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ChemPren: a new and economical technology for conversion of waste plastics to light olefins

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React. Chem. Eng., 2024, Advance Article
DOI: 10.1039/D4RE00354C, Perspective
Anne Gaffney, Debtanu Maiti, Debasish Kuila, Gennaro Mafia
With the ever-increasing demand for plastics, sustainable recycling methods is a key necessity.
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Bifunctional catalysts for the coupling processes of CO2 capture and conversion: a minireview

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React. Chem. Eng., 2024, Advance Article
DOI: 10.1039/D4RE00334A, Minireview
Chengxiong Dang, Hao Yu
A bifunctional catalyst for integrated CO2 capture and utilization (ICCU).
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Development and Simulation of Annular Flow Photoreactors: Integration of Light-Diffusing Fibers as optical diffusers with Laser Diodes

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React. Chem. Eng., 2024, Accepted Manuscript
DOI: 10.1039/D4RE00400K, Paper
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Sergio Carrillo De Hert, Rafael Lopez-Rodriguez, Michael Di Maso, Jonathan McMullen, Steven Ferguson
Continuous flow chemical photoreactors have emerged as a highly attractive platform, garnering considerable attention in both industry and academia. Utilizing thin channels, these reactors offer a promising solution for achieving...
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Digital strategies to improve the product quality and production efficiency of fluorinated polymers: 2. Heat removal performance of reactor with internal and external cooling systems

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React. Chem. Eng., 2024, Advance Article
DOI: 10.1039/D4RE00203B, Paper
Xi-Bao Zhang, Yin-Ning Zhou, Hao Chen, Zheng-Hong Luo, Liyang Zhou, Guojun Yu, Wenwu Liu, Shiping Zhu
A reactor's heat transfer efficiency can be significantly enhanced and the fluid temperature uniformity can be controlled through introducing cooling water in the agitator and regulating the flow ratio of cooling water in the agitator and jacket.
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One-pot enzymatic synthesis of L-5-methyltetrahydrofolate from folic acid using enzyme cascades

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React. Chem. Eng., 2024, Advance Article
DOI: 10.1039/D4RE00237G, Communication
Linjiang Zhu, Yuxin Wang, Linyan Pan, Enyong Lin, Jiayan Wang, Xiaolong Chen
A simple and cost-effective one-pot three-enzyme cascade reaction for high-yield production of L-5-methyltetrahydrofolate, including dihydrofolate reductase, tetrahydrofolate-dependent methyltransferase and alcohol dehydrogenase.
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Technoeconomic analysis of fine chemical electrosynthesis: a case study using electrooxidation of 2-methylnaphthelene to vitamin K3

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React. Chem. Eng., 2024, Advance Article
DOI: 10.1039/D4RE00346B, Paper
Qifeng Yang, Liping Liang, Ning Xu, Yang Li, Zhihui Wang, Dadong Shen, Yiming Mo
A cerium-mediated electrooxidation method was developed for synthesizing vitamin K3 in a green and efficient manner. A systematic technoeconomic analysis was provided to understand its potential for practical implementation.
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Kinetics of the valorization of hexoses with Sn-USY catalysts in methanolic media: glycosidation vs. retroaldol cleavage

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React. Chem. Eng., 2024, Advance Article
DOI: 10.1039/D4RE00307A, Paper
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
J. M. Jimenez-Martin, M. El Tawil-Lucas, C. García-Jerez, J. Moreno, A. García, B. Hernández, J. Iglesias
Two operational regions in the transformation of hexoses have been revealed by experimental and kinetic analysis: glycosidation and retroaldol cleavage at low and high temperatures, respectively.
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Evaluating metal-free quaternized boronate esters as efficient catalysts for the fixation of CO2 with epoxides to form cyclic carbonates under suitable conditions

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React. Chem. Eng., 2024, 9,2938-2953
DOI: 10.1039/D4RE00282B, Paper
Eyyup Yasar, Emine Aytar, Ahmet Kilic
The conversion of CO2 into high value-added chemicals is receiving increasing attention from the scientific community, commercial enterprises, and policymakers due to environmental problems like global warming.
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The graph automorphism group of the dissociation microequilibrium of polyprotic acids

