Org. Chem. Front., 2024, Accepted Manuscript
DOI: 10.1039/D4QO00552J, Research Article

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Liyao Ma, Sonia Mallet-Ladeira, Julien MONOT, Blanca Maria MARTIN VACA, Didier Bourissou
Cycloisomerization reactions involving C–P bond formation have been overlooked to prepare P-heterocycles. We discovered here a simple, efficient and versatile route to benzophosphole oxides by reacting ortho-alkynyl secondary phosphine oxides...
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Org. Chem. Front., 2024, Advance Article
DOI: 10.1039/D4QO00317A, Research Article

Guohui Zeng, Hui Luo, Kai Jiang, Jianpeng Cai, Biaolin Yin
Amine-tethered spiro-cyclic skeletons were obtained through photo-induced 100%-atom-economic dearomatization, involving the cleavage of the α-C(sp³)–H of amines. Pentacyclic framework was achieved from pyridinyl ring within two steps.
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Org. Chem. Front., 2024, Advance Article
DOI: 10.1039/D4QO00474D, Research Article

Peng He, Zongkang Wang, Qiongwen Kang, Nana Fei, Chengyu Wang, Yanzhong Li
An efficient B(C₆F₅)₃ catalyzed protocol for the synthesis of oxindole fused 1,3-oxazepanes from pyrrolidine substituted aryl alkynones has been developed.
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Org. Chem. Front., 2024, Advance Article
DOI: 10.1039/D4QO00356J, Research Article

Bohao Zhang, Sifan He, Na Dong, Antong Zhu, Haojie Duan, Dunjia Wang, Yao Zhou
An unprecedented metal-free divergent cyclization reaction of benzo[c][1,2]dithiol-3-ones with hexahydro-1,3,5-triazines to assemble six- and eight-membered N-containing heterocycles has been developed.
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Org. Chem. Front., 2024, Accepted Manuscript
DOI: 10.1039/D4QO00347K, Research Article

Zhengqiang Cao, Fang Hu, Yunpeng Chu, Jiaxue Pei, Xin-Ping Hui
A novel N-heterocyclic carbene-catalyzed asymmetric [4 + 2] annulation of in situ generated oxindole-embedded o-quinone methides with aldehydes has been developed for the assembly of complicated spirooxindoles. The methodology provides...
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Org. Chem. Front., 2024, Advance Article
DOI: 10.1039/D4QO00368C, Research Article

Jia-Hao Shen, Yong-Jie Long, Min Shi, Yin Wei
A palladium-catalyzed and ligand-controlled divergent synthesis of spiro-cyclohexadienones from p-quinone methides and VDCP-diesters was realized via zwitterionic π-propargyl palladium species and the mechanism was clarified by DFT calculations.
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Org. Chem. Front., 2024, Advance Article
DOI: 10.1039/D4QO00411F, Research Article

Lulu Liu, Jiaqi Hou, Yingying Ma, Hongwei Wang, Yu Zhong, Fangcan Liang, Luyao Wang, Qingling Wang, Ji-Quan Liu, Wen-Hua Xu, Dianhu Zhu
Selective reductive disulfuration of alkyl halides with di/trithiosulfonate reagents was developed through ligand regulation, with key features of broad substrate scope, good tolerance and excellent selectivity to disulfides over trisulfides.
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Org. Chem. Front., 2024, Advance Article
DOI: 10.1039/D4QO00412D, Research Article

Chengbo Li, Yu Guo, Jianke Su, Xinyuan Hu, Qingqing Xuan, Qiuling Song
A deaminative functionalization of aliphatic tertiary amines via the cleavage of C(sp³)–N bonds under transition metal-free conditions was disclosed, which goes through S_N2 reaction with various phosphorus and sulfur nucleophiles.
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Org. Chem. Front., 2024, Advance Article
DOI: 10.1039/D4QO00481G, Research Article

