or pushing forces in particular at the end of a closed channel. Simulations and approximate theoretical calculation for the squirmer model are employed to predict this behavior.
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Phenylboronate-salicylate ester cross-linked self-healing hydrogel composed of modified hyaluronan at physiological pH

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Soft Matter, 2024, 20,2926-2936
DOI: 10.1039/D3SM01417G, Paper
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Ryotaro Miki, Tsutomu Yamaki, Masaki Uchida, Hideshi Natsume
A self-healing hydrogel can be easily prepared at physiological pH by using phenylboronic acid-modified hyaluronic acid and salicylic acid-modified hyaluronic acid.
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Self-adhesion of uncrosslinked poly(butadiene-co-acrylonitrile), i.e. nitrile rubber, an inhomogeneous and associative polymer

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Soft Matter, 2024, 20,2978-2985
DOI: 10.1039/D3SM01630G, Paper
Valentine Hervio, Annie Brûlet, Costantino Creton, Gabriel E. Sanoja
The precursor of NBR, poly(acrylonitrile-co-butadiene), experiences thermodynamic forces for self-assembly and kinetic barriers for processing. We introduce three strategies to overcome such barriers and enable polymer self-adhesion in the bulk.
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A bio-inspired co-simulation crawling robot enabled by a carbon dot-doped dielectric elastomer

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Soft Matter, 2024, Advance Article
DOI: 10.1039/D4SM00029C, Paper
Yubing Han, Bori Shi, En Xie, Peng Huang, Yaozhong Zhou, Chang Xue, Weijia Wen, Huayan Pu, Mengying Zhang, Jinbo Wu
The introduction of NCDs@SiO2 cluster particles not only improves the mechanical and dielectric properties of an elastomer but also exhibits fluorescence and actuation response under the co-stimulation of UV and electricity, respectively.
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Agent-based modeling of stress anisotropy driven nematic ordering in growing biofilms

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Soft Matter, 2024, Advance Article
DOI: 10.1039/D3SM01535A, Paper
Open Access
Changhao Li, Japinder Nijjer, Luyi Feng, Qiuting Zhang, Jing Yan, Sulin Zhang
Our agent-based model reveals complex spatiotemperal evolution of the morphology and internal cell ordering of Vibrio cholerae biofilms.
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Slip of a liquid crystal droplet rotator in viscous fluids

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Soft Matter, 2024, 20,3066-3072
DOI: 10.1039/D3SM01028G, Paper
Keita Saito, Yasuyuki Kimura
The boundary conditions at the droplet surface depend on the surrounding solution. In glycerol solutions, slip occurs at the droplet surface and is enhanced as glycerol concentration increases.
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Form II to form I transition in solution-crystallized isotactic polybutene-1

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Soft Matter, 2024, 20,3191-3202
DOI: 10.1039/D4SM00152D, Paper
Peng Fu, Jiaxin Huo, Jingqing Li, Claudio De Rosa, Shichun Jiang
Different polymer chains in a solution or melt have different conformations with corresponding entropy at each moment, which would be confined after crystallization.
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Steering droplets on substrates with plane-wave wettability patterns and deformations

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Soft Matter, 2024, 20,3161-3174
DOI: 10.1039/D4SM00213J, Paper
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Josua Grawitter, Holger Stark
Motivated by strategies for targeted microfluidic transport of droplets, we investigate how sessile droplets can be steered toward a preferred direction using travelling waves in substrate wettability or deformations of the substrate.
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A microrheological examination of insulin-secreting β-cells in healthy and diabetic-like conditions

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Soft Matter, 2024, Advance Article
DOI: 10.1039/D3SM01141K, Paper
Open Access
Lukas Woolley, Adam Burbidge, Jan Vermant, Fotis Christakopoulos
We provide an insight into the compliance of β-cells and explore structural changes in conditions relevant to type-2 diabetes, showing an altered transport behavior and hindering the effective control of insulin secretion.
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A computational study of cell membrane damage and intracellular delivery in a cross-slot microchannel

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Soft Matter, 2024, Advance Article
DOI: 10.1039/D4SM00047A, Paper
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Ruixin Lu, Peng Yu, Yi Sui
The inertial effect increases the cell deformation and membrane damage in the channel cross-slot; however, the enhancement can be reversed by the cell membrane viscosity.
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Adsorption of semiflexible wormlike polymers to a bar and their double-chain complex formation

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Soft Matter, 2024, Advance Article
DOI: 10.1039/D4SM00188E, Paper
Open Access
A. N. Semenov, I. A. Nyrkova
The quantitative transfer matrix approach and scaling arguments in terms of trains, loops, tails and supertrains allowed us to characterize the main regimes of semiflexible chain adsorption on a bar and double-chain complex formation.
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Faceted wrinkling by contracting a curved boundary