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React. Chem. Eng., 2024, 9,2925-2937
DOI: 10.1039/D4RE00271G, Paper
Nicolás Salas, Justin López, Carlos A. Arango
Effect of permutations σ12,0 and σ21 on graph G2.
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Kinetics of thermal dry reforming of methane for syngas production and solid carbon capture

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React. Chem. Eng., 2024, 9,2902-2914
DOI: 10.1039/D4RE00312H, Paper
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Manas Mokashi, Akash Bhimrao Shirsath, Sinan Demir, Ahmet Çelik, Patrick Lott, Steffen Tischer, Olaf Deutschmann
By combining numerical simulations and experiments, catalyst-free thermal dry reforming of biogas for sustainable syngas production and solid carbon capture is investigated under industrially viable conditions.
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Combination of near-infrared spectroscopy and a transient flow method for efficient kinetic analysis of the Claisen rearrangement

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React. Chem. Eng., 2024, 9,2975-2983
DOI: 10.1039/D4RE00301B, Paper
Yoshihiro Takebayashi, Kiwamu Sue, Sho Kataoka
An automated flow reactor with a rapid inline monitoring using a compact near-infrared spectrometer and a flow rate ramp control enabled high-density kinetic data acquisition.
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Dual jet-mixing reactor for fully continuous synthesis of core@shell Au@Ag nanocomposites

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React. Chem. Eng., 2024, 9,2915-2924
DOI: 10.1039/D3RE00417A, Paper
Open Access
Pinaki Ranadive, Faiz Khan, Jessica O. Winter, Nicholas Brunelli
Sequential jet mixing reactors enable core@shell nanomaterial synthesis.
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Optimization of reaction parameters for the synthesis of natural aroma esters by factorial design

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React. Chem. Eng., 2024, 9,2994-3002
DOI: 10.1039/D4RE00265B, Paper
Open Access
Adrian Ioan Dudu, Csaba Paizs, Monica Ioana Toşa
In this study, the synthesis of aroma esters by the direct esterfication of carboxylic acids with aromatic alcohols mediated by lipase B from Candida antarctica encapsulated in a sol–gel matrix in a solvent-free system is presented.
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Current research status on the structural properties and modification of LiFePO4 cathode materials

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React. Chem. Eng., 2024, 9,2830-2845
DOI: 10.1039/D4RE00263F, Review Article
Guo Xiaoying, Bao Yuanyuan, Li Wei, Zhao Siqin, Huang Chao
With the current global economy developing at a rapid pace, research into lithium-ion batteries has become a focal point in many major areas.
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Closed-loop identification of enzyme kinetics applying model-based design of experiments

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React. Chem. Eng., 2024, 9,2984-2993
DOI: 10.1039/D4RE00127C, Paper
Leon Hennecke, Lucas Schaare, Mirko Skiborowski, Andreas Liese
This study presents an automated reactor platform for the identification of enzyme kinetic models using model-based design of experiments on the example of the reduction of NAD+ by formate dehydrogenase from Candida boidinii.
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Bayesian-optimization-based design of highly active and stable Fe–Cu/SSZ-13 catalysts for the selective catalytic reduction of NOx with NH3

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React. Chem. Eng., 2024, 9,3029-3037
DOI: 10.1039/D4RE00327F, Paper
Sanha Lim, Hwangho Lee, Hyun Sub Kim, Jun Seop Shin, Jong Min Lee, Do Heui Kim
Bayesian optimization approach facilitates an efficient optimization of multi-components catalyst for NH3-SCR reaction.
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Review of hydrogen ortho–para conversion: experimental data and reaction kinetics