Jia-Chen Xiang, Yu-Die Wang, Peng Yuan, Hui-Min Zhu, Tong Lei, An-Xin Wu, Zhixin Liao
Three typical substrates for the Mannich reaction, p-anisidine, aldehyde, and a nucleophile, did not afford the predictable linear Mannich base under an aerobic copper oxidation condition, but rendering a 2,2-disubstituted indolin-3-one product.
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Org. Chem. Front., 2024, Advance Article
DOI: 10.1039/D4QO00322E, Research Article

Zhi Yang, Shangxian Luan, Linxi Wan, Jingxi Chen, Xiaofang Wei, Pei Tang, Fen-Er Chen
An iridium-catalyzed asymmetric hydrogenation of 2-esteryl-5-hydroxypyridinium salts is reported, providing chiral cis-5-hydroxypiperidine-2-carboxylates in excellent yields with high levels of enantioselectivities and diastereoselectivities.
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Energy Environ. Sci., 2024, Accepted Manuscript
DOI: 10.1039/D4EE04370G, Paper

Zezhou Lin, Yiran Ying, Zhihang Xu, Gao Chen, Xi Gong, Zehua Wang, Daqin Guan, Leqi Zhao, Mingyang Yang, Ke Fan, Tiancheng Liu, Hao LI, Honglei Zhang, Huangxu Li, Xi Zhang, Ye Zhu, Zhou-Guang Lu, Zongping Shao, Peiyu Hou, Haitao Huang
Increasing upper cut-off voltage is a useful way for enhancing specific capacity of LiCoO₂ (LCO) cathode and the energy density of corresponding lithium-ion batteries (LIBs), while the main challenge is...
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J. Mater. Chem. A, 2024, 12,8689-8693
DOI: 10.1039/D3TA07506K, Communication

Quanxiao Peng, Dandan Xing, Liuqi Dong, Yuhan Fu, Jixue Lu, Xiaoyu Wang, Changhong Wang, Chunxian Guo
An amorphous oxidized copper (a-O–Cu) is designed to investigate for electrochemical nitrate reduction to ammonia. It is found that a-O–Cu has high capability for water dissociation and amorphous structure-enabled high catalytic activity.
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J. Mater. Chem. A, 2024, 12,9212-9231
DOI: 10.1039/D3TA06821H, Paper

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Dilli babu Padmanaban, Paul Maguire, Davide Mariotti
We demonstrate the synthesis of zinc oxide (ZnO) nanoscale tetrapods (nTPs) using an atmospheric pressure microplasma with a metal wire as a sacrificial electrode.
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J. Mater. Chem. A, 2024, Advance Article
DOI: 10.1039/D4TA00237G, Paper

Sanjit Mondal, Gabriel Mark, Ayelet Tashakory, Michael Volokh, Menny Shalom
A polymeric carbon nitride layer with controlled directionality, morphology, and nitrogen defects serves as a photoanode to allow photoelectrochemical (PEC) water-splitting and benzylamine oxidation.
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J. Mater. Chem. A, 2024, Advance Article
DOI: 10.1039/D4TA00580E, Paper

Gang Li, Fulong Hu, Jinxiu Chen, Xiaozhong Fan, Xiong Xiao, Longtao Ma, Long Kong
A pre-polarized ion channels are constructed to inhibit the tip effect and selectively accelerate ion transport, achieving stable and uniform ion deposition, suppressing dendrite growth and side reaction for long-term Zn striping/plating.
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J. Mater. Chem. A, 2024, 12,9247-9247
DOI: 10.1039/D4TA90071E, Retraction

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Mojtaba Mahyari, Ahmad Shaabani
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J. Mater. Chem. A, 2024, Accepted Manuscript
DOI: 10.1039/D3TA07365C, Paper

Yifan Huang, Shihan Liu, Bo Wang, Ying Wang, Yifan Zhang, Pengyang Deng
In this paper, the aggregation effect between oligomeric Ir photosensitizers on photocatalytic hydrogen evolution was first discovered and investigated. Four oligomeric Ir photosensitizers were synthesized by copolymerization of [Ir(ppy)2(dabpy)](PF6) (H1)...
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J. Mater. Chem. A, 2024, Accepted Manuscript
DOI: 10.1039/D4TA00619D, Paper