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Soft Matter, 2024, Advance Article
DOI: 10.1039/D3SM01347B, Paper
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Anshuman S. Pal, Luka Pocivavsek, Thomas A. Witten
A novel mode of wrinkling avoids stretching by forming tilted, triangular facets.
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Measuring mechanical cues for modeling the stromal matrix in 3D cell cultures

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Soft Matter, 2024, Advance Article
DOI: 10.1039/D3SM01425H, Paper
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Linda Srbova, Ossi Arasalo, Arttu J. Lehtonen, Juho Pokki
An approach to quantify microscale viscoelasticity in breast-cancer-associated stromal tissues was developed for cell-scale analyses of physiologically stiff 3D cell cultures.
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Enzymatic functionalization of decellularized tilapia skin scaffolds with enhanced skin regeneration

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Soft Matter, 2024, Advance Article
DOI: 10.1039/D3SM01742G, Paper
Cuixia Chen, Wenwen Tao, Di Jiang, Yanyan Yang, Tiantian Liang, Qilong Gu, Yuran Xu, Junjuan Zhao, Xing Zhou, Xinglong Fan
The enzymatic dTS/RGD scaffolds, possessing medium mechanical strength, a rapid degradation rate and enough cell responsive motifs, provide a suitable microenvironment for wound healing, which make them potential in skin regeneration engineering.
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Pinning–depinning transition of droplets on inclined substrates with a three-dimensional topographical defect

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Soft Matter, 2024, Advance Article
DOI: 10.1039/D4SM00081A, Paper
Ninad V. Mhatre, Satish Kumar
The influence of defect geometry on the critical inclination angle required for droplet depinning on inclined substrates is studied.
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Dynamic compaction of cohesive granular materials: scaling behavior and bonding structures

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Soft Matter, 2024, Advance Article
DOI: 10.1039/D3SM01116J, Paper
Open Access
Max Sonzogni, Jean-Mathieu Vanson, Katerina Ioannidou, Yvan Reynier, Sébastien Martinet, Farhang Radjai
The compaction of cohesive granular materials is a common operation in powder-based manufacture of many products.
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Hydrogen bonding enhanced drug–polymer interaction for efficient drug loading and delivery

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Soft Matter, 2024, Advance Article
DOI: 10.1039/D4SM00003J, Communication
Xiaotian Qu, Junran Li, Yishu Yu, Jie Yang
A carrier design strategy of hydrogen bonding enhanced drug–carrier interaction is developed to prepare a polymeric nanomedicine with high drug loading content and superb loading efficiency as well as tunable nanostructures.
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Self-healing polyacrylates based on dynamic disulfide and quadruple hydrogen bonds

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Soft Matter, 2024, Advance Article
DOI: 10.1039/D4SM00257A, Paper
Longjin Du, Yuting Zhong, Linying Zhao, Chengzhen Hu, Liang Shen, Yuping Yang, Jiang Zhong
Herein, a self-healing polyacrylate system was successfully prepared by introducing crosslinking agents containing disulfide bonds and monomers capable of forming quadruple hydrogen bonds through free radical copolymerization.
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Temperature dependence of micelle shape transitions in copolymer solutions: the role of inter-block incompatibility

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Soft Matter, 2024, Advance Article
DOI: 10.1039/D4SM00331D, Paper
Open Access
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M. J. Greenall, M. J. Derry
The incompatibility of the blocks in a copolymer strongly affects the temperature dependence of the micelle shape transitions in solution.
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Spontaneous crumpling of active spherical shells

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Soft Matter, 2024, Advance Article
DOI: 10.1039/D4SM00015C, Paper
Open Access
M. C. Gandikota, Shibananda Das, A. Cacciuto
The existence of a crumpled Flory phase for equilibrated self-avoiding elastic surfaces has remained contentious. Here, we show that a crumpled phase develops reliably upon subjecting a thin spherical self-avoiding shell to active fluctuations.
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The interplay of chirality and restricted rotation: stabilisation of chiral, frustrated mesophases over a wide thermal range

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Soft Matter, 2024, Advance Article
DOI: 10.1039/D4SM00126E, Paper
Sachin A. Bhat, Channabasaveshwara V. Yelamaggad
Chiral dimers formed by linking cholesterol to phenyl 3-(4-(n-alkoxy)phenyl)propiolate via ω-oxyalkanoyloxy spacer exhibit odd–even effect, stabilizing SmA, N*, BPI/II, & TGBC* phases. TGBC* phase width increases with longer terminal tails.
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Multiple physical crosslinked highly adhesive and conductive hydrogels for human motion and electrophysiological signal monitoring

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Soft Matter, 2024, Advance Article
DOI: 10.1039/D4SM00195H, Paper
Qirui Wu, Anbang Chen, Yidan Xu, Songjiu Han, Jiayu Zhang, Yujia Chen, Jianren Hang, Xiaoxiang Yang, Lunhui Guan
Ionic conducting hydrogel (ICHgel) was synthesized by doping fumed SiO2, which exhibited superior stretchability, conductivity, and adhesiveness, making it a promising bridge for effective communication between electronic devices and human tissues.
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