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React. Chem. Eng., 2024, 9,2846-2862
DOI: 10.1039/D4RE00259H, Review Article
Fuyu Jiao, Saif Al Ghafri, Keelan T. O'Neill, Paul S. Stanwix, Guinevere M. Sellner, Einar O. Fridjonsson, Neil Robinson, Eric F. May, Michael L. Johns
This work reviews ortho–para hydrogen conversion data for various types of catalysts at cryogenic temperatures and evaluates different reaction kinetic expressions employed to describe these experimental data.
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Fabrication of black TiO2 through microwave heating for visible light-driven photocatalytic degradation of rhodamine 6G

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React. Chem. Eng., 2024, 9,3003-3015
DOI: 10.1039/D4RE00202D, Paper
Riska Rachmantyo, Afif Akmal Afkauni, Ricky Reinaldo, Lei Zhang, Arramel Arramel, Muhammad Danang Birowosuto, Arie Wibowo, Hermawan Judawisastra
This study shows that a narrower band gap TiO2, namely black TiO2, can be prepared using NaBH4 as a reducing material and microwave heating, which is a faster, greener, and simpler method than the existing method using furnace heating.
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Complete kinetic model and process reengineering of glyoxal oxidation by nitric acid in a capillary microreactor

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React. Chem. Eng., 2024, 9,3016-3028
DOI: 10.1039/D4RE00313F, Paper
Junnan Wang, Wei Zhan, Yating Li, Ting Wang, Chengxiang He, Chunying Zhu, Youguang Ma, Taotao Fu
The oxidation of glyoxal by nitric acid to glyoxylic acid is a complex process with parallel and consecutive side reactions.
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Boosting the kinetics of PET glycolysis

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React. Chem. Eng., 2024, 9,3038-3046
DOI: 10.1039/D4RE00235K, Paper
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Maria Schlüter, Ryota Enomoto, Shin Makino, Lisa Weihs, Cyra Lina Stamm, Kerstin Wohlgemuth, Christoph Held
Glycolysis is the most promising chemical recycling method to depolymerize poly(ethylene terephthalate) (PET) with ethylene glycol (EG) into the monomer bis(2-hydroxyethyl) terephthalate (BHET).
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Immobilization of cationic dye on photoluminescent hydroxyapatite particles through a citric acid bonding layer

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React. Chem. Eng., 2024, 9,2863-2867
DOI: 10.1039/D4RE00277F, Communication
Daichi Noda, Wanyu Shi, Aiga Yamada, Zizhen Liu, Motohiro Tagaya
Promotion of the immobilization of cationic porphyrin on Eu(III) ion-doped hydroxyapatite nanoparticles through citric acid as the bonding layer was achieved.
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Kinetic analysis of kraft lignin conversion via the Fenton process: process optimization and stochastic modelling

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React. Chem. Eng., 2024, Advance Article
DOI: 10.1039/D4RE00401A, Paper
Lucas Ramos, Giovani Maltempi-Mendes, Adriano Francisco Siqueira, Diovana Aparecida dos Santos Napoleão, Anuj Kumar Chandel
Lignin conversion through an advanced oxidative process.
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“25 years of The Netherlands' Catalysis and Chemistry Conference (NCCC)” themed collection – A personal invitation Aromatization of n-alkanes: a mini review on catalysts and reactants

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React. Chem. Eng., 2024, Accepted Manuscript
DOI: 10.1039/D4RE00384E, Minireview
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Hongqi Wang, Raveendran N. Shiju
The catalytic aromatization of n-alkanes is an important process in the chemical industry, especially for the production of valued-added aromatics from the abundant and unreactive small alkanes. This mini review...
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Scalable electrocatalyzed formation of C–O bonds using flow reactor technology

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React. Chem. Eng., 2024, Advance Article
DOI: 10.1039/D4RE00438H, Paper
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Michael Prieschl, David Cantillo, C. Oliver Kappe, Gabriele Laudadio
A scalable C–O bond formation via continuous-flow Ni-electrocatalysis was developed, enabling the gram-scale preparation of a key delamanid intermediate, a pharmaceutical used to treat multidrug-resistant tuberculosis.
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Kinetic insights into structure sensitivity of Ru catalyzed L-alanine hydrogenation to alaninol