Xiaoqi Jiang, Shengdong Sun, Yuqiao Wang, Lebing Zhao, Fangzhi Huang, Shikuo Li
Regulating charge transfer is a great challenge to improving the efficiency of piezoelectric photocatalytic reactions. Herein, sandwich-like Bi2WO6@Ag/MXene nanoflower spheres (BWO@Ag/MXene) with piezoelectric/plasma dual characteristics were synthesized by a facile...
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J. Mater. Chem. A, 2024, Accepted Manuscript
DOI: 10.1039/D4TA00415A, Paper

Yiming Yang, Jiachen Lu, Xinyu Zhang, Yanuo Shi, Peng Du, Xiao Ling, Nan Yang, Qianli Chen
Y-doped Ba(Zr,Ce)O₃ (BZCY) proton conducting ceramics have attracted extensive attention for their promising applications as electrolytes for intermediate-temperature proton ceramic electrochemical cells. The proton conductivity of BZCY is governed by...
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J. Mater. Chem. A, 2024, Accepted Manuscript
DOI: 10.1039/D4TA01230E, Paper

Guihong Mao, Liming Zeng, Jieyu Yang, Tengyu Yao, Fanming Xiao, Renheng Tang, Xin Shu, Ying Wang, Laifa Shen
Due to with high specific capacity, high nickel layered oxides have been at the forefront of the development of high-energy density lithium-ion batteries. However, high nickel cathodes invariably suffer from...
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J. Mater. Chem. A, 2024, Accepted Manuscript
DOI: 10.1039/D4TA00629A, Paper

Xintao Long, Yizhou Liu, Dongxin Wang, Yihang Nie, Xiaoyong Lai, Dan Luo, Xin Wang
Zinc ion batteries are expected to be the next generation of rechargeable aqueous metal ion batteries, but their application is limited by its severe dendrite growth caused by inhomogeneous plating...
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J. Mater. Chem. A, 2024, Accepted Manuscript
DOI: 10.1039/D4TA00586D, Paper

Sagar Varangane, Ragunath Madhu, Saad Mehmood, Bhavya Jaksani, Vidha Bhasin, Moses Abraham Abraham Bokinala, Ammavasi Nagaraj, Chandra Shobha Vennapoosa, Venkata Subba Reddy Basireddy, Subrata Kundu, Ujjwal Pal
Developing acid-stable oxygen evolution/reduction reaction (OER/ORR) electrocatalysts is essential for high-performance water splitting. Still, the slow kinetics of the ORR and OER during the discharge and charge processes seriously impede...
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J. Mater. Chem. A, 2024, Advance Article
DOI: 10.1039/D3TA07984H, Paper

Jian-an Chen, Xuejun Hou, Xueli Wang, Chunxia Wang, Jiawei Wen, Yongjie Bu, Guoyong Huang, Tiantian Cao, Shengming Xu
Operating principle of aqueous zinc-ion batteries (ZIBs).
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J. Mater. Chem. A, 2024, Advance Article
DOI: 10.1039/D4TA01240B, Paper

Qiong Wan, Jiaxun Zhang, Xuan Liu, Huizhi Li, Abdullah, Taotao Ren, Qiyuan Liu, Yongheng Xu, Jia Liu, Jicheng Liu, Bingqing Yao, Yiyun Fang, Xinzhe Li, Chi He
Atomic restructuring in Pd/Fe₂O₃ catalysts weakens Pd binding to chemisorbed 4-aminophenylacetylene and hydrogen intermediates, boosting conversion and selectivity in 4-aminophenylacetylene semi-hydrogenation, surpassing Pd/C and other catalysts.
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J. Mater. Chem. A, 2024, Advance Article
DOI: 10.1039/D4TA00240G, Paper

Laijun Liu, Kaiyuan Chen, Dawei Wang, Manuel Hinterstein, Anna-Lena Hansen, Michael Knapp, Biaolin Peng, Xianran Xing, Yuanpeng Zhang, Jing Kong, Abhijit Pramanick, Mads Ry Vogel Jørgensen, Frederick Marlton
Local structure information of relaxor ferroelectrics is key to a clear understanding of their structure–property relationships. The size of polar nanoregions is determined based on the local atomic displacement and dielectric response.
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J. Mater. Chem. A, 2024, Accepted Manuscript
DOI: 10.1039/D4TA00618F, Paper

Chao Li, Lijiang Guan, Jin Zhang, Cheng Cheng, Zhaoqi Guo, Zhihong Tian, Li-Ming Yang, Shangbin Jin
Covalent triazine frameworks (CTFs) of designable nitrogen-rich structures, which can form Schottky Junction with Pt nanoparticles, have been extensively studied in photocatalysis. However, how to tune the interaction inside the...
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J. Mater. Chem. A, 2024, Accepted Manuscript
DOI: 10.1039/D4TA00416G, Paper

Bipul Sarkar, Bhanu Joshi, Omvir Singh, Ankit Agrawal, Neha Dhiman, Bhanu Prasad Vempatapu, Navin Gopinathan , Anjan Ray
Unlike coal, oil, or natural gas, waste cooking oil (WCO) acts as a renewable source of carbon. It can be converted into energy, fuels, and fine chemicals, instead of being...
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J. Mater. Chem. A, 2024, Advance Article
DOI: 10.1039/D4TA00300D, Paper

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Yujia Fan, Xiaopeng Liu, Nibagani Naresh, Yijia Zhu, Iman Pinnock, Tianlei Wang, Mingqing Wang, Ivan P. Parkin, Buddha Deka Boruah
Proposing a planar zinc-ion micro-capacitor, featuring battery type anode and supercapacitor type cathode to offer intermediate energy storage performance, boasting greater energy density than typical supercapacitors, superior power density compared to batteries, and minimal self-discharge rates.
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J. Mater. Chem. A, 2024, Advance Article
DOI: 10.1039/D4TA00524D, Paper

Tianfang Yang, Bingcheng Ge, XuPo Liu, Zunjie Zhang, Ye Chen, Yang Liu
A practical strategy is reported to design single-Fe atom decorated S/N-doped C (Fe SAs@S/N–C) catalysts with a high Fe loading of 5.45 wt%. The prepared catalysts exhibit excellent performances for liquid and all-solid-state Zn–air batteries.
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J. Mater. Chem. A, 2024, Accepted Manuscript
DOI: 10.1039/D3TA06986A, Paper

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Antonija Ferbezar, Roman Zettl, Katharina Hogrefe, Harald Fitzek, Bernhard Gadermaier, Martin Wilkening, Ilie Hanzu
Solid-state ion conductors have improved significantly in the past decade. Envisioned applications range from metal anode batteries and fuel cells to sensors and medical technologies. The choice of solid electrolytes...
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J. Mater. Chem. A, 2024, Accepted Manuscript
DOI: 10.1039/D4TA00754A, Paper

Wei Guan, Lin Zhang, Peng Wang, Ying Wang, Haoyu Wang, Xingchen Dong, Liyan Yu, Zhixing Gan, Lifeng Dong, Lina Sui
The purposeful design and construction of two-dimensional (2D) semiconductor heterojunctions offers a promising avenue for achieving efficient photocatalytic activity. However, the challenge of enabling efficient charge migration at the interface...
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J. Mater. Chem. A, 2024, Advance Article
DOI: 10.1039/D4TA00649F, Paper

Lei Shi, Wenyue Zhao, Zhao Wang, Wenjing Hua, Xiaoxia Yang, Weidong Fei, Yu Zhao
The photovoltaic responses and temperature stabilities of A²⁺–Zr⁴⁺ (A = Ca, Sr, Ba) composite doped BiFeO₃ films with self-polarization were enhanced in the R to M_A phase transition.
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J. Mater. Chem. A, 2024, Advance Article
DOI: 10.1039/D4TA00665H, Paper

Shiyu Zhang, Yibing Peng, Mengna Wu, Qinghai Li, Yanguo Zhang, Hui Zhou
CO₂ gasification-reforming facilitates CO₂ utilization and yields CO-rich syngas for municipal waste management. Catalysts are essential for enhancing syngas production via catalytic tar reforming.
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J. Mater. Chem. A, 2024, Accepted Manuscript
DOI: 10.1039/D4TA01713G, Paper