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React. Chem. Eng., 2024, Advance Article
DOI: 10.1039/D4RE00420E, Paper
Rui Song, Chang Yao, Wenhua Li, Nihong An, Yafeng Shen, Nina Fei, Xiaohu Ge, Yueqiang Cao, Xuezhi Duan, Xinggui Zhou
Ru(101) sites are identified as the dominant active sites for the hydrogenation of L-alanine to alaninol.
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Two-temperature model of the non-thermal chemical dissociation of CO2

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React. Chem. Eng., 2024, Advance Article
DOI: 10.1039/D4RE00300D, Paper
Q. Shen, A. Pikalev, F. J. J. Peeters, J. Gans, M. C. M. van de Sanden
A two-temperature model with a vibrational temperature different from the gas temperature is presented for the decomposition of CO2.
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Transesterification or polymerization? Reaction mechanism and kinetics of 2-(diethylamino)ethyl methacrylate with methanol and the competitive effect on free-radical polymerization

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React. Chem. Eng., 2024, Advance Article
DOI: 10.1039/D4RE00406J, Paper
Judith Cabello-Romero, Román Torres-Lubián, Javier Francisco Enríquez-Medrano, Adrián Ochoa-Terán, Jesús Jara-Cortés, Iván Zapata-González
Transesterification of 2-(diethylamino)ethyl methacrylate (DEAEMA) with methanol leads to the formation of methyl methacrylate (MMA) and amino alcohol. This reaction significantly affects DEAEMA polymerization giving rise to poly(DEAEMA-co-MMA).
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Unveiling the dynamic CO2 capture performance of MgO promoted with molten salts and CaCO3 via fixed bed reactor experiments

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React. Chem. Eng., 2024, Advance Article
DOI: 10.1039/D4RE00432A, Paper
Open Access
Theodoros Papalas, Andy N. Antzaras, Angeliki A. Lemonidou
MgO promoted with molten alkali salts and CaCO3 displayed efficient CO2 capture activity in a fixed bed reactor, attaining 75% CO2 removal at 275 °C and stable cyclic performance, with the promoters providing an alternative carbonation mechanism.
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Removal of gaseous Hg0 by Cl-loaded carbonaceous material prepared from rice husk

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React. Chem. Eng., 2024, Advance Article
DOI: 10.1039/D4RE00414K, Paper
Naoto Tsubouchi, Momone Yoshizawa, Javzandogole Bud, Yuuki Mochizuki
The main objective of this study was to investigate the removal of gaseous Hg0 from the residue obtained during the chlorination of rice husk char to recover silica.
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Selective Separation of Li, Ni, Co and Mn from Model Spent Li Ion Battery Cathode by Dry Processing using Combination of Chlorination and Oxidation

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React. Chem. Eng., 2024, Accepted Manuscript
DOI: 10.1039/D4RE00328D, Paper
Naoto Tsubouchi, Yuuki Mochizuki
The volatilization of Li, Ni, Co, and Mn during chlorination treatment of LNO, LCO, and LMO (model materials for used LIB cathode material) was investigated with the aim of developing...
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Design and performance evaluation of low-volatility and low-viscosity absorbents for CO2 capture

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React. Chem. Eng., 2024, Advance Article
DOI: 10.1039/D4RE00379A, Paper
Ning Ma, Liu Yang, Zhenchang Fang, Kaijia Jiang, Xinling Li, Zhen Huang
This study synthesized a novel homogeneous non-aqueous absorbent and analyzed hydrogen bonds and viscosities, which were rarely studied before.
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Synthesis of ethylphenols and xanthenes via reaction of calcium carbide and phenol: experimental and theoretical studies

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React. Chem. Eng., 2024, Advance Article
DOI: 10.1039/D4RE00397G, Paper
Xin Liu, Yuxin Yan, Zhenyu Liu, Qingya Liu
A novel synthesis of xanthenes and ethylphenols by the reaction of phenol with CaC2 without catalysts and solvents.
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Trapping bond exchange phenomenon revealed for off-stoichiometry cross-linking of phase-separated vitrimer-like materials