Zeyad M. Abdulhamid, Abhishek C. Lokhande, Adewale Hammed Pasanaje, Daniel S Choi, Nirpendra Singh, Kyriaki Polychronopoulou, Dalaver H. Anjum
Few-layer two-dimensional (2D) molybdenum disulfide (MoS2) has great potential in designing high-performance supercapacitors due to its high theoretical specific capacity, tunable bandgap, and fascinating 2D layered structure. However, the lack...
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J. Mater. Chem. A, 2024, Advance Article
DOI: 10.1039/D4TA01549E, Paper

Ying Luo, Da Lei, Maohua Li, Yuansheng Ge, Jiguang Li, Baiyi Zu, Jun Yao, Xincun Dou
Metal organic frameworks (MOFs) have made great progress in the field of fluorescent sensing; however, whether the electronic structure and recognized sites can be adjusted by external functionalization still remains challenging.
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J. Mater. Chem. A, 2024, Accepted Manuscript
DOI: 10.1039/D4TA01884B, Paper

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Xue Jia, Hao Li
Low-cost metal oxides have emerged as promising candidates used as electrocatalysts for oxygen reduction reaction (ORR) due to their remarkable stability under oxidizing conditions, particularly in alkaline media. Recent studies...
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J. Mater. Chem. A, 2024, Accepted Manuscript
DOI: 10.1039/D4TA01317D, Paper

Zihan Wang, Yue Sun, Shenglong Wang, Da Xiong, Guo Tian, Longchao Huang, Boling Lan, Long Jin, Weiqing Yang, Weili Deng
ZnO is a performance-rich material due to its unique coupling of piezoelectricity and semiconductor properties. However, the intrinsic piezoelectric screening effect of ZnO weakens the electromechanical conversion efficiency and greatly...
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J. Mater. Chem. A, 2024, Advance Article
DOI: 10.1039/D4TA01191K, Paper

Xiubo Zhang, Chang Yu, Yuanyang Xie, Jinhe Yu, Yingbin Liu, Yi Yang, Jianjian Wang, Shuqin Lan, Siyi Hou, Kunlun Liu, Jieshan Qiu
The effective specific surface area is proposed and well correlated with Zn²⁺ storage, guiding maximum Zn²⁺ storage within carbon. Multiple in situ spectroscopy techniques clarify the co-adsorption mechanism of hydrated Zn²⁺, SO₄²⁻, and H⁺.
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J. Mater. Chem. C, 2024, Advance Article
DOI: 10.1039/D4TC03506B, Paper

Wenping Hu, Nan Wu, Dechao Li, Yefang Yang, Shaowen Qie, Shuai Su, Ruijie Xu, Wenting Li, Ming Hu
A Zn coordination polymer was constructed to identify chiral cinchonine and cinchonidine with high sensitivity, selectivity, and reproducibility.
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J. Mater. Chem. C, 2024, Accepted Manuscript
DOI: 10.1039/D4TC04013A, Paper

Mahdi Gassara, Jose Garcés-Garcés, Luis Lezama, Javier Ortiz, Fernando Fernandez-Lazaro, Samrana Kazim, Angela Sastre-Santos, Shahzada Ahmad
We synthesized molecular hole-transporting materials (HTMs) featuring a zinc phthalocyanine (ZnPc) central core and modulated the non-perypheral position with different numbers of tert-butyl groups. The synthesized molecules were also integrated...
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Chem. Sci., 2024, Accepted Manuscript
DOI: 10.1039/D4SC06723A, Edge Article

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Doyoung Kim, Hyewon Ju, Wooseok Lee, Sungwoo Hong
Cyclopropanes, valuable C3 building blocks in organic synthesis, possess high strain energy and inherent stability. We present an efficient, environmentally benign 1,3-oxyheteroarylation of aryl cyclopropanes using azine N-oxides as bifunctional...
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