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Soft Matter, 2024, 20,2961-2968
DOI: 10.1039/D4SM00074A, Paper
Takumi Kito, Mikihiro Hayashi
Unusual relaxation and creep properties by the trapping bond exchange phenomenon is revealed for vitrimer-like materials with bond exchangeable domains of quaternized pyridines, in the special case of off- stoichiometric cross-linking condition.
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Kinetics of phase separation and aging dynamics of segregating fluid mixtures in the presence of quenched disorder

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Soft Matter, 2024, 20,2969-2977
DOI: 10.1039/D4SM00204K, Paper
Rounak Bhattacharyya, Bhaskar Sen Gupta
Phase separation of segregating fluid mixtures in the presence of quenched disorder.
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A computational study of nematic core structure and disclination interactions in elastically anisotropic nematics

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Soft Matter, 2024, 20,2900-2914
DOI: 10.1039/D3SM01616A, Paper
Lucas Myers, Carter Swift, Jonas Rønning, Luiza Angheluta, Jorge Viñals
The structure of isolated disclinations and disclination dipoles in anisotropically elastic nematic liquid crystals is explored via a singular potential computational model.
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Preparation of modified humic acid/TiO2/P(AA-co-AM) nanocomposite hydrogels with enhanced dye adsorption and photocatalysis

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Soft Matter, 2024, 20,2937-2954
DOI: 10.1039/D3SM01749D, Paper
Xuankun Gong, Amatjan Sawut, Rena Simayi, Ziyue Wang, Yurou Feng
A novel composite hydrogel with exceptional adsorption and photocatalytic properties was synthesized using modified coal-based humic acid (HA-C), modified titanium dioxide (TiO2) nanoparticles, acrylic acid (AA), and acrylamide (AM) as precursors.
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Motion of microswimmers in cylindrical microchannels

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Soft Matter, 2024, 20,3007-3020
DOI: 10.1039/D3SM01480K, Paper
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Florian A. Overberg, Gerhard Gompper, Dmitry A. Fedosov
Microswimmers in confinement slow down, and can exert pulling or pushing forces in particular at the end of a closed channel. Simulations and approximate theoretical calculation for the squirmer model are employed to predict this behavior.
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Phenylboronate-salicylate ester cross-linked self-healing hydrogel composed of modified hyaluronan at physiological pH

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Soft Matter, 2024, 20,2926-2936
DOI: 10.1039/D3SM01417G, Paper
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Ryotaro Miki, Tsutomu Yamaki, Masaki Uchida, Hideshi Natsume
A self-healing hydrogel can be easily prepared at physiological pH by using phenylboronic acid-modified hyaluronic acid and salicylic acid-modified hyaluronic acid.
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Self-adhesion of uncrosslinked poly(butadiene-co-acrylonitrile), i.e. nitrile rubber, an inhomogeneous and associative polymer

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Soft Matter, 2024, 20,2978-2985
DOI: 10.1039/D3SM01630G, Paper
Valentine Hervio, Annie Brûlet, Costantino Creton, Gabriel E. Sanoja
The precursor of NBR, poly(acrylonitrile-co-butadiene), experiences thermodynamic forces for self-assembly and kinetic barriers for processing. We introduce three strategies to overcome such barriers and enable polymer self-adhesion in the bulk.
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Hydrodynamically induced aggregation of two dimensional oriented active particles

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Soft Matter, 2024, Advance Article
DOI: 10.1039/D3SM01670F, Paper
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Roee Bashan, Naomi Oppenheimer
We show that in many cases aligned active particles in a two-dimensional fluid attract and form fractal-like clusters.
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Analysis of the adhesive secreting cells of Arion subfuscus: insights into the role of microgels in a tough, fast-setting hydrogel glue

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Soft Matter, 2024, Advance Article
DOI: 10.1039/D4SM00071D, Paper
Andrew M. Smith, Patrick Flammang
A model for the rapid setting of a gastropod hydrogel adhesive. Cross-linked microgels mix with microscopic packets of polysaccharides; these flow onto surfaces until the packets rupture, joining the microgels together.
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Agent-based modeling of stress anisotropy driven nematic ordering in growing biofilms

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Soft Matter, 2024, Advance Article
DOI: 10.1039/D3SM01535A, Paper
Open Access
Changhao Li, Japinder Nijjer, Luyi Feng, Qiuting Zhang, Jing Yan, Sulin Zhang
Our agent-based model reveals complex spatiotemperal evolution of the morphology and internal cell ordering of Vibrio cholerae biofilms.
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Slip of a liquid crystal droplet rotator in viscous fluids

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Soft Matter, 2024, 20,3066-3072
DOI: 10.1039/D3SM01028G, Paper
Keita Saito, Yasuyuki Kimura
The boundary conditions at the droplet surface depend on the surrounding solution. In glycerol solutions, slip occurs at the droplet surface and is enhanced as glycerol concentration increases.
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Conformational and static properties of tagged chains in solvents: effect of chain connectivity in solvent molecules

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Soft Matter, 2024, 20,3073-3081
DOI: 10.1039/D3SM01473H, Paper
Hong-Yao Li, Bokai Zhang, Zhi-Yong Wang
The radius of gyration of tagged polymer chain: effect of chain length in solvent molecules.
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The fractal geometry of polymeric materials surfaces: surface area and fractal length scales

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Soft Matter, 2024, 20,3082-3096
DOI: 10.1039/D3SM01497E, Paper
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
H. Eduardo Roman, Federico Cesura, Rabia Maryam, Igor Levchenko, Katia Alexander, Claudia Riccardi
Non-treated (NT) and plasma-treated (PT) polymeric surfaces display self-affine fractal scaling. The plasma increases both the surface area and the fractal length scales, helping the design of PT interfaces with larger surface areas at the nm scale.
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Solutal Marangoni force controls lateral motion of electrolytic gas bubbles

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Soft Matter, 2024, 20,3097-3106
DOI: 10.1039/D3SM01646C, Paper
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Hongguang Zhang, Yunqing Ma, Mengyuan Huang, Gerd Mutschke, Xianren Zhang
The MD and CFD indicate that the lateral solutal Marangoni force originating from an asymmetric distribution of dissolved gas causes bubbles oscillation and self-pinning effect.
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Surfactant-induced alterations in optoelectronic properties of perylene diimide dyes: modulating sensing responses in the aqueous environment

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Soft Matter, 2024, 20,3044-3052
DOI: 10.1039/D3SM01694C, Paper
Animesh Pal, Nilanjan Dey
The compartmentalization effect of microheterogeneous systems, like surfactant aggregates, showcases altered optoelectronic properties of a perylene diimide-based chromogenic dye (PDI-Ala) compared to bulk water.
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Disorder-to-order transition of long fibers contained in evaporating sessile drops

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Soft Matter, 2024, 20,3107-3117
DOI: 10.1039/D3SM01735D, Paper
S. Sannyamath, R. Vetter, H. Bonart, M. Hartmann, R. Ganguly, S. Hardt
We demonstrate self-organization of hydrophilic fibers, contained in a sessile droplet in a disordered initial configurations, to transform into an order deposit. Findings suggest new avenues to decorate solid surfaces with filamental structures.
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Shear zones in granular mixtures of hard and soft particles with high and low friction

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Soft Matter, 2024, 20,3118-3130
DOI: 10.1039/D4SM00100A, Paper
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  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Aditya Pratap Singh, Vasileios Angelidakis, Thorsten Pöschel, Sudeshna Roy
Granular materials show inhomogeneous flows characterized by strain localization.
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Self-assembly of rod–coil–rod block copolymers in a coil-selective solvent: coarse-grained simulation results

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Soft Matter, 2024, 20,3131-3142
DOI: 10.1039/D4SM00251B, Paper
Chiraz Toujani, Luis A. Padilla, Nour Alhraki, Su-Mi Hur, Abelardo Ramírez-Hernández
Parameters that govern the self assembly of a symmetric triblock copolymer.